Related papers: Two-Dimensional Electronic Spectroscopy Using Inco…
Interpretation of time-resolved spectroscopies such as transient absorption (TA) or two-dimensional (2D) spectroscopy often relies on the perturbative description of light-matter interaction. In many cases the third order of nonlinear…
The development of attosecond technology has enabled the real-time observation of coherent electron motion in atoms, molecules and condensed phases. Experimentally, it is now possible to generate laser pulses of durations of only a few tens…
The homogeneous spectral linewidth associated with light-matter interactions is a fundamental descriptor of the optical properties of materials, governed by the quantum dynamics of the condensed-matter system. We discuss here that the…
Electromagnetically induced transparency in an optically thick, cold medium creates a unique system where pulse-propagation velocities may be orders of magnitude less than $c$ and optical nonlinearities become exceedingly large. As a…
We investigate how optical second-order cross correlations witness the quantum features of a prototype donor-acceptor light-harvesting unit. By considering a pair of detuned two-level emitters electronically coupled and incoherently driven…
Transition-edge sensors (TES) are photon-number resolving calorimetric spectrometers with near unit efficiency. Their recovery time, which is on the order of microseconds, limits the number resolving ability and timing accuracy in high…
Time-resolved photoelectron spectroscopy (trPES) can directly detect transient electronic structure, thus bringing out its promising potential to clarify nonequilibrium processes arising in condensed matters. Here we report the result of…
The nonlinear propagation of intense incoherent photons in a photon gas is considered. The photon-photon interactions are governed by a pair of equations comprising a wave-kinetic equation for the incoherent photons in the presence of the…
We discuss in depth the validity and limitations of a theoretical scheme to evaluate photo-electron spectra (PES) through collecting the phase oscillations at a given measuring point. Problems appear if the laser pulse is still active when…
Amplified spontaneous emission is a common noise source in active optical systems, it is generally seen as being an incoherent process. Here we excite an ensemble of rare earth ion dopants in a solid with a {\pi}-pulse, resulting in…
We provide a complete and exact quantum description of coherent light scattering in a one-dimensional multi-mode transmission line coupled to a two-level emitter. Using recently developed scattering approach we discuss transmission…
Photon indistinguishability is an essential concept to understanding mysterious quantum features from the viewpoint of the wave-particle duality in quantum mechanics. The physics of indistinguishability lies in the manipulation of quantum…
We study in theory the generation and detection of electron spin coherence in nonlinear optical spectroscopy of semiconductor quantum dots doped with single electrons. In third-order differential transmission spectra, the inverse width of…
Rate equations are used to model spectroscopic observation of incoherent energy transfer in light-harvesting antenna systems based upon known structures. A two-parameter two-dimensional model is proposed. The transfer rates obtained, by…
Single molecule spectroscopy aims at unveiling often hidden but potentially very important contributions of single entities to a system's ensemble response. Albeit contributing tremendously to our ever growing understanding of molecular…
Measuring the spectral phase of a pulse is key for performing wavelength resolved ultrafast measurements in the few femtosecond regime. However, accurate measurements in real experimental conditions can be challenging. We show that the…
The influence of coherent optical nonlinearities on polariton propagation effects is studied within a theory-experiment comparison. A novel approach that combines a microscopic treatment of the boundary problem in a sample of finite…
Using the theory of imaging with partially coherent light, we derive general expressions for different kinds of interferometric setups like double slit, shift and mirror interference. We show that in all cases the interference patterns…
XUV and X-ray Free Electron Lasers (FELs) produce short wavelength pulses with high intensity, ultrashort duration, well-defined polarization and transverse coherence, and have been utilised for many experiments previously possible at long…
Images of electron flow through a two-dimensional electron gas from a quantum point contact (QPC) can be obtained at liquid He temperatures using scanning probe microscopy (SPM). A negatively charged SPM tip depletes the electron gas…