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We characterize the transport properties of functionalized graphene nanoribbons using extensive first-principles calculations based on density functional theory (DFT) that encompass both monovalent and divalent ligands, hydrogenated defects…

Materials Science · Physics 2009-09-08 Giovanni Cantele , Young-Su Lee , Domenico Ninno , Nicola Marzari

We will present brief overview on the electronic and transport properties of graphene nanoribbons focusing on the effect of edge shapes and impurity scattering. The low-energy electronic states of graphene have two non-equivalent massless…

Mesoscale and Nanoscale Physics · Physics 2009-09-30 Katsunori Wakabayashi , Yositake Takane , Masayuki Yamamoto , Manfred Sigrist

We study by density functional and large scale tight-binding transport calculations the electronic structure, magnetism and transport properties of the recently proposed graphene ribbons with edges rolled to form nanotubes. Edges with…

Mesoscale and Nanoscale Physics · Physics 2015-06-11 M. A. Akhukov , Shengjun Yuan , A. Fasolino , M. I. Katsnelson

Doping of the graphene lattice with transition metal atoms resulting in high magnetic anisotropy energy (MAE) is an important goal of materials research owing to its potential application in spintronics. In this article, by using…

The indirect exchange interaction is one of the key factors in determining the overall alignment of magnetic impurities embedded in metallic host materials. In this work we examine the range of this interaction in magnetically-doped…

Mesoscale and Nanoscale Physics · Physics 2013-08-30 J. M. Duffy , P. D. Gorman , S. R. Power , M. S. Ferreira

We theoretically design a graphene-based all-organic ferromagnetic semiconductor by terminating zigzag graphene nanoribbons (ZGNRs) with organic magnets. A large spin-split gap with 100% spin polarized density of states near the Fermi…

Materials Science · Physics 2017-09-13 D. Hou , J. H. Wei , S. J. Xie

Armchair graphene nanoribbons with different proportions of edge oxygen atoms are investigated by using crystal orbital method based on density functional theory. All the nanoribbons are energetically favorable, although buckled edges are…

Materials Science · Physics 2014-11-07 Hongyu Ge , Guo Wang , Yi Liao

The effective interaction between resonant magnetic Anderson impurities in graphene, mediated by conduction electrons, is studied as a function of the strength of the onsite energy level of the impurities and the amplitude of coupling to…

Mesoscale and Nanoscale Physics · Physics 2019-03-06 M. Agarwal , E. G. Mishchenko

Two magnetic impurities on the edge of a zigzag graphene nanoribbon strongly interact with each other via indirect coupling, which can be mediated by conducting carriers. By means of Quantum Monte Carlo (QMC) simulations, we find that the…

Strongly Correlated Electrons · Physics 2015-03-09 F. M. Hu , Liangzhi Kou , Thomas Frauenheim

The independent predictions of edge ferromagnetism and the Quantum Spin Hall phase in graphene have inspired the quest of other two dimensional honeycomb systems, such as silicene, germanene, stanene, iridiates, and organometallic lattices,…

Mesoscale and Nanoscale Physics · Physics 2014-07-28 J. L. Lado , J. Fernández-Rossier

The problem of a magnetic impurity, atomic or molecular, absorbed on top of a carbon atom in otherwise clean graphene is studied using the numerical renormalization group. The spectral, thermodynamic, and scattering properties of the…

Strongly Correlated Electrons · Physics 2009-01-27 P. S. Cornaglia , Gonzalo Usaj , C. A. Balseiro

We present a theoretical study using density functional calculations of the structural, electronic and magnetic properties of 3d transition metal, noble metal and Zn atoms interacting with carbon monovacancies in graphene. We pay special…

Mesoscale and Nanoscale Physics · Physics 2015-05-14 Elton J. G. Santos , Andres Ayuela , Daniel Sanchez-Portal

Magnetic order emerging in otherwise non-magnetic materials as carbon is a paradigmatic example of a novel type of s-p electron magnetism predicted to be of exceptional high-temperature stability. It has been demonstrated that atomic scale…

Theoretical calculations, based on hybrid exchange density functional theory, are used to show that in graphene a periodic array of defects generates a ferromagnetic ground state at room temperature for unexpectedly large defect…

Materials Science · Physics 2009-11-13 L. Pisani , B. Montanari , N. M. Harrison

When Fe, which is a typical ferromagnet using d- or f-orbital states, is combined with 2D materials such as graphene, it offers many opportunities for spintronics. The origin of 2D magnetism is from magnetic insulating behaviors, which…

We examine the electronic structure of recently fabricated in-plane heterojunctions of zigzag graphene nanoribbons embedded in hexagonal boron nitride. We focus on hitherto unexplored interface configurations in which both edges of the…

Mesoscale and Nanoscale Physics · Physics 2024-06-03 Michele Pizzochero , Nikita V. Tepliakov , Johannes Lischner , Arash A. Mostofi , Efthimios Kaxiras

The correlation between structural distortion and emergence of magnetism in graphene containing a single vacancy was investigated using first-principles calculations based on density functional theory (DFT). Our results have shown that a…

Mesoscale and Nanoscale Physics · Physics 2015-06-12 Wendel S. Paz , Wanderlã L. Scopel , Jair C. C. Freitas

We used a quantum Monte Carlo method to study the magnetic impurity adatoms on graphene. We found that by tuning the chemical potential we could switch the values of the impurity's local magnet moment between relatively large and small…

Strongly Correlated Electrons · Physics 2011-08-05 F. M. Hu , Tianxing Ma , Hai-Qing Lin , J. E. Gubernatis

Based on a tight-binding model and a recursive Green's function technique, spin-depentent ballistic transport through tinny graphene sheets (flakes) is studied. The main interest is focussed on: electrical conductivity, giant…

Mesoscale and Nanoscale Physics · Physics 2015-05-13 S. Krompiewski

Using a first principles density functional electronic structure method, we study the energy gaps and magnetism in bilayer graphene nanoribbons as a function of the ribbon width and the strength of an external electric field between the…

Materials Science · Physics 2009-11-13 Bhagawan Sahu , Hongki Min , Allan. H. MacDonald , Sanjay K. Banerjee