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Time resolved measurements provide a new way to disentangle complex interactions in quantum materials due to their different timescales. We used pump-probe Raman scattering to investigate the apical oxygen vibration in…

Superconductivity · Physics 2021-12-07 N. Pellatz , S. Roy , J-W. Lee , J. L. Schad , H. Kandel , N. Arndt , C. B. Eom , A. F. Kemper , D. Reznik

In the past decade, the advent of time-resolved spectroscopic tools has provided a new ground to explore fundamental interactions in solids and to disentangle degrees of freedom whose coupling leads to broad structures in the frequency…

Time and angular resolved photoelectron spectroscopy is a powerful technique to measure electron dynamics in solids. Recent advances in this technique have facilitated band and energy resolved observations of the effect that excited…

Materials Science · Physics 2020-09-30 Umberto De Giovannini , Hannes Hübener , Shunsuke A. Sato , Angel Rubio

Ultrafast spectroscopies have become an important tool for elucidating the microscopic description and dynamical properties of quantum materials. In particular, by tracking the dynamics of non-thermal electrons, a material's dominant…

Time- and angle-resolved photoemission spectroscopy (TR-ARPES) accesses the electronic structure of solids under optical excitation, and is a powerful technique for studying the coupling between electrons and collective modes. One approach…

Relaxation of electrons in a Hubbard model coupled to a dissipative bosonic bath is studied to simulate the pump-probe photoemission measurement. From this insight, we propose an experimental method of eliciting unoccupied part of the…

Strongly Correlated Electrons · Physics 2016-08-15 Youhei Yamaji , Masatoshi Imada

Understanding the interaction of charge carriers with lattice vibrations in the quasi-equilibrium regime is crucial for semiconductor functionality. However, the structural signatures of these interactions are often too subtle for…

Materials Science · Physics 2026-03-11 Guy Reuveni , Maya Levy Greenberg , Matan Menahem , Olle Hellman , Omer Yaffe

Oscillatory signals from coherently excited phonons are regularly observed in ultrafast pump-probe experiments on condensed matter samples. Electron-phonon coupling implies that coherent phonons also modulate the electronic band structure.…

We study the role of excited phonon populations in the relaxation rates of nonequilibrium electrons using a nonequilibrium Green's function formalism. The transient modifications in the phononic properties are accounted for by…

Strongly Correlated Electrons · Physics 2018-12-12 O. Abdurazakov , D. Nevola , A. Rustagi , J. K. Freericks , D. B. Dougherty , A. F. Kemper

The coupling between quasiparticles and bosonic excitations rules the energy transfer pathways in condensed matter systems. The possibility of inferring the strength of specific coupling channels from their characteristic time scales…

Comprehending nonequilibrium electron-phonon dynamics at the microscopic level and at the short time scales is one of the main goals in condensed matter physics. Effective temperature models and time-dependent Boltzmann equations are…

Materials Science · Physics 2023-08-07 Nina Girotto , Fabio Caruso , Dino Novko

Despite their fundamental role in determining material properties, detailed momentum-dependent information on the strength of electron-phonon and phonon-phonon coupling (EPC and PPC, respectively) across the entire Brillouin zone (BZ) has…

Recent advancements in ultrafast laser systems and high harmonic generation (HHG) techniques have enabled time-resolved photoemission spectroscopy on femtosecond timescales, opening up unprecedented opportunities to explore quantum…

Strongly Correlated Electrons · Physics 2025-11-03 Takeshi Suzuki , Kozo Okazaki

We present an exact Monte Carlo method to simulate the nonequilibrium dynamics of electron-phonon models in the adiabatic limit of zero phonon frequency. The classical nature of the phonons allows us to sample the equilibrium phonon…

Strongly Correlated Electrons · Physics 2022-02-16 Manuel Weber , James K. Freericks

The non-equilibrium dynamics of matter excited by light may produce electronic phases that do not exist in equilibrium, such as laser-induced high-transition-temperature superconductivity. Here we simulate the dynamics of a metal driven at…

Strongly Correlated Electrons · Physics 2022-12-05 John Sous , Benedikt Kloss , Dante M. Kennes , David R. Reichman , Andrew J. Millis

The probing of coherent lattice vibrations in solids has been conventionally carried out using time-resolved transient spectroscopy where only the relative oscillation amplitude can be obtained. Using time-resolved X-ray techniques,…

Mesoscale and Nanoscale Physics · Physics 2024-03-25 Jicai Zhang , Ziwen Wang , Frank Lengers , Daniel Wigger , Doris E. Reiter , Tilmann Kuhn , Hans Jakob Wörner , Tran Trung Luu

We review recent work on the theory for pump/probe photoemission spectroscopy of electron-phonon mediated superconductors in both the normal and the superconducting states. We describe the formal developments that allow one to solve the…

Superconductivity · Physics 2017-10-11 A. F. Kemper , M. A. Sentef , B. Moritz , T. P. Devereaux , J. K. Freericks

In time-resolved photoemission experiments, more than one electron can be emitted from the solid by a single ultra-short pulse. We theoretically demonstrate how correlations between the momenta of outgoing electrons relate to time-dependent…

Strongly Correlated Electrons · Physics 2019-06-26 Christopher Stahl , Martin Eckstein

Quantitative knowledge of electron-phonon coupling is important for many applications as well as for the fundamental understanding of nonequilibrium relaxation processes. Time-resolved diffraction provides direct access to this knowledge…

Materials Science · Physics 2021-11-18 Daniela Zahn , Hélène Seiler , Yoav William Windsor , Ralph Ernstorfer

The spectral response and physical features of the 2D Hubbard-Holstein model are calculated both in equilibrium at zero and low chemical dopings, and after an ultra short powerful light pulse, in undoped systems. At equilibrium and at…

Strongly Correlated Electrons · Physics 2015-06-05 G. De Filippis , V. Cataudella , E. A. Nowadnick , T. P. Devereaux , A. S. Mishchenko , N. Nagaosa
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