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An obstacle for spin-based quantum sensors is magnetic noise due to proximal spins. However, such a spin cluster surrounding the sensor can become an asset, if it can be controlled. Here, we polarize and readout a cluster of three nitrogen…

Quantum Physics · Physics 2016-09-07 Helena S. Knowles , Dhiren M. Kara , Mete Atatüre

Electronic spins associated with the Nitrogen-Vacancy (NV) center in diamond offer an opportunity to study spin-related phenomena with extremely high sensitivity owing to their high degree of optical polarization. Here, we study both…

Quantum Physics · Physics 2023-07-03 Anand Patel , Zainab Chowdhry , Anil Prabhakar , A. Rathi , V. P. Bhallamudi

Nuclear spins in certain solids couple weakly to their environment, making them attractive candidates for quantum information processing and inertial sensing. When coupled to the spin of an optically-active electron, nuclear spins can be…

Quantum Physics · Physics 2022-11-11 Alexander A. Wood , Russell M. Goldblatt , Robert E. Scholten , Andy M. Martin

Dynamic nuclear polarization via contact with electronic spins has emerged as an attractive route to enhance the sensitivity of nuclear magnetic resonance (NMR) beyond the traditional limits imposed by magnetic field strength and…

Dynamic nuclear polarization (DNP) of molecules in a solution at room temperature has potential to revolutionize nuclear magnetic resonance spectroscopy and imaging. The prevalent methods for achieving DNP in solutions are typically most…

Chemical Physics · Physics 2016-03-02 Qiong Chen , Ilai Schwarz , Fedor Jelezko , Alex Retzker , Martin B Plenio

We report bulk, room-temperature hyperpolarization of 13C nuclear spins observed via high-field nuclear magnetic resonance (NMR). The hyperpolarization is achieved by optical pumping (OP) of nitrogen vacancy defect centers in diamond…

The electronic spins of the nitrogen-vacancy centers (NV centers) in Chemical-Vapor-Deposition (CVD) grown diamonds form ideal probes of magnetic fields and temperature, as well as promising qu-bits for quantum information processing.…

Quantum Physics · Physics 2021-03-31 C. Pellet-Mary , P. Huillery , M. Perdriat , A. Tallaire , G. Hétet

We report the detection and polarization of nuclear spins in diamond at room temperature by using a single nitrogen-vacancy (NV) center. We use Hartmann-Hahn double resonance to coherently enhance the signal from a single nuclear spin while…

Key to future spintronics and spin-based information processing technologies is the generation, manipulation, and detection of spin polarization in a solid state platform. Here, we theoretically explore an alternative route to spin…

Mesoscale and Nanoscale Physics · Physics 2014-07-29 Carlos A. Meriles , Marcus W. Doherty

Optically polarizable nitrogen-vacancy (NV) center in diamond enables the hyperpolarization of $^{13}$C nuclear spins at low magnetic field and room temperature. However, achieving a high level of polarization comparable to conventional…

Quantum Physics · Physics 2024-10-01 Vladimir V. Kavtanyuk , Changjae Lee , Keunhong Jeong , Jeong Hyun Shim

Efficient polarization of organic molecules is of extraordinary relevance when performing nuclear magnetic resonance (NMR) and imaging. Commercially available routes to dynamical nuclear polarization (DNP) work at extremely…

We experimentally investigate the protection of electron spin coherence of nitrogen vacancy (NV) center in diamond by dynamical nuclear polarization. The electron spin decoherence of an NV center is caused by the magnetic ield fluctuation…

Nitrogen-vacancy (NV) defect centers in diamond are strong candidates to generate entangled states in solid-state environments even at room temperature. Quantum correlations in spatially separated NV systems, for distances between NVs…

Other Condensed Matter · Physics 2018-08-09 Viviana Gómez Azuero , Ferney Rodríguez Dueñas , Luis Quiroga Puello

We report hyperpolarization of the electronic spins associated with substitutional nitrogen defects in bulk diamond crystal. Hyperpolarization is achieved by optical pumping of nitrogen vacancy centers followed by rapid cross relaxation at…

Mesoscale and Nanoscale Physics · Physics 2017-02-22 M. Loretz , H. Takahashi , T. F. Segawa , J. M. Boss , C. L. Degen

The negatively charged nitrogen-vacancy center in diamond is a prototype photoluminescent point defect spin qubit with promising quantum technology applications, enabled by its efficient optical spin polarization and readout. Its low-lying…

A promising approach for multi-qubit quantum registers is to use optically addressable spins to control multiple dark electron-spin defects in the environment. While recent experiments have observed signatures of coherent interactions with…

Efficient optical readout of a single, solid-state electronic spin at room temperature is a key challenge for nanoscale quantum sensing. Here we apply the technique of spin-to-charge conversion to enhance the optical spin-state readout of a…

Nitrogen-Vacancy (NV) centers in diamonds provide a room-temperature platform for various emerging quantum technologies, e.g. the long nuclear spin coherence times as potential quantum memory registers. We demonstrate a freezing protocol…

Quantum Physics · Physics 2023-08-14 Abhishek Kejriwal , Dasika Shishir , Sumiran Pujari , Kasturi Saha

Nitrogen vacancy (NV-) color centers in diamond are a prime candidate for use in quantum information devices, owing to their spin-1 ground state, straightforward optical initialization and readout, and long intrinsic coherence times in a…

Quantum Physics · Physics 2015-06-19 Anna J. Parker , Hai-Jing Wang , Yiran Li , Alexander Pines , Jonathan P. King

The interplay between disorder and transport is a problem central to the understanding of a broad range of physical processes, most notably the ability of a system to reach thermal equilibrium. Disorder and many body interactions are known…