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We propose a free-energy-perturbation approach accelerated by machine-learning potentials to efficiently compute transition temperatures and entropies for all rungs of Jacob's ladder. We apply the approach to the dynamically stabilized…

Materials Science · Physics 2025-05-05 Axel Forslund , Jong Hyun Jung , Yuji Ikeda , Blazej Grabowski

A classical thermometer typically works by exchanging energy with the system being measured until it comes to equilibrium, at which point the readout is related to the final energy state of the thermometer. A recent paper noted that…

Quantum Physics · Physics 2016-09-07 W. K. Tham , H. Ferretti , A. V. Sadashivan , A. M. Steinberg

Fluctuation theorems have become an important tool in single molecule biophysics to measure free energy differences from non-equilibrium experiments. When significant coarse-graining or noise affect the measurements, the determination of…

Statistical Mechanics · Physics 2016-03-09 Reinaldo García-García , Sourabh Lahiri , David Lacoste

We present a lattice Boltzmann algorithm based on an underlying free energy that allows the simulation of the dynamics of a multicomponent system with an arbitrary number of components. The thermodynamic properties, such as the chemical…

Soft Condensed Matter · Physics 2009-11-13 Qun Li , A. J. Wagner

Computing phase diagrams of model systems is an essential part of computational condensed matter physics. In this paper we discuss in detail the interface pinning (IP) method for calculation of the Gibbs free energy difference between a…

Statistical Mechanics · Physics 2015-10-26 Ulf R. Pedersen

The interfacial free energy between a crystal and a fluid, {\gamma} cf, is a highly relevant parameter in phenomena such as wetting or crystal nucleation and growth. Due to the difficulty of measuring {\gamma} cf experimentally, computer…

Statistical Mechanics · Physics 2015-06-23 J. R. Espinosa , C. Vega , E. Sanz

We develop a thermodynamic theory for machine learning (ML) systems. Similar to physical thermodynamic systems which are characterized by energy and entropy, ML systems possess these characteristics as well. This comparison inspire us to…

Machine Learning · Computer Science 2024-04-23 Dong Zhang

We investigate the thermalization of a stochastic system with discrete phase space, initially at equilibrium at temperature $T_i$ and then termalizing in an environment at temperature $T_f$ , considering both cases $T_i > T_f$ and $T_i <…

Statistical Mechanics · Physics 2025-08-05 A. Imparato

Simulated tempering (ST) has attracted a great deal of attention in the last years, due to its capability to allow systems with complex dynamics to escape from regions separated by large entropic barriers. However its performance is…

Statistical Mechanics · Physics 2015-08-11 A. Valentim , Cláudio J. daSilva , Carlos E. Fiore

We investigate how the temperature calculated from the microcanonical entropy compares with the canonical temperature for finite isolated quantum systems. We concentrate on systems with sizes that make them accessible to numerical exact…

Statistical Mechanics · Physics 2023-04-05 Phillip C. Burke , Masudul Haque

Low-temperature-differential (LTD) Stirling engines are heat engines that can operate autonomously with a slight temperature difference between low-temperature heat reservoirs and are thus expected to contribute to a sustainable society. A…

Adaptation and Self-Organizing Systems · Physics 2023-11-15 Songhao Yin , Hiroshi Kori , Yuki Izumida

A novel thermodynamic integration (TI) scheme is presented that allows computing the free energy of grain boundaries (GBs) in crystals from atomistic computer simulation. Unlike previous approaches, the method can be applied at arbitrary…

Statistical Mechanics · Physics 2018-09-12 Saswati Ganguly , Jürgen Horbach

Thermal sensation is crucial to enhancing our comprehension of the world and enhancing our ability to interact with it. Therefore, the development of thermal sensation presentation technologies holds significant potential, providing a novel…

Human-Computer Interaction · Computer Science 2023-10-24 Jiayi Xu , Shoichi Hasegawa , Kiyoshi Kiyokawa , Naoto Ienaga , Yoshihiro Kuroda

We examine in full generality the phase behavior of systems whose constituent particles interact by means of potentials which do not diverge at the origin, are free of attractive parts and decay fast enough to zero as the interparticle…

Soft Condensed Matter · Physics 2009-10-31 C. N. Likos , A. Lang , M. Watzlawek , H. Lowen

The Jarzynski equality (JE) provides a nonequilibrium method to measure and calculate the free energy difference (FED). Note that if two systems share the same Hamiltonian at two equilibrium states, respectively, they share the same FED…

Statistical Mechanics · Physics 2020-07-16 Liyun Zhu , Jiao Wang

Accurate measurement of efficiency for thermoelectric generator (TEG) is of great importance for materials research and development. Approximately all the parameters of a material are temperature dependent, so we can't directly apply the…

Materials Science · Physics 2016-06-08 Kumar Gaurav , Sudhir K Pandey

The thermoelectric figure of merit ZT, which is defined using electrical conductivity, Seebeck coefficient, thermal conductivity, and absolute temperature T, has been widely used as a simple estimator of the conversion efficiency of a…

Applied Physics · Physics 2020-05-18 Byungki Ryu , Jaywan Chung , Eun-Ae Choi , Pawel Ziolkowski , Eckhard Müller , SuDong Park

Melting properties are critical for designing novel materials, especially for discovering high-performance, high-melting refractory materials. Experimental measurements of these properties are extremely challenging due to their high melting…

Materials Science · Physics 2024-08-19 Li-Fang Zhu , Fritz Koermann , Qing Chen , Malin Selleby , Joerg Neugebauer , and Blazej Grabowski

This work builds on the previous introduction [1] of a coupled experimental-computational system devised to fully characterize the thermal behavior of complex 3D submicron electronic devices. The new system replaces the laser-based surface…

Materials Science · Physics 2007-09-13 Peter E. Raad , Pavel L. Komarov , M. Burzo

Simulation of warm dense matter requires computational methods that capture both quantum and classical behavior efficiently under high-temperature, high-density conditions. Currently, density functional theory molecular dynamics is used to…

Chemical Physics · Physics 2015-10-21 Attila Cangi , Aurora Pribram-Jones
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