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Charged excitons, or X$^{\pm}$-trions, in monolayer transition metal dichalcogenides have binding energies of several tens of meV. Together with the neutral exciton X$^0$ they dominate the emission spectrum at low and elevated temperatures.…

We present a microscopic theory of neutral excitons and charged excitons (trions) in monolayers of transition metal dichalcogenides, including molybdenum disulfide. Our theory is based on an effective mass model of excitons and trions,…

Materials Science · Physics 2015-08-12 Timothy C. Berkelbach , Mark S. Hybertsen , David R. Reichman

The ultrathin transition metal dichalcogenides (TMDs) have emerged as promising materials for various applications using two dimensional (2D) semiconductors. They have attracted increasing attention due to their unique optical properties…

Mesoscale and Nanoscale Physics · Physics 2016-09-20 Aïda Hichri , Imen Ben Amara , Sabrine Ayari , Sihem Jaziri

The optical properties of semiconducting transition metal dichalcogenides are dominated by both neutral excitons (electron-hole pairs) and charged excitons (trions) that are stable even at room temperature. While trions directly influence…

Mesoscale and Nanoscale Physics · Physics 2016-07-26 Kai Hao , Lixiang Xu , Philipp Nagler , Akshay Singh , Kha Tran , Chandriker Kavir Dass , Christian Schüller , Tobias Korn , Xiaoqin Li , Galan Moody

We analyze the lineshape of the quasiparticle photoluminescence of monolayer and bilayer molybdenum ditelluride in temperature- and excitation intensity-dependent experiments. We confirm the existence of a negatively charged trion in the…

Monolayer transition metal dichalcogenides host a variety of optically excited quasiparticles species that stem from two-dimensional confinement combined with relatively large carrier effective masses and reduced dielectric screening. The…

Electric field-controlled, two-dimensional (2D) exciton dynamics in transition metal dichalcogenide monolayers is a current research focus in condensed matter physics. We have experimentally investigated the spectral and temporal properties…

Mesoscale and Nanoscale Physics · Physics 2019-12-11 Michael Engel , Mathias Steiner

Monolayers of semiconducting transition metal dichalcogenides are a strongly emergent platform for exploring quantum phenomena in condensed matter, building novel opto-electronic devices with enhanced functionalities. Due to their atomic…

We report charged exciton (trion) formation dynamics in doped monolayer transition metal dichalcogenides (TMDs), specifically molybdenum diselenide (MoSe2), using resonant two-color pump-probe spectroscopy. When resonantly pumping the…

Semiconducting Transition Metal Dichalcogenides (TMDs) have significant nonlinear optical effects. In this work we have used second-harmonic generation (SHG) and the four-wave mixing (FWM) spectroscopy in resonance with the excitons in…

We revisit low-temperature optical spectra of transition-metal dichalcogenide monolayers and point to a possible crystallization of electrons (or holes) at low to moderate charge densities. To calculate the excitonic spectra under such…

Mesoscale and Nanoscale Physics · Physics 2023-08-16 Dinh Van Tuan , Hanan Dery

The monolayers of semiconducting transition metal dichalcogenides host strongly bound excitonic complexes and are an excellent platform for exploring many-body physics. Here we demonstrate a controlled kinetic manipulation of the…

Mesoscale and Nanoscale Physics · Physics 2022-04-05 Suman Chatterjee , Sarthak Das , Garima Gupta , Kenji Watanabe , Takashi Taniguchi , Kausik Majumdar

One of the most striking features of novel 2D semiconductors (e.g., transition metal dichalcogenide monolayers or phosphorene) is a strong Coulomb interaction between charge carriers resulting in large excitonic effects. In particular, this…

Mesoscale and Nanoscale Physics · Physics 2015-11-18 Kirill A. Velizhanin , Avadh Saxena

The optical spectra of transition metal dichalcogenide (TMDC) monolayers are dominated by excitons and trions. Here we establish the dependences of these optical transitions on disorder from hyperspectral imaging of h-BN encapsulated…

Mesoscale and Nanoscale Physics · Physics 2022-12-13 Jue Wang , Christina Manolatou , Yusong Bai , James Hone , Farhan Rana , Xiaoyang Zhu

The optical emission spectra of semiconducting transition-metal dichalcogenide monolayers highlight fascinating recombination processes of charged excitons (trions). When charge tunable WSe$_2$ monolayers are moderately doped with…

Mesoscale and Nanoscale Physics · Physics 2025-01-22 V. Jindal , K. Mourzidis , A. Balocchi , C. Robert , P. Li , D. Van Tuan , L. Lombez , D. Lagarde , P. Renucci , T. Taniguchi , K. Watanabe , H. Dery , X. Marie

Multi-exciton states such as biexcitons, albeit theoretically predicted, have remained challenging to identify in atomically thin transition metal dichalcogenides so far. Here, we use excitation-power, electric-field and magnetic-field…

Exciton spectroscopy serves as a sensitive probe of electronic states in two-dimensional semiconductors. A prominent feature in optical spectra is the trion peak arising from the binding of a charge carrier to an exciton. The splitting…

Mesoscale and Nanoscale Physics · Physics 2025-07-23 Arthur Christianen , Atac Imamoglu

Monolayer transition metal dichalcogenide (TMDC) semiconductors exhibit strong excitonic optical resonances which serve as a microscopic, non-invasive probe into their fundamental properties. Like the hydrogen atom, such excitons can…

The possibility of almost linear tuning of the band gap and of the electrical and optical properties in monolayers (MLs) of semiconducting transition metal dichalcogenide (S-TMD) alloys opens up the way to fabricate materials with on-demand…

In the last decade atomically thin 2D materials have emerged as a perfect platform for studying and tuning light-matter interaction and electronic properties in nanostructures. The optoelectronic properties in layered materials such as…

Mesoscale and Nanoscale Physics · Physics 2024-10-07 Roberto Rosati , Ioannis Paradisanos , Ermin Malic , Bernhard Urbaszek
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