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We report a single-crystal neutron diffraction study of the layered $\rm Sr_2IrO_4$. This work unambiguously determines the magnetic structure of the system and reveals that the spin orientation rigidly tracks the staggered rotation of the…

Strongly Correlated Electrons · Physics 2013-04-23 Feng Ye , Songxue Chi , Bryan C. Chakoumakos , Jaime A. Fernandez-Baca , Tongfei Qi , G. Cao

Single crystal neutron diffraction reveals two distinct components to the magnetic ordering in geometrically frustrated SrEr$_2$O$_4$. One component is a long-range ordered ${\bf k}=0$ structure which appears below $T_N = 0.75$ K. Another…

Strongly Correlated Electrons · Physics 2014-08-15 T. J. Hayes , G. Balakrishnan , P. P. Deen , P. Manuel , L. C. Chapon , O. A. Petrenko

A complete structural solution of the bilayer iridate compound Sr3Ir2O7 presently remains outstanding. Previously reported structures for this compound vary and all fail to explain weak structural violations observed in neutron scattering…

Strongly Correlated Electrons · Physics 2016-04-22 Tom Hogan , Lars Bjaalie , Liuyan Zhao , Carina Belvin , Xiaoping Wang , Chris G. Van de Walle , David Hsieh , Stephen D. Wilson

By means of neutron scattering techniques we have investigated the frustrated pyrochlore magnet Ho_2Sn_2O_7, which was found to show a ferromagnetic spin-ice behavior below T \simeq 1.4 K by susceptibility measurements. High-resolution…

Disordered Systems and Neural Networks · Physics 2007-05-23 Hiroaki Kadowaki , Yoshinobu Ishii , Kazuyuki Matsuhira , Yukio Hinatsu

Through a neutron scattering, charge transport, and magnetization study, the correlated ground state in the bilayer iridium oxide Sr$_3$Ir$_2$O$_7$ is explored. Our combined results resolve scattering consistent with a high temperature…

We report on the properties of SrTb2O4, a frustrated zigzag ladder antiferromagnet, studied by single crystal neutron diffraction (with polarised neutrons in zero field and unpolarised neutrons in an applied magnetic field), as well as by…

The nature of insulating phase in 5$d$ based Sr$_2$IrO$_4$ is quite debated as the theoretical as well as experimental investigations have put forward evidences in favor of both magnetically driven Slater-type and interaction driven…

Strongly Correlated Electrons · Physics 2017-02-08 Imtiaz Noor Bhatti , A. K. Pramanik

We report a comprehensive neutron diffraction study of the crystal structure and magnetic order in a series of single-crystal and powder samples of SrFeO$_{3-\delta}$ in the vacancy range $0 \leq \delta \leq 0.23$. The data provide detailed…

Strongly Correlated Electrons · Physics 2015-06-05 M. Reehuis , C. Ulrich , A. Maljuk , Ch. Niedermayer , B. Ouladdiaf , A. Hoser , T. Hofmann , B. Keimer

Neutron diffraction has been used to investigate the magnetic correlations in single crystals of the spin ice materials Ho2Ti2O7 and Dy2Ti2O7 in an external magnetic field applied along either the [001] or [1-10] crystallographic…

Other Condensed Matter · Physics 2009-11-11 T. Fennell , O. A. Petrenko , B. Fak , J. S. Gardner , S. T. Bramwell , B. Ouladdiaf

Neutron diffraction and inelastic spectroscopy is used to characterize the magnetic Hamiltonian of SrHo2O4 and SrDy2O4. Through a detailed computation of the crystal-field levels we find site- dependent anisotropic single-ion magnetism in…

This report presents azimuthal dependent and polarisation dependent x-ray resonant magnetic scattering at the Ir L3 edge for the bilayered iridate compound, Sr3Ir2O7. Two magnetic wave vectors, k1=(1/2,1/2,0) and k2=(1/2,-1/2,0), result in…

Strongly Correlated Electrons · Physics 2012-08-31 S. Boseggia , R Springell , H C Walker , A T Boothroyd , D Prabhakaran , S P Collins , D F McMorrow

Time-of-flight inelastic neutron scattering measurements on Sr2IrO4 single crystals were performed to access the spin Hamiltonian in this canonical Jeff=1/2 spin-orbital Mott insulator. The momentum of magnetic scattering at all inelastic…

Strongly Correlated Electrons · Physics 2018-12-12 S. Calder , D. M. Pajerowski , M. B. Stone , A. F. May

Using Raman spectroscopy to study the correlated 4$d$-electron metal Sr$_2$RhO$_4$, we observe pronounced excitations at 220 meV and 240 meV with $A_\mathrm{1g}$ and $B_\mathrm{1g}$ symmetries, respectively. We identify them as transitions…

A rare combination of strong spin-orbit coupling and electron-electron correlations makes the iridate Mott insulator Sr$_2$IrO$_4$ a promising host for novel electronic phases of matter. The resemblance of its crystallographic, magnetic and…

Strongly Correlated Electrons · Physics 2016-01-11 L. Zhao , D. H. Torchinsky , H. Chu , V. Ivanov , R. Lifshitz , R. Flint , T. Qi , G. Cao , D. Hsieh

By performing time-of-flight neutron scattering measurements on a large amount of single crystals of Sr$_2$RuO$_4$, we studied detailed structure of the imaginary part of the dynamic spin susceptibility over a wide range of phase space. In…

Strongly Correlated Electrons · Physics 2015-05-28 K. Iida , M. Kofu , N. Katayama , J. Lee , R. Kajimoto , Y. Inamura , M. Nakamura , M. Arai , Y. Yoshida , M. Fujita , K. Yamada , S. -H. Lee

Sr2IrO4 is a prototype of the class of Mott insulators in the strong spin-orbit interaction (SOI) limit described by a $J_{\mathrm{eff}}=1/2$ ground state. In Sr2IrO4, the strong SOI is predicted to manifest itself in the slaving of the…

Strongly Correlated Electrons · Physics 2013-09-30 S. Boseggia , H. C. Walker , J. Vale , R. Springell , Z. Feng , M. Moretti Sala , H. M. Rønnow , S. P. Collins , D. F. McMorrow

We report a neutron scattering study of the metallic triangular lattice antiferromagnet PdCrO$_2$. Powder neutron diffraction measurements confirm that the crystalline space group symmetry remains $R\bar{3}m$ below $T_N$. This implies that…

The antiferromagnetic structure of Sr3Ir2O7, the bilayer analogue of a spin-orbital Mott insulator Sr2IrO4, was revealed by resonant magnetic x-ray diffraction. Contrasting intensities of the magnetic diffraction at the Ir LIII and LII…

Strongly Correlated Electrons · Physics 2015-06-05 Shigeki Fujiyama , K. Ohashi , H. Ohsumi , K. Sugimoto , T. Takayama , T. Komesu , M. Takata , T. Arima , H. Takagi

We address the concomitant metal-insulator transition (MIT) and antiferromagnetic ordering in the novel pyrochlore iridate Eu2Ir2O7 by combining x-ray absorption spectroscopy, x-ray and neutron diffractions and density functional theory…

We have used Raman scattering to investigate the magnetic excitations and lattice dynamics in the prototypical spin-orbit Mott insulators Sr2IrO4 and Sr3Ir2O7. Both compounds exhibit pronounced two-magnon Raman scattering features with…

Strongly Correlated Electrons · Physics 2016-04-06 H. Gretarsson , N. H. Sung , M. Hoeppner , B. J. Kim , B. Keimer , M. Le Tacon
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