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We have investigated second harmonic generation (SHG) from Ag-coated LiNbO3 (LN) core-shell nanocuboids and found that giant SHG can occur via deliberately designed double plasmonic resonances. By controlling the aspect ratio, we can tune…

Optics · Physics 2014-11-19 Ming-Liang Ren , Si-Yuan Liu , Ben-Li Wang , Bao-Qin Chen , Jiafang Li , Zhi-Yuan Li

Optical harmonic generation on excitons is found in ZnSe/BeTe quantum wells with type-II band alignment. Two experimental approaches with spectrally-broad femtosecond laser pulses and spectrally-narrow picosecond pulses are used for…

Nanogenerators based on ZnO nanowires (NWs) realize the energy conversion at nanoscale, which are ascribed to the piezoelectric property caused by the lattice distortion of the ZnO NWs. The lattice distortion can significantly tune the…

Optics · Physics 2016-08-01 Xiaobo Han , Kai Wang , Hua Long , Hongbo Hu , Jiawei Chen , Bing Wang , Peixiang Lu

This research will examine the computational methods to calculate the nonlinear optical process of second harmonic generation (SHG) that will be hypothesized to be present during lithium ion insertion into silicon nanowires. First it will…

Optics · Physics 2021-10-19 Donald C. Boone

Since the first observation of second harmonic generation (SHG), there have been extensive studies on this nonlinear phenomenon not only to clarify its physical origin but also to realize unconventional functionalities. Nonetheless, a…

We report the realization of Zinc Sulfide (ZnS) nanowaveguides and the experimental observation of second harmonic generation (SHG) in such structures, demonstrating their potential for integrated nonlinear photonics. ZnS thin films were…

Optical resonances in nanostructures enable strong enhancement of nonlinear processes at the nanoscale, such as second-harmonic generation (SHG), with high-$Q$ modes providing intensified light--matter interactions and sharp spectral…

This study presents an investigation of second harmonic generation (SHG) resulting from interaction of radially polarized laser beam propagating in homogeneous, unmagnetized plasma. Lorentz force and continuity equations have been used to…

Plasma Physics · Physics 2025-09-30 Shivani Aggarwal , Saumya Singh , Dinkar Mishra , Bhupesh Kumar , Pallavi Jha

The enhanced electric field at plasmonic resonances in nanoscale antennas can lead to efficient harmonic generation, especially when the plasmonic geometry is asymmetric on either inter-particle or intra-particle levels. The planar…

Second-harmonic generation (SHG) is a powerful surface-specific probe for centrosymmetric materials, with broad relevance to energy and biological interfaces. Plasmonic nanomaterials have been extensively utilized to amplify this nonlinear…

We develop a multipolar theory of second-harmonic generation (SHG) by dielectric nanoparticles made of noncentrosymmetric materials with bulk quadratic nonlinearity. We specifically analyze two regimes of optical excitation: illumination by…

We report on the optical second harmonic generation (SHG) on the 1S exciton-polariton resonance in bulk ZnSe that is subject to an external magnetic field applied perpendicular to the light wave vector $\mathbf k$ (Voigt geometry). For the…

Mesoscale and Nanoscale Physics · Physics 2025-07-18 J. Mund , D. R. Yakovlev , A. Farenbruch , N. V. Siverin , M. A. Semina , M. M. Glazov , E. L. Ivchenko , M. Bayer

Second harmonic generation is enhanced at the surface lattice resonance in plasmonic nanoparticle arrays. We carried out a parametric investigation on two-dimensional lattices composed of gold nanobars where the centrosymmetry is broken at…

Second-order nonlinearity gives rise to many distinctive physical phenomena, e.g., second-harmonic generation, which plays an important role in fundamental science and various applications. Lithium niobate, one of the most widely used…

The in-plane anisotropic properties of two-dimensional (2D) group IV monochalcogenides provide an additional degree of freedom which can be used in future optoelectronic devices. Here, it is shown that the third harmonic generation (THG)…

We show that optical second-harmonic generation (SHG) can be observed from individual single-walled carbon nanotubes (SWCNTs) and, furthermore, allows imaging of individual tubes. Detailed analysis of our results suggests that the…

We present a combined experimental and theoretical study of enhanced third-harmonic generation (THG) in silicon nitride metasurfaces. These structures exhibit strong resonant nonlinear responses, enabling up to two orders of magnitude…

High harmonic generation (HHG) is a powerful probe of electron dynamics on attosecond to femtosecond timescales and has been successfully used to detect electronic and structural changes in solid-state quantum materials, including…

Materials Science · Physics 2026-01-21 Daniel A. Rehn , Towfiq Ahmed , Jinkyoung Yoo , Rohit Prasankumar , Jian-Xin Zhu

We report observation of strongly enhanced surface SHG in BaTiO_3 due to excitation of a photorefractive surface electromagnetic wave. Surface SH intensity may reach 10^{-2} of the incident fundamental light intensity. Angular, crystal…

Materials Science · Physics 2009-10-31 Igor I. Smolyaninov , Chi H. Lee , Christopher C. Davis

The outstanding optical properties for plasmon resonances in noble metal nanoparticles enable the observation of non-linear optical processes such as second-harmonic generation (SHG) at the nanoscale. Here, we investigate the SHG process in…