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The process in which Raman scattering produces correlated Stokes and anti-Stokes radiation is known as Stokes--anti-Stokes (SaS) scattering. It has been shown recently that this process can generate entangled photon pairs, making it a…

Quantum Physics · Physics 2025-09-30 Raul Corrêa , Marcelo F. Santos , Carlos H. Monken , Ado Jorio

We demonstrate experimentally and theoretically a controllable way of shifting the frequency of an optical pulse by using a combination of spectral hole burning, slow light effect, and linear Stark effect in a rare-earth-ion doped crystal.…

Quantum Physics · Physics 2016-04-27 Qian Li , Yupan Bao , Axel Thuresson , Adam N. Nilsson , Lars Rippe , Stefan Kröll

Coherent anti-Stokes Raman scattering is a widely used imaging technique that provides chemical contrast without the need for labels, making it an extremely valuable tool in physics, chemistry, and biology. In this work, we explore its…

Quantum Physics · Physics 2025-08-05 Giacomo Sorelli , Manuel Gessner , Frank Schlawin

The exceptional nonlinearity of alkali-metal vapors enables highly efficient nonlinear optical processes even at relatively low optical intensities. However, such processes have traditionally relied on centimeter-scale vapor cells. Here, we…

Optics · Physics 2026-05-05 Heleni Krelman , Ori Nefesh , Liron Stern

We theoretically examine Raman photoassociation of a Bose-Einstein condensate, revisiting stimulated Raman adiabatic passage (STIRAP). Due to collisional mean-field shifts, efficient molecular conversion requires strong coupling and low…

Atomic Physics · Physics 2007-05-23 Matt Mackie , Kari Harkonen , Anssi Collin , Kalle-Antti Suominen , Juha Javanainen

Using a high-Q diamond microresonator (Q > 300,000) interfaced with high-power-handling directly-written doped-glass waveguides, we demonstrate a Raman laser in an integrated platform pumped in the near-visible. Both TM-to-TE and TE-to-TE…

We demonstrate stimulated Raman gain using a broadband LED Stokes source to measure vibrational spectra of aqueous glucose solutions. This versatile and cost-effective method increases Raman signal for a variety of applications. We measured…

Applied Physics · Physics 2018-09-14 Peter Bullen , Ioannis Kymissis , Adler Perotte

We experimentally demonstrate transitions between electronic angular momentum states with a difference in magnetic quantum numbers $\Delta \mathrm{m_J} = $ 3, 4, and 5 via resonant four- and six-photon stimulated Raman transitions in a…

We report a study of soliton self-frequency shifting in hydrogen-filled hollow-core fiber. The combination of hydrogen and short 40-fs input pulses underlies clean and efficient generation of Raman solitons between 1080 and 1600 nm. With…

Achieving a high population of antihydrogen/hydrogen atoms in the 2S level is essential for spectroscopy measurements testing similarities between matter and antimatter. We propose and examine the efficiency of applying the STIRAP…

Atomic Physics · Physics 2025-09-19 AbdAlGhaffar K. Amer , A. Capra , T. Friesen , M. C. Fujiwara , T. Momose , C. So , F. Robicheaux

Any amplifier requires coupling to its internal degrees of freedom for energy gain. This coupling introduces extra quantum noise to the output. On the other hand, if the internal degree of the amplifier can be accessed and manipulated, we…

Quantum Physics · Physics 2025-11-18 Jianmin Wang , Rong Zhu , Yue Li , Z. Y. Ou

We present the development and performance of a Fourier transformation (FT) based Raman spectrometer working with visible laser (532 nm) excitation. It is generally thought that FT-Raman spectrometers are not viable in the visible range…

The principle and experimental realization of a novel Raman spectroscopic technique entitled stimulated Raman phase shift (SRPS) spectroscopy was demonstrated. This technique depends on the measurement of the stimulated Raman scattering…

Optics · Physics 2024-03-07 Meng Qi , Wenrong Wang , Yuan-ji Li , Jin-xia Feng , Kuan-shou Zhang

Large-area quantum networks based on optical fibers allow photons at near-infrared wavelengths to travel with minimal loss. Quantum frequency conversion is a method to alter the wavelength of a single photon while maintaining its quantum…

Quantum Physics · Physics 2025-06-09 Anica Hamer , Frank Vewinger , Michael H. Frosz , Simon Stellmer

We consider the microwave-to-optical frequency conversion based on the Lamb shift, fine structure and forbidden transitions. The theory of such a conversion is developed and the efficiency of the microwave-to-optical frequency conversion is…

Quantum Physics · Physics 2018-06-20 Sergey A. Rashkovskiy

We present a novel approach to transient Raman spectroscopy, which combines stochastic probe pulses and a covariance-based detection to measure stimulated Raman signals in alpha-quartz. A coherent broadband pump is used to simultaneously…

In its usual implementation, the Raman amplifier features only one pump carrier frequency. However, pulses with well-separated frequencies can also be Raman amplified while compressed in time. Amplification with frequency-separated pumps is…

Plasma Physics · Physics 2018-04-04 Ido Barth , Nathaniel J. Fisch

We formulate the energy conversion efficiency from a high-order soliton to fundamental solitons by including the influence of interpulse Raman scattering in the fission process. The proposed analytical formula agrees closely with numerical…

Optics · Physics 2023-02-15 Robi Kormokar , Md Hosne Mobarok Shamim , Martin Rochette

The operator solution of a completely quantum mechanical Hamiltonian of the Raman processes is used here to investigate the possibility of obtaining intermodal entanglement between different modes involved in the Raman processes (e.g. pump…

Quantum Physics · Physics 2022-06-10 Biswajit Sen , Sandip Kumar Giri , Swapan Mandal , C. H. Raymond Ooi , Anirban Pathak

We present the possibility of steering the direction of correlations between the off-resonant Raman scattered photons from the angularly multimode atomic memory based on warm rubidium vapors. Using acousto-optic deflectors (AOD) driven by…

Quantum Physics · Physics 2017-01-05 Mateusz Mazelanik , Michał Dąbrowski , Wojciech Wasilewski