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A fully stabilized mid-infrared optical frequency comb spanning from 2.9 to 3.4 um is described. The comb is based on half-harmonic generation in a femtosecond optical parametric oscillator, which transfers the high phase coherence of a…

Optics · Physics 2017-04-05 Markku Vainio , Juho Karhu

We demonstrate a robust and simple method for measurement, stabilization and tuning of the frequency of cw mid-infrared (MIR) lasers, in particular of quantum cascade lasers. The proof of principle is performed with a quantum cascade laser…

Quantum Cascade Lasers (QCL) are increasingly being used to probe the mid-infrared "molecular fingerprint" region. This prompted efforts towards improving their spectral performance, in order to reach ever-higher resolution and precision.…

Laser frequency combs are coherent light sources that emit a broad spectrum consisting of discrete, evenly spaced narrow lines, each having an absolute frequency measurable within the accuracy of an atomic clock. Their development, a decade…

Optics · Physics 2017-06-13 Albert Schliesser , Nathalie Picqué , Theodor W. Hänsch

The advancement of technologies for the precise interrogation of molecules offers exciting possibilities for new studies in the realms of precision spectroscopy and quantum technologies. Experiments in these domains often address molecular…

Optics · Physics 2022-09-15 Mudit Sinhal , Anatoly Johnson , Stefan Willitsch

A continuous-wave Fabry-Perot quantum cascade laser (QCL) emitting at 8.1 $\mu$m operating in the single mode regime has been coherently phase locked to a turn-key low-noise commercial mid-Infrared (mid-IR) optical frequency comb. The…

The mid-infrared (mid-IR) regime (typically the wavelength regime of $\lambda \sim 2.5-20 \ \mathrm{\mu m}$) is an important spectral range for spectroscopy as many molecules have their fundamental rotational-vibrational absorption in this…

Optical frequency comb synthesizers (FCs) [1] are laser sources covering a broad spectral range with a number of discrete, equally spaced and highly coherent frequency components, fully controlled through only two parameters: the frequency…

We present a new method for accurate mid-infrared frequency measurements and stabilization to a near-infrared ultra-stable frequency reference, transmitted with a long-distance fibre link and continuously monitored against state-of-the-art…

Quantum cascade laser (QCL) frequency combs have revolutionized mid-infrared (MIR) spectroscopy by their high brightness and fast temporal resolution, and are a promising technology for fully-integrated and cost-effective sensors. As for…

Over the last two decades, frequency combs have brought breakthroughs in length metrology with traceability to length standards. In particular, frequency-comb-based spectral interferometry is regarded as a promising technology for…

Optics · Physics 2025-01-20 Yoon-Soo Jang , Heulbi Ahn , Sunghoon Eom , Jungjae Park , Jonghan Jin

We demonstrate a powerful tool for high-resolution mid-IR spectroscopy and frequency metrology with quantum cascade lasers (QCLs). We have implemented frequency stabilization of a QCL to an ultra-low expansion (ULE) reference cavity, via…

We report the upgrade and operation of a frequency-comb-assisted high-resolution mid-infrared molecular spectrometer allowing us to combine high spectral purity, SI-traceability, wide tunability and high sensitivity. An optical frequency…

We describe a coherent mid-infrared continuum source with 700 cm-1 usable bandwidth, readily tuned within 600 - 2500 cm-1 (4 - 17 \mum) and thus covering much of the infrared "fingerprint" molecular vibration region. It is based on…

Quantum Physics · Physics 2015-06-04 Fritz Keilmann , Sergiu Amarie

We report the synthesis and measurement of an ultra-precise and extremely stable optical frequency in the telecommunications window around 1543 nm. Using a fibre-based femtosecond frequency comb we have phase-stabilised a fibre laser at 194…

Optics · Physics 2009-11-13 Gesine Grosche , Burghard Lipphardt , Harald Schnatz

Mid infrared (MIR) photonics is a key region for molecular physics [1]. High-resolution spectroscopy in the 1--10 {\mu}m region, though, has never been fully tackled for the lack of widely-tunable and practical light sources. Indeed, all…

We demonstrate a new simple technique to measure IR frequencies near 30 THz using a femtosecond (fs) laser optical comb and sum-frequency generation. The optical frequency is directly compared to the distance between two modes of the fs…

Precision laser spectroscopy is key to many developments in atomic and molecular physics and the advancement of related technologies such as atomic clocks and sensors. However, in important spectroscopic scenarios, such as astronomy and…

Mid-infrared (MIR) spectrometers are invaluable tools for molecular fingerprinting and hyper-spectral imaging. Among the available spectroscopic approaches, GHz MIR dual-comb absorption spectrometers have the potential to simultaneously…

In this paper, we present an experimental study of the metrological stabilization of a solid-state frequency comb for embedded metrology applications. The comb is a passively mode-locked laser diode based on InGaAs/InP Quantum-dash…

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