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While preserving many of the unusual features of single-layer graphene, few-layer graphene (FLG) provides a richness and flexibility of electronic structure that render this set of materials of great interest for both fundamental studies…

Mesoscale and Nanoscale Physics · Physics 2009-08-04 Kin Fai Mak , Matthew Y. Sfeir , James A. Misewich , Tony F. Heinz

We investigated the electronic structure and lattice dynamics of multiferroic MnWO4 by optical spectroscopy. With variation of polarization, temperature, and magnetic field, we obtained optical responses over a wide range of photon…

Strongly Correlated Electrons · Physics 2010-05-17 Woo Seok Choi , K. Taniguchi , S. J. Moon , S. S. A. Seo , T. Arima , H. Hoang , I. -S. Yang , T. W. Noh , Y. S. Lee

Using density functional theory (DFT) calculations and state-of-the-art many-body perturbation theory, we investigate the electronic and optical properties of the inverse spinel CoFe$_{2}$O$_{4}$, a common anode material for photocatalytic…

Materials Science · Physics 2023-11-28 Shohreh Rafiezadeh , Vijaya Begum-Hudde , Rossitza Pentcheva

How atoms acquire three-dimensional bulk character is one of the fundamental questions in materials science. Before addressing this question, how atomic layers become a bulk crystal might give a hint to the answer. While atomically thin…

Mesoscale and Nanoscale Physics · Physics 2018-09-28 Ryuta Yagi , Taiki Hirahara , Ryoya Ebisuoka , Tomoaki Nakasuga , Shingo Tajima , Kenji Watanabe , Takashi Taniguchi

Cobalt ferrite ultrathin films with inverse spinel structure are among the best candidates for spin-filtering at room temperature. We have fabricated high-quality epitaxial ultrathin CoFe2O4 layers on Ag(001) following a three-step method:…

We use optical spectroscopy to investigate the excitations responsible for the structure in the optical self-energy of thin epitaxial films of La1.83Sr0.17CuO4. Using Eliashberg formalism to invert the optical spectra we extract the…

Superconductivity · Physics 2009-11-13 J. Hwang , E. Schachinger , J. P. Carbotte , F. Gao , D. B. Tanner , T. Timusk

The weak ferromagnetism of La_{1.99}Sr_{0.01}CuO_4 epitaxial thin films is investigated using magnetoresistance measurement. While a steplike negative magnetoresistance associated with the weak ferromagnetic transition is clearly observed…

Superconductivity · Physics 2009-11-10 I. Tsukada

We report an investigation of perovskite-type LaNiO3 thin films by Raman scattering in both various scattering configurations and as a function of temperature. The room-temperature Raman spectra and the associated phonon mode assignment…

Materials Science · Physics 2010-07-30 N. Chaban , M. Weber , S. Pignard , J. Kreisel

In the layered quantum spin systems TiOCl and TiOBr the magnetic susceptibility shows a very weak temperature dependence at high temperatures and transition-induced phenomena at low temperatures. There is a clear connection of the observed…

Strongly Correlated Electrons · Physics 2010-03-09 P. Lemmens , K. Y. Choi , R. Valenti , T. Saha-Dasgupta , E. Abel , Y. S. Lee , F. C. Chou

In this letter we study the electronic structures and optical properties of partially and fully fluorinated graphene by a combination of abinitio G0W0 calculations and large-scale multi-orbital tight-binding simulations. We find that for…

Mesoscale and Nanoscale Physics · Physics 2015-02-25 Shengjun Yuan , Malte Rosner , Alexander Schulz , Tim O. Wehling , Mikhail I. Katsnelson

The structure, magnetic and transport properties of thin films of the Heusler ferrimagnet Mn_{2}CoAl have been investigated for properties related to spin gapless semiconductors. Oriented films were grown by molecular beam epitaxy on GaAs…

Materials Science · Physics 2013-10-01 Michelle E. Jamer , Badih A. Assaf , Trithep Devakul , Don Heiman

The nitrogen substitution into the oxygen sites of several oxide materials leads to a reduction of the band gap to the visible light energy range, which makes these oxynitride semiconductors potential photocatalysts for efficient solar…

Taking advantage of the large electron escape depth of soft x-ray angle resolved photoemission spectroscopy we report electronic structure measurements of (111)-oriented [LaNiO3/LaMnO3] superlattices and LaNiO3 epitaxial films. For thin…

We report on the fabrication of high quality (1 1 1)-oriented ferrimagnetic normal spinel CoCr2O4 epitaxial thin films on single crystal Al2O3 substrates. The structural, electronic and magnetic properties were characterized by in-situ…

Strongly Correlated Electrons · Physics 2015-06-19 Xiaoran Liu , M. Kareev , Yanwei Cao , Jian Liu , S. Middey , D. Meyers , J. W. Freeland , J. Chakhalian

A growth diagram of Lu-Fe-O compounds on MgO (111) substrates using pulsed laser deposition is constructed based on extensive growth experiments. The LuFe$_2$O$_4$ phase can only be grown in a small range of temperature and O$_2$ pressure…

Based on first-principles calculations we show that the oxidation of ultrathin films of Ca$_2$N electrides, electrenes, drives a hexagonal$\rightarrow$tetragonal structural transition. The ground state configuration of the oxidized…

Materials Science · Physics 2020-05-06 Pedro H. Souza , José E. Padilha , Roberto H. Miwa

The equilibrium structure and functional properties exhibited by brownmillerite oxides, a family of perovskite-derived structures with alternating layers of $B$O$_6$ octahedra and $B$O$_4$ tetrahedra, viz., ordered arrangements of oxygen…

Materials Science · Physics 2015-11-24 Joshua Young , James M. Rondinelli

We present a systematic study of the magnetic properties of semiconducting ZnFe$_2$O$_4$ thin films fabricated by pulsed laser deposition at low and high oxygen partial pressure and annealed in oxygen and argon atmosphere, respectively. The…

Applied Physics · Physics 2020-10-28 Vitaly Zviagin , Chris Sturm , Pablo Esquinazi , Marius Grundmann , Rüdiger Schmidt-Grund

Covalent organic frameworks (COFs) offer a high degree of chemical and structural flexibility. There is a large family of COFs built from 2D sheets that are stacked to form extended crystals. While it has been common to represent the…

Materials Science · Physics 2022-10-11 Ju Huang , Matthias J. Golomb , Seán R. Kavanagh , Kasper Tolborg , Alex M. Ganose , Aron Walsh

AlN thin films have been grown on Si (100) substrates by reactive ion beam sputter deposition (IBSD) at different substrate temperatures varying from room temperature (RT) to 500oC. Substrate temperature induced microstructural transition…

Materials Science · Physics 2016-02-23 Neha Sharma , Shilpam Sharma , K. Prabakar , S. Amirthapandian , S. Ilango , S. Dash , A. K. Tyagi