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We present an effective linear response approach to pump-probe femtosecond coherence spectroscopy in the well separated pulse limit. The treatment presented here is based on a displaced and squeezed state representation for the…

Chemical Physics · Physics 2009-11-06 Anand T. N. Kumar , Florin Rosca , Allan Widom , Paul M. Champion

We propose a new method of calculating nonlinear optical responses of interacting electronic systems. In this method, the total Hamiltonian (system + system-pump interaction) is transformed into a different form that (apparently) does not…

Materials Science · Physics 2009-10-31 Jun-ichi Inoue , Akira Shimizu

We explore stimulated photo-association in the context of attosecond pump-probe schemes of atomic matter. An attosecond pulse -- the probe -- is used to induce photo-association of an electronic wave packet which had been created before,…

Atomic Physics · Physics 2009-11-13 Paula Rivière , Camilo Ruiz , Jan-Michael Rost

We investigate theoretically the dissociative ionization of a H2+ molecule using two ultrashort laser (pump-probe) pulses. The pump pulse prepares a dissociating nuclear wave packet on an ungerade surface of H2+. Next, an UV (or XUV) probe…

Quantum Physics · Physics 2013-05-29 Szczepan Chelkowski , André D. Bandrauk

We theoretically explore a variant of RABBITT spectroscopy in which the attosecond-pulse train comprises isolated pairs of consecutive harmonics of the fundamental infrared probe frequency. In this scheme, one-photon and two-photon…

Atomic Physics · Physics 2019-05-15 Bejan Ghomashi , Nicolas Douguet , Luca Argenti

Integrated microring resonators have a broad range of applications in diverse fields with the potential to design compact, robust, energy-efficient devices crucial for quantum applications. Degenerate optical parametric oscillations (DOPOs)…

Spontaneous emission (SE) from a two-level atom in a photonic crystal (PC) with anisotropic one-band model is investigated using the fractional calculus. Analytically solving the kinetic equation in terms of the fractional exponential…

Other Condensed Matter · Physics 2015-05-13 Jing-Nuo Wu , Chih-Hsien Huang , Szu-Cheng Cheng , Wen-Feng Hsieh

When a suspension consisting of dielectric particles having nonlinear characteristics is subjected to a sinusoidal (ac) field, the electrical response will in general consist of ac fields at frequencies of the higher-order harmonics. These…

Soft Condensed Matter · Physics 2007-05-23 J. P. Huang , Jones T. K. Wan , C. K. Lo , K. W. Yu

In this work, nonlinear optical (NLO) studies of nickel oxide doped (ranging from 0.2 to 1.0 mol%) Li2SO4-MgO-P2O5 glasses are reported. A combination of femtosecond (fs) laser, as a pumping light source and a high-accuracy polarimeter with…

Femtosecond laser exposure in the non-ablative regime induces a variety of bulk structural modifications, in which anisotropy may depend on the polarization of the writing beam. In this work, we investigate the correlation between…

Optics · Physics 2016-09-15 Ben McMillen , Yves Bellouard

We define, compute and analyze the nonequilibrium differential optical conductivity of the one-dimensional extended Hubbard model at half-filling after applying a pump pulse, using the time-dependent density matrix renormalization group…

Strongly Correlated Electrons · Physics 2021-08-19 Julian Rincon , Adrian E. Feiguin

The ionization dynamics of a two-electron atom in an attosecond XUV-infrared pump-probe experiment is simulated by solving the time-dependent two-electron Schr\"odinger equation. A dramatic change of the double ionization (DI) yield with…

Atomic Physics · Physics 2010-11-29 S. Bauch , K. Balzer , M. Bonitz

We theoretically investigate the quantum interference of entangled two-photon states generated in a nonlinear crystal pumped by femtosecond optical pulses. Interference patterns generated by the polarization analog of the Hong-Ou-Mandel…

Quantum Physics · Physics 2012-08-27 J. Perina, , A. V. Sergienko , B. M. Jost , B. E. A. Saleh , M. C. Teich

Low dimensionality in CDW systems leads to anisotropic optical properties, in both equilibrium and non-equilibrium conditions. Here we perform polarized two-color pump probe measurements on a quasi-1D material ZrTe$_3$, in order to study…

Strongly Correlated Electrons · Physics 2023-10-20 Li Yue , Amrit Raj Pokharel , Jure Demsar , Sijie Zhang , Yuan Li , Tao Dong , Nanlin Wang

We study optical response of a resonant medium possessing nonlinear coupling to external field driven by a few-cycle pump pulse sequence. We demonstrate the possibility to directly produce unipolar half-cycle pulses from the medium…

Real-time simulations of laser-driven electron dynamics contain information about molecular optical properties through all orders in response theory. These properties can be extracted by assuming convergence of the power series expansion of…

We study the dipole-dipole spectral broadening of a resonance line at high atomic densities when the self-broadening dominates. The selective reflection spectrum of a weak probe beam from the interface of the cell window and rubidium vapor…

Quantum Physics · Physics 2009-03-09 Hebin Li , Vladimir A. Sautenkov , Yuri V. Rostovtsev , Marlan O. Scully

Phase-modulated non-linear spectroscopy with higher harmonic demodulation has recently been suggested to provide information on many-body excitations. In the present work we theoretically investigate the application of this method to infer…

Quantum Physics · Physics 2017-05-29 Zeng-Zhao Li , Lukas Bruder , Frank Stienkemeier , Alexander Eisfeld

Linear and non-linear spectroscopies are powerful tools used to investigate the energetics and dynamics of electronic excited states of both molecules and crystals. While highly accurate \emph{ab initio} calculations of molecular spectra…

Materials Science · Physics 2019-09-26 Alan M. Lewis , Timothy C. Berkelbach

We present a microscopic analysis and evaluation of the dielectric susceptibility of a dielectric medium consisting of vector-type two-energy-level atoms responding on a weak probe mode when the atoms are driven by a strong coherent field.…

Quantum Physics · Physics 2026-01-06 A. S. Usoltsev , L. V. Gerasimov , A. D. Manukhova , S. P. Kulik , D. V. Kupriyanov