Related papers: Quantum-classical lifetimes of Rydberg molecules
We study the excitation dynamics of Rydberg atoms in a one-dimensional lattice with periodic boundary conditions where the atomic Rydberg states are resonantly excited from the electronic ground state. Our description of the corresponding…
We present a novel binding mechanism where a neutral Rydberg atom and an atomic ion form a molecular bound state at large internuclear distance. The binding mechanism is based on Stark shifts and level crossings which are induced in the…
Atoms in highly excited Rydberg states exhibit remarkable properties and constitute a powerful tool for studying quantum phenomena in strongly interacting many-particle systems. We investigate alkali atoms that are held in a ring lattice…
Circular Rydberg states are ideal tools for quantum technologies, with huge mutual interactions and extremely long lifetimes in the tens of milliseconds range, two orders of magnitude larger than those of laser-accessible Rydberg states.…
Atomic processing units require robust entanglement between individual qubits, typically achieved via excitation to highly interacting Rydberg states. However, short Rydberg lifetimes and ionization risks limit the quantum volume score of…
Strongly Rydberg-blockaded two-level atoms form a Rydberg superatom, which is excited only to a collective symmetrical Dicke state. However, emerging often in the alkali-earth atoms, the spontaneous decay from the Rydberg state to an…
Long-range Rydberg molecules are typically bound in wells formed in their oscillatory potential energy curves. In alkaline Rydberg molecules, bound vibrational states exist even when these potential wells are disrupted by level repulsion…
The coupling of an isolated quantum state to a continuum is typically associated with decoherence and decreased lifetime. Here, we demonstrate that Rydberg macrodimers, weakly bound pairs of Rydberg atoms, can overcome this dissipative…
Recent experiments with Bose-Einstein condensates have entered a regime in which thousands of ground-state condensate atoms fill the Rydberg-electron orbit. After the excitation of a single atom into a highly excited Rydberg state,…
We report the observation of spin-singlet ultra-long range Rydberg butterfly molecules consisting of a ground-state atom bound to a Rydberg atom by $P$-wave scattering of $^{87}$Rb Rydberg electrons from $^{87}$Rb(5s) atoms. A three-photon…
Vibrational properties of ultralong Rydberg Cs$_2$ molecules are investigated on corresponding potential curves obtained by perturbation theory. The Rydberg Cs$_2$ molecules are associated by a Rydberg Cs($nS/nP$) atom $(n=30-70)$ and a…
We examine interactions between atoms continuously and coherently driven between the ground state and a Rydberg state, producing "Rydberg-dressed atoms." Because of the large dipolar coupling between two Rydberg atoms, a small admixture of…
It is common knowledge that atoms can form molecules if they attract each other. Here, we show that it is possible to create molecules where bound states of the atoms are not the result of attractive interactions but have the topological…
Atoms with a highly excited electron, called Rydberg atoms, can form unusual types of molecular bonds. The bond differs from the well known ionic and covalent bonds not only by its binding mechanism, but also by its bond length ranging up…
Rydberg atoms with principal quantum number n >> 1 have exaggerated atomic properties including dipole-dipole interactions that scale as n^4 and radiative lifetimes that scale as n^3. It was proposed a decade ago to take advantage of these…
Experiments involving ultracold molecules require sufficiently long lifetimes, which can be very short for excited rovibrational states in the molecular potentials. For alkali atoms such as rubidium, a lowest rovibrational molecular state…
We unravel some peculiar properties of ultralong-range Rydberg molecules formed by an $s$-state $^{87}$Rb Rydberg atom and a corresponding ground-state atom whose electronic orbitals are spherically symmetric and therefore should not be…
We introduce the Rydberg Composite, a new class of Rydberg matter where a single Rydberg atom is interfaced with a dense environment of neutral ground state atoms. The properties of the Composite depend on both the Rydberg excitation, which…
Coherence time and gate fidelities in Rydberg atom quantum simulators and computers are fundamentally limited by the Rydberg state lifetime. Circular Rydberg states are highly promising candidates to overcome this limitation by orders of…
Assemblies of interacting Rydberg atoms show promise for the quantum simulation of transport phenomena, quantum chemistry and condensed matter systems. Such schemes are typically limited by the finite lifetime of Rydberg states. Circular…