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Assuming Gaussian chain statistics along the chain contour, we generate by means of a proper fractal generator hyperbranched polymer trees which are marginally compact. Static and dynamical properties, such as the radial intrachain pair…

Soft Condensed Matter · Physics 2022-02-01 M. Dolgushev , J. P. Wittmer , A. Johner , O. Benzerara , H. Meyer , J. Baschnagel

We elucidate the elastic behavior of a wormlike chain in 3D under compression and provide exact solutions for the experimentally accessible force-extension relation in terms of generalized spheroidal wave functions. In striking contrast to…

Soft Condensed Matter · Physics 2019-11-11 Christina Kurzthaler

We present exact and analytically accurate results for the problem of a flexible polymer chain in shear flow. Under such a flow the polymer tumbles, and the probability distribution of the tumbling times $\tau$ of the polymer decays…

Statistical Mechanics · Physics 2008-11-13 Dibyendu Das , Sanjib Sabhapandit

The Hamiltonian dynamics of chains of nonlinearly coupled particles is numerically investigated in two and three dimensions. Simple, off-lattice homopolymer models are used to represent the interparticle potentials. Time averages of…

Statistical Mechanics · Physics 2007-05-23 Alessandro Mossa , Marco Pettini , Cecilia Clementi

We develop a continuum elastic approach to examining the bending mechanics of semiflexible filaments with a local internal degree of freedom that couples to the bending modulus. We apply this model to study the nonlinear mechanics of a…

Soft Condensed Matter · Physics 2013-02-12 Arthur A. Evans , Alex J. Levine

Polymers exposed to shear flow exhibit a rich tumbling dynamics. While rigid rods rotate on Jeffery orbits, flexible polymers stretch and coil up during tumbling. Theoretical results show that in both of these asymptotic regimes the…

Soft Condensed Matter · Physics 2014-05-27 Philipp S. Lang , Benedikt Obermayer , Erwin Frey

The properties of semiflexible polymers tethered by one end to an impenetrable wall and exposed to oscillatory shear flow are investigated by mesoscale simulations. A polymer, confined in two dimensions, is described by a linear bead-spring…

Soft Condensed Matter · Physics 2021-12-14 Antonio Lamura , Roland G. Winkler , Gerhard Gompper

We show using Brownian dynamics simulations and theory how the shear relaxation modulus G(t) of dilute solutions of relatively stiff semiflexible polymers differs qualitatively from that of rigid rods. For chains shorter than their…

Soft Condensed Matter · Physics 2009-10-31 Matteo Pasquali , V. Shankar , David C. Morse

Active polymers play a central role in many biological systems, from bacterial flagella to cellular cytoskeletons. Minimal models of semiflexible active filaments have been used to study a variety of interesting phenomena in active systems,…

Soft Condensed Matter · Physics 2020-02-19 Matthew S. E. Peterson , Michael F. Hagan , Aparna Baskaran

Conformations of partially or fully adsorbed semiflexible polymer chains are studied varying both contour length $L$, chain stiffness, $\kappa$, and the strength of the adsorption potential over a wide range. Molecular Dynamics simulations…

Soft Condensed Matter · Physics 2019-10-02 Andrey Milchev , Kurt Binder

We revisit a model of semiflexible Gaussian chains proposed by Winkler \textit{et al}, solve the dynamics of the discrete description of the model and derive exact algebraic expressions for some of the most relevant dynamical observables,…

Soft Condensed Matter · Physics 2022-11-02 Andres R. Tejedor , Jaime R. Tejedor , Jorge Ramirez

Spurred by an experimental controversy in the literature, we investigate the end-monomer dynamics of semiflexible polymers through Brownian hydrodynamic simulations and dynamic mean-field theory. Precise experimental observations over the…

Soft Condensed Matter · Physics 2009-06-20 Michael Hinczewski , Xaver Schlagberger , Michael Rubinstein , Oleg Krichevsky , Roland R. Netz

We explore the elastic behavior of a wormlike chain under compression in terms of exact solutions for the associated probability densities. Strikingly, the probability density for the end-to-end distance projected along the applied force…

Soft Condensed Matter · Physics 2019-11-11 Christina Kurzthaler , Thomas Franosch

We derive the Frank elastic constants for nematic solutions of semiflexible polymers. We plot these results as a function of the coarse-grained Maier-Saupe quadrupole aligning strength and polymer stiffness ranging from rigid to highly…

Soft Condensed Matter · Physics 2022-07-18 Quinn MacPherson

The non-equilibrium structural and dynamical properties of semiflexible polymers confined to two dimensions are investigated by molecular dynamics simulations. Three different scenarios are considered: The force-extension relation of…

Soft Condensed Matter · Physics 2013-01-08 A. Lamura , R. G. Winkler

Synthetic copolymers and biopolymers, such as polypeptides and double-stranded DNA, often exhibit strong variations in bending stiffness along their contour, which can significantly impact conformational behavior at larger scales. To…

Soft Condensed Matter · Physics 2025-11-04 Yannick Witzky , Friederike Schmid , Arash Nikoubashman

The freely rotating chain is one of the classic discrete models of a polymer in dilute solution. It consists of a broken line of N straight segments of fixed length such that the angle between adjacent segments is constant and the N-1…

Probability · Mathematics 2017-11-15 Philip Kilanowski , Peter March , Marko Samara

Taking into account the nonequivalence of fixed-force and fixed-length ensembles in the weak-force regime, equations of state are derived that describe the equilibrium extension or compression of an ideal Gaussian polymer chain in response…

Soft Condensed Matter · Physics 2007-05-23 Richard M. Neumann

We consider a semiflexible polymer in $\mathbb Z^d$ which is a random interface model with a mixed gradient and Laplacian interaction. The strength of the two operators is governed by two parameters called lateral tension and bending…

Probability · Mathematics 2020-06-24 Alessandra Cipriani , Biltu Dan , Rajat Subhra Hazra

Using extensive computer simulations, the behavior of the structural modes --- more precisely, the eigenmodes of a phantom Rouse polymer --- are characterized for a polymer in the three-dimensional repton model, and are used to study the…

Soft Condensed Matter · Physics 2015-03-18 Gerard T. Barkema , Debabrata Panja , J. M. J. van Leeuwen