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When a pulse of light traverses a material, it incurs a time delay referred to as the group delay. Should the group delay experienced by photons be attributed to the time they spend as atomic excitations? However reasonable this connection…

The photoionization of the CO molecule from the C$-1s$ orbital does not obey the Franck-Condon approximation, as a consequence of the nuclear recoil that accompanies the direct emission and intra-molecular scattering of the photoelectron.…

Atomic Physics · Physics 2021-11-24 Bejan Ghomashi , Nicolas Douguet , Luca Argenti

The time-dependent variational principle is used to optimize the linear and nonlinear parameters of Gaussian basis functions to solve the time-dependent Schrodinger equation in 1 and 3 dimensions for a one-body soft Coulomb potential in a…

We present experimental data on the strong-field ionization of the argon dimer in a co-rotating two-color (CoRTC) laser field. We observe a sub-cycle interference pattern in the photoelectron momentum distribution and infer the Wigner time…

The photoelectric effect, explained by Einstein in 1905, is often regarded as a one-electron phenomenon. However, in multi-electron systems, the interaction of the escaping electron with other electrons, referred to as electron correlation,…

This paper concerns the theory of non-recollisional ionization or detachment of atoms or ions by intense few-cycle pulses. It is shown that in certain conditions of pulse duration, peak intensity and carrier-envelope phase, the ionization…

Atomic Physics · Physics 2014-09-04 C. C. Chirila , R. M. Potvliege

We use the non-relativistic random phase approximation with exchange to perform calculations of valence shell photoionization of Ne, Ar, Kr and Xe from their respective thresholds to photon energy of 200 eV. The energy derivative of the…

Atomic Physics · Physics 2026-03-03 A. S. Kheifets

We analyze the electronic correlation contribution to the time delay in the photo-ionization of the excited ortho- and para-Helium states. A simple estimation, based on the ionization probability amplitudes, shows that the different form of…

Atomic Physics · Physics 2024-03-21 Pedro Sancho

Advances in ultra-intense laser technology are enabling, for the first time, relativistic intensities at mid-infrared (mid-IR) wavelengths. Anticipating further experimental research in this domain, we present high-resolution two…

A photoelectron forced to pass through two atomic energy levels before receding from the residual ion shows interference fringes in its angular distribution as manifestation of a two-slit-type interference experiment in wave-vector space.…

Quantum Physics · Physics 2019-07-16 Jonas Wätzel , Andrew James Murray , Jamal Berakdar

The X-ray radiation delay law dependence on the diffraction asymmetry parameters is analyzed. It is shown that the use of subpicosecond pulses allows to observe the time delay of pulse in crystal phenomenon and to investigate the delay law…

Optics · Physics 2007-05-23 Vladimir G. Baryshevsky

Photoelectron spectra obtained from the ab initio solution of the time-dependent Schr\"odinger equation can be in striking disagreement with predictions by the strong-field approximation (SFA) not only at low energy but also around twice…

Atomic Physics · Physics 2016-12-14 Th. Keil , S. V. Popruzhenko , D. Bauer

We propose a general technique to retrieve the information of dipole-forbidden resonances in the autoionizing region. In the simulation, a helium atom is pumped by an isolated attosecond pulse in the extreme ultraviolet (EUV) combined with…

Atomic Physics · Physics 2014-03-28 Wei-Chun Chu , Toru Morishita , C. D. Lin

Atmospheric pressure helium plasmas are investigated through molecular dynamics simulations at room temperature (300 K) for various ionization fractions ($\chi_i = 10^{-1} - 10^{-5}$) in the strongly coupled regime (ion coupling parameter,…

Plasma Physics · Physics 2024-10-24 Swati Swagatika Mishra , Pascal Brault , Sudeep Bhattacharjee

We theoretically study the photoelectron angular distributions (PADs) from two-color two-photon near-threshold ionization of hydrogen and noble gas (He, Ne, and Ar) atoms by a combined action of femtosecond extreme ultraviolet (EUV) and…

Atomic Physics · Physics 2015-06-22 Kenichi L. Ishikawa , A. K. Kazansky , N. M. Kabachnik , Kiyoshi Ueda

This is the first of two subsequent publications where the probability distribution of delay-times in scattering of wave packets is discussed. The probability distribution is expressed in terms of the on-shell scattering matrix, the…

Mathematical Physics · Physics 2017-05-24 Uzy Smilansky

A technique for measuring photoionization time delays with attosecond precision is combined with calculations of photoionization matrix elements to demonstrate how multi-electron dynamics affect photoionization time delays in carbon…

Digital camera pixels measure image intensities by converting incident light energy into an analog electrical current, and then digitizing it into a fixed-width binary representation. This direct measurement method, while conceptually…

Computer Vision and Pattern Recognition · Computer Science 2021-04-13 Atul Ingle , Trevor Seets , Mauro Buttafava , Shantanu Gupta , Alberto Tosi , Mohit Gupta , Andreas Velten

Free electrons in the interstellar medium cause frequency-dependent delays in pulse arrival times due to both scattering and dispersion. Multi-frequency measurements are used to estimate and remove dispersion delays. In this paper, we focus…

High Energy Astrophysical Phenomena · Physics 2015-06-23 M. T. Lam , J. M. Cordes , S. Chatterjee , T. Dolch

Saturable absorption is a nonlinear effect where a material's ability to absorb light is frustrated due to a high influx of photons and the creation of electron vacancies. Experimentally induced saturable absorption in copper revealed a…