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We analyze a class of inner-shell x-ray laser systems in which the initial conditions of the emission are set by a resonant x-ray difference-frequency drive. Using a microscopic density-matrix framework, we show that two coherent x-ray…

Atomic Physics · Physics 2026-01-26 Carles Serrat

The design and characterization of a new laser-desorption molecular beam source, tailored for use in x-ray-free-electron-laser and ultrashort-pulse-laser imaging experiments, is presented. It consists of a single mechanical unit containing…

Recent studies of the performance of radio-frequency (RF) copper cavities operated at cryogenic temperatures have shown a dramatic increase in the maximum achievable surface electric field. We propose to exploit this development to enable a…

We theoretically investigated how the quantum entanglement between the spin of the photoelectron and the polarization of the emitted X-ray photon depends on the excited core-level, using the 3$d\rightarrow\ $2$p$ and 3$d\rightarrow\ $3$p$…

Quantum Physics · Physics 2025-11-27 Ryo B. Tanaka , Goro Oohata , Takayuki Uozumi

We apply time-dependent R-matrix theory to study inner-shell ionization of C atoms in ultra-short high-frequency light fields with a photon energy between 170 and 245 eV. At an intensity of 10$^{17}$ W/cm$^2$, ionization is dominated by…

Atomic Physics · Physics 2015-08-12 H. F. Rey , H. W. van der Hart

We report a novel experimental technique for the comparison of ionization processes in ultrafast laser pulses irrespective of pulse ellipticity. Multiple ionization of xenon by 50 fs 790 nm, linearly and circularly polarized laser pulses is…

In this paper the use of betatron radiation as a seed for the Free Electron Laser (FEL) is presented. The scheme shown can be adopted from all FEL driven by plasma accelerated electron beams via Particle or Laser Wake Field Acceleration.…

Accelerator Physics · Physics 2022-09-22 A. Ghigo , M. Galletti , V. Shpakov , A. Curcio , V. Petrillo

The processes of energy gain and redistribution in a dense gas subject to an intense ultrashort laser pulse are investigated theoretically for the case of high-pressure argon. The electrons released via strong-field ionization and driven by…

Ab initio based accurate simulation of phonon-assisted optical spectra of semiconductors at finite temperatures remains a formidable challenge, as it requires large supercells for phonon sampling and computationally expensive high-accuracy…

Materials Science · Physics 2025-05-07 Qiangqiang Gu , Shishir Kumar Pandey , Zhanghao Zhouyin

The onset of antiprotonic X-ray transitions at high principal quantum numbers and the occurence of electronic X-rays in antiprotonic argon, krypton, and xenon has been analyzed with the help of Multiconfiguration Dirac-Fock calculations.…

Atomic Physics · Physics 2008-04-17 D. Gotta , K. Rashid , B. Fricke , P. Indelicato , L. M. Simons

Photoelectron angular distributions (PADs) obtained from ionization of potassium atoms using moderately intense femtosecond IR fields ($\sim$10$^{12}$Wcm$^{-2}$) of various polarization states are shown to provide a route to "complete"…

Atomic Physics · Physics 2015-01-15 Paul Hockett , Matthias Wollenhaupt , Christian Lux , Thomas Baumert

Ionization of atoms and molecules in strong laser fields is a fundamental process in many fields of research, especially in the emerging field of attosecond science. So far, demonstrably accurate data have only been acquired for atomic…

The European X-ray Free Electron Laser (XFEL), currently being constructed in Hamburg and planning to be operational in 2017 for users, will deliver 27,000 fully coherent, high brilliance X-ray pulses per second with duration less than 100…

Instrumentation and Detectors · Physics 2015-06-18 Jiaguo Zhang , Eckhart Fretwurst , Heinz Graafsma , Robert Klanner , Ioannis Kopsalis , Joern Schwandt

We perform numerical simulations for photoionization of the argon atom when exposed to a combined field of an infrared laser (abbreviated IR) and its 13th harmonic (H13) by solving the Time-Dependent Schr\"odinger Equation (TDSE)], noting…

Atomic Physics · Physics 2022-08-26 Soumia Chqondi , Souhaila Chaddou , Abdelkader Makhoute

We have employed the VULCAN laser facility to generate a laser plasma X-ray source for use in photoionisation experiments. A nanosecond laser pulse with an intensity of order ${10}^{15}$ W{cm}$^{-2}$ was used to irradiate thin Ag or Sn foil…

The complex physics of inner shell ionization of target atoms by heavy ion impact has remained only partially solved for decades. Recently, agreement between theory and experiment has been achieved by considering inner shell ionization of…

Atomic Physics · Physics 2025-03-24 Manpreet Kaur , Soumya Chatterjee , T. Nandi

A method is suggested to produce, with the help of colliding laser photons with bunches of relativistic ions having two energy levels, both intense beams of monochromatic polarized X-ray fluorescence photons and significant number of X-ray…

High Energy Physics - Experiment · Physics 2010-04-05 K. A. Ispirian , M. K. Ispiryan

The unprecedented brilliance of X-ray free-electron lasers (XFELs) [1, 2] has enabled first studies of nonlinear interactions in the hard X-ray range. In particular, X-ray-optical mixing [3], X-ray second harmonic generation (XSHG) [4] and…

The generation of X-rays and {\gamma}-rays based on synchrotron radiation from free electrons, emitted in magnet arrays such as undulators, forms the basis of much of modern X-ray science. This approach has the drawback of requiring very…

Strong field ionization of benzene, fluorobenzene, benzonitrile and 1-chloro-2-fluorobenzene, is studied within the framework of real-space and real-time time-dependent density functional theory. Analysis of the ionization rates as function…

Chemical Physics · Physics 2018-11-20 Eldad Yahel , Amir Natan