Related papers: Rovibrational cooling of molecules by optical pump…
We demonstrate experimentally a method of all-optical selective rotational control in gas mixtures. Using an optical centrifuge - an intense laser pulse whose linear polarization rotates at an accelerated rate, we simultaneously excite two…
Interaction between light and molecular vibrations leads to hybrid light-matter states called vibrational polaritons. Even though many intriguing phenomena have been predicted for single-molecule vibrational strong coupling (VSC), several…
We report the operation of a $^{87}$Rb maser in the self-oscillating mode, using a laser diode as the optical pumping source. The maser uses a TE$_{021}$ cavity surrounding a cell containing the atoms and 11 Torr of N$_{2}$ as the buffer…
The formation of diatomic molecules with rotational and vibrational coherence is demonstrated experimentally in free-to-bound two-photon femtosecond photoassociation of hot atoms. In a thermal gas at a temperature of 1000 K, pairs of…
Circularly-polarized (CP) vibrations are the nuclear-motion analog of CP light, emerging in molecules with non-Abelian point-group symmetry that support orthogonal and degenerate vibrational normal modes. Here, we explore the optical…
Methods for controlling the motion of single particles, optically levitated in vacuum, have developed rapidly in recent years. The technique of cold damping makes use of feedback-controlled, electrostatic forces to increase dissipation…
Selectively exciting target molecules to high vibrational states is inefficient in the liquid phase, which restricts the use of IR pumping to catalyze ground-state chemical reactions. Here, we demonstrate that this inefficiency can…
The precise control and knowledge over the atomic dynamics is central to the advancement of quantum technology. The different experimental conditions namely, atoms in a vacuum, an anti-relaxation coated and a buffer gas filled atomic cell…
A pulsed cooling scheme for optomechanical systems is presented that is capable of cooling at much faster rates, shorter overall cooling times, and for a wider set of experimental scenarios than is possible by conventional methods. The…
Atoms in spatially dependent light fields are attracted to local intensity maxima or minima depending on the sign of the frequency difference between the light and the atomic resonance. For light fields confined in open high-Q optical…
We propose to introduce additional control in levitated optomechanics by trapping a meta-atom, i.e. a subwavelength and high-permittivity dielectric particle supporting Mie resonances. In particular, we theoretically demonstrate that…
Ultracold polar molecules are promising for quantum information processing and searches for physics beyond the Standard Model. Laser cooling to ultracold temperatures is an established technique for trapped diatomic and triatomic molecules.…
We report the observation of collective-emission-induced, velocity-dependent light forces. One third of a falling sample containing 3 x 10^6 cesium atoms illuminated by a horizontal standing wave is stopped by cooperatively emitting light…
Refrigeration of a solid-state system with light has potential applications for cooling small-scale electronics and photonics. We show theoretically that two coupled semiconductor quantum wells are efficient cooling media for optical…
Improved optical control of molecular quantum states promises new applications including chemistry in the quantum regime, precision tests of fundamental physics, and quantum information processing. While much work has sought to prepare…
We report on the implementation of degenerate Raman sideband cooling of $^{40}$K atoms. The scheme incorporates a 3D optical lattice, which confines the atoms and drives the Raman transitions. The optical cooling cycle is closed by two…
We study a single incoherently pumped atom moving within an optical high-Q resonator in the strong coupling regime. Using a semiclassical description for the atom and field dynamics, we derive a closed system of differential equations to…
We present efficient theoretical tools for describing the optical pumping of atoms by light propagating at arbitrary directions with respect to an external magnetic field, at buffer-gas pressures that are small enough for velocity-selective…
Following excitation by a strong ultra-short laser pulse, molecules develop coordinated rotational motion, exhibiting transient alignment along the direction of the laser electric field, followed by periodic full and fractional revivals…
Atomic-resolution-imaging approaches for single molecules, such as coherent x-ray diffraction at free-electron lasers, require the delivery of high-density beams of identical molecules. However, even very cold beams of biomolecules…