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Excitation of a model photosynthetic molecular aggregate by incoherent sunlight is systematically examined. For a closed system, the excited state coherence induced by the sunlight oscillates with an average amplitude that is inversely…

Chemical Physics · Physics 2014-08-25 Jan Olšina , Arend G. Dijkstra , Chen Wang , Jianshu Cao

The question of whether sunlight induces coherent dynamics in biological systems is under debate. Here we show, on the basis of an exact fully quantum mechanical treatment, that thermal light induces excited-state coherences in matter…

Quantum Physics · Physics 2015-05-04 David Avisar , Asaf Eilam , A. D. Wilson-Gordon

The nature of excited states of open quantum systems produced by incoherent natural thermal light is analyzed based on a description of the generator of the dynamics. Natural thermal light is shown to generate long-lasting coherent dynamics…

Quantum Physics · Physics 2017-09-05 Leonardo A. Pachon , Juan D. Botero , Paul Brumer

We study the natural excitation of molecular systems, applicable to, for example, photosynthetic light-harvesting complexes, by natural incoherent light. In contrast with the conventional classical models, we show that the light need not…

Chemical Physics · Physics 2022-01-11 Aurélia Chenu , Paul Brumer

In this paper we consider dynamics of a molecular system subjected to external pumping by a light source. Within a completely quantum mechanical treatment, we derive a general formula, which enables to asses effects of different light…

Biological Physics · Physics 2012-01-30 Tomas Mancal , Leonas Valkunas

One of the most pertinent problems in the debate on non-trivial quantum effects in biology concerns natural photosynthesis. Since sunlight is composed of thermal photons, it was argued to be unable to induce quantum coherence in matter, and…

Quantum Physics · Physics 2018-07-30 Vyacheslav N. Shatokhin , Mattia Walschaers , Frank Schlawin , Andreas Buchleitner

In many important cases, the rate of excitation of a system embedded in an environment is significantly smaller than the internal system relaxation rates. An important example is that of light-induced processes under natural conditions, in…

Chemical Physics · Physics 2018-10-17 Simon Axelrod , Paul Brumer

Light induced processes in nature occur by irradiation with slowly turned-on incoherent light. The general case of time-dependent incoherent excitation is solved here analytically for V-type systems using a newly developed master equation…

Chemical Physics · Physics 2017-09-13 Amro Dodin , Timur V. Tscherbul , Paul Brumer

Excitation of molecules by incident incoherent electromagnetic radiation, such as sunlight, is described in detail and contrasted with the effect of coherent (e.g. laser) light. The nature of the quantum coherences induced by the former,…

Quantum Physics · Physics 2022-02-23 Amro Dodin , Paul Brumer

We study a generic open quantum system where the coupling between the system and its environment is of an energy-preserving quantum nondemolition (QND) type. We obtain the general master equation for the evolution of such a system under the…

Quantum Physics · Physics 2007-10-02 Subhashish Banerjee , R. Ghosh

To control and utilize quantum features in small scale for practical applications such as quantum transport, it is crucial to gain deep understanding of quantum characteristics of states such as coherence. Here by introducing a technique…

Quantum Physics · Physics 2018-01-03 Laleh Memarzadeh , Azam Mani

The conditions under which an open quantum mechanical system may be described by mixed quantum-classical dynamics are investigated. Decoherence is studied using influence functional methods in a model composite quantum system comprising two…

Mesoscale and Nanoscale Physics · Physics 2009-11-07 Kazutomu Shiokawa , Raymond Kapral

Entanglement within a given device provides a potential resource for quantum information processing. Entanglement between system and environment leads to decoherence (thus suppressing non-classical features within the system) but also opens…

Quantum Physics · Physics 2007-05-23 Guenter Mahler , Jochen Gemmer , Mathias Michel

We study the Markovian process of a multi-mode open system connecting with a non-equilibrium environment, which consists of several heat baths with different temperatures. As an illustration, we study the steady state of three linearly…

Quantum Physics · Physics 2014-03-12 Sheng-Wen Li , Li-Ping Yang , C. P. Sun

We analyze in detail the heating of bosonic atoms in an optical lattice due to incoherent scattering of light from the lasers forming the lattice. Because atoms scattered into higher bands do not thermalize on the timescale of typical…

Quantum Gases · Physics 2011-02-21 H. Pichler , A. J. Daley , P. Zoller

In nature, objects which are in thermal contact with each other, usually approach the same temperature, unless a heat source (or sink) cherishes a persistent flow of heat. Accordingly, in a well-isolated apartment flat, most items are at a…

Soft Condensed Matter · Physics 2019-12-04 Suvendu Mandal , Benno Liebchen , Hartmut Löwen

The impact of disorder in the vibrational bath of an ensemble of open quantum systems is explored, arising either from variation in the overall coupling strength or from uncertainty in the shape of the environment spectral function. Such…

Quantum Physics · Physics 2015-05-21 Samuel L. Smith , Alex W. Chin

For open quantum systems coupled to a thermal bath at inverse temperature $\beta$, it is well known that under the Born-, Markov-, and secular approximations the system density matrix will approach the thermal Gibbs state with the bath…

Quantum Physics · Physics 2011-03-15 Gernot Schaller

Recent numerical simulations of a disordered system (Preprint arXiv:condmat/0307554) have shown the existence of two different relaxational processes (called stimulated and spontaneous) characterizing the relaxation observed in structural…

Disordered Systems and Neural Networks · Physics 2007-05-23 F. Ritort

Decoherence of a quantum state coupled to an exterior environment is at the foundation of our understanding of the emergence of classical behavior from the quantum world, but how does it emerge in a finite closed quantum system? Here this…

Quantum Physics · Physics 2015-06-16 O. Fialko
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