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Related papers: Phonon Softening and Dispersion in EuTiO3

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The reflectivity of single-crystalline CoO has been studied by optical spectroscopy for wave numbers ranging from 100 to 28,000\wn and for temperatures 8 $< T <$ 325 K\@. A splitting of the cubic IR-active phonon mode on passing the…

Strongly Correlated Electrons · Physics 2009-01-20 Ch. Kant , T. Rudolf , F. Schrettle , F. Mayr , J. Deisenhofer , P. Lunkenheimer , M. V. Eremin , A. Loidl

The phonon dispersion was measured at room temperature along (0,0,L) in the tetragonal phase of LaFeAsO using inelastic x-ray scattering. Spin-polarized first-principles calculations imposing various types of antiferromagnetic order are in…

Neutron inelastic scattering measurements of the polar TO phonon mode dispersion in the cubic relaxor Pb(Zn_1/3Nb_2/3)_0.92Ti_0.08O_3 at 500K reveal anomalous behavior in which the optic branch appears to drop precipitously into the…

Materials Science · Physics 2009-10-31 P. M. Gehring , S. E. Park , G. Shirane

We report first principles calculations of the phonon dispersions of PbTe both for its observed structure and under compression. At the experimental lattice parameter we find a near instability of the optic branch at the zone center, in…

Materials Science · Physics 2008-10-27 Jiming An , Alaska Subedi , David J. Singh

Exploring the origin of the pseudogap is important for the understanding of superconductivity in cuprates. Here we report a systematical experimental study on the phonon vibrational properties of…

Phonon measurements in the A15-type superconductors were complicated in the past because of the unavailability of large single crystals for inelastic neutron scattering, e.g., in the case of Nb$_3$Sn, or unfavorable neutron scattering…

Superconductivity · Physics 2019-04-19 A. Sauer , D. A. Zocco , A. H. Said , R. Heid , A. Böhmer , F. Weber

We have studied spectral evolution of the $E_u^1$ phonon line of a topological insulator Bi$_{2-x}$Sr$_x$Se$_3$ with temperature. Unlike the Raman-active phonons, the $E_u^1$ mode demonstrates softening upon cooling the crystal, and the…

Materials Science · Physics 2022-01-19 A. A. Melnikov , K. N. Boldyrev , Yu. G. Selivanov , S. V. Chekalin

We investigate the low energy acoustical and optical modes in $\mathrm{HgBa_2CuO_{4+\delta}}$ using inelastic x-ray scattering (IXS). The experimental phonon dispersion and the dynamical structure factor are compared with an atomic shell…

Superconductivity · Physics 2009-11-10 Matteo D'Astuto , Alessandro Mirone , Paola Giura , Dorothee Colson , Anne Forget , Michael Krisch

We report that the lowest energy transverse-optic phonon in metallic SnTe softens to near zero energy at the structural transition at $T_C=75 \text{~K}$ and importantly show that the energy of this mode below $T_C$ increases as the…

Results of in-plane and out-of-plane thermal conductivity measurements on $\rm La_{1.8-x}Eu_{0.2}Sr_xCuO_4$ ($0\leq x\leq0.2$) single crystals are presented. The most characteristic features of the temperature dependence are a pronounced…

Superconductivity · Physics 2016-08-16 C. Hess , B. Büchner , U. Ammerahl , A. Revcolevschi

The relaxor ferroelectric PbMg1/Nb2/3O3 was investigated by means of broad-band dielectric and Fourier Transform Infrared (FTIR) transmission spectroscopy in the frequency range from 1 MHz to 15 THz at temperatures between 20 and 900 K…

Materials Science · Physics 2009-11-10 S. Kamba , M. Kempa , V. Bovtun , J. Petzelt , K. Brinkman , N. Setter

We report a Raman scattering investigation of multiferroic bismuth ferrite BiFeO3 epitaxial (c-axis oriented) thin films from -192 to 1000C. Phonon anomalies have been observed in three temperature regions: in the gamma-phase from 930C to…

Materials Science · Physics 2015-05-14 R. Palai , J. F. Scott , R. S. Katiyar

We use variable-temperature x-ray thermal diffuse scattering and inelastic scattering to investigate the lattice dynamics in single crystals of multiferroic CaMn7O12 which undergo a series of orbital and magnetic transitions at low…

Strongly Correlated Electrons · Physics 2016-11-24 S. M. Souliou , Y. Li , X. Du , M. Le Tacon , A. Bosak

Polycrystalline ceramic samples and a single crystal of EuTiO3 have been investigated by Raman spectroscopy in the temperature range 80-300 K. Although synchrotron XRD data clearly indicated the cubic to tetragonal phase transition around…

Materials Science · Physics 2021-04-21 P. Pappas , E. Liarokapis , M. Calamiotou , A. Bussmann-Holder

We report a molecular dynamics study of ab initio quality of the ferroelectric phase transition in crystalline PbTiO3. We model anharmonicity accurately in terms of potential energy and polarization surfaces trained on density functional…

Materials Science · Physics 2025-04-02 Pinchen Xie , Yixiao Chen , Weinan E , Roberto Car

We present evidence for a concomitant structural and ferroelectric transformation around $T_S\sim 360$ K in multiferroic BiFeO$_3$/LaAlO$_3$ thin films close to the tetragonal phase. Phonon excitations are investigated by using Raman…

Strongly Correlated Electrons · Physics 2015-05-30 K. -Y. Choi , S. H. Do , P. Lemmens , D. Wulferding , C. S. Woo , J. H. Lee , K. Chu , C. -H. Yang

Neutron scattering measurements of the lowest-energy TO phonons in the relaxor Pb(Mg1/3Nb2/3)O3 (PMN) are reported for 10<=T<=750 K. The soft mode, which is overdamped by the polar nanoregions below the Burns temperature T_d = 620 K,…

Materials Science · Physics 2009-11-07 S. Wakimoto , C. Stock , R. J. Birgeneau , Z. -G. Ye , W. Chen , W. J. L. Buyers , P. M. Gehring , G. Shirane

We analyze the ground states and the elementary collective excitations (phonons) of a class of systems, which form cluster crystals in the absence of attractions. Whereas the regime of moderate-to-high-temperatures in the phase diagram has…

Soft Condensed Matter · Physics 2015-05-19 Tim Neuhaus , Christos N. Likos

Temperature dependent inelastic neutron-scattering measurements of the generalized phonon density-of-states for superconducting MgCNi_3, T_c=8 K, give evidence for a soft-mode behavior of low-frequency Ni phonon modes. Results are compared…

Superconductivity · Physics 2009-11-10 R. Heid , B. Renker , H. Schober , P. Adelmann , D. Ernst , K. -P. Bohnen

The polarized Raman spectra of stoichiometric LaTiO$_3$ (T$_N = 150$ K) were measured between 6 and 300 K. In contrast to earlier report on half-metallic LaTiO$_{3.02}$, neither strong background scattering, nor Fano shape of the Raman…

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