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In this work, we report observation of strain effect on physical properties of Sr2IrO4 thin films grown on SrTiO3 (001) and LaAlO3 (001) substrates. It is found that the film on LaAlO3 with compressive strain has a lower antiferromagnetic…

Strongly Correlated Electrons · Physics 2023-09-19 N. Hu , Y. K. Weng , K. Chen , B. You , Y. Liu , Y. T. Chang , R. Xiong , S. Dong , C. L. Lu

We have synthesized thermodynamically metastable Ca2IrO4 thin-films on YAlO3 (110) substrates by pulsed laser deposition. The epitaxial Ca2IrO4 thin-films are of K2NiF4-type tetragonal structure. Transport and optical spectroscopy…

Strongly Correlated Electrons · Physics 2016-05-23 M. Souri , J. H. Gruenewald , J. Terzic , J. W. Brill , G. Cao , S. S. A. Seo

We have synthesized epitaxial Sr2IrO4 thin-films on various substrates and studied their electronic structures as a function of lattice-strains. Under tensile (compressive) strains, increased (decreased) Ir-O-Ir bond-angles are expected to…

Strongly Correlated Electrons · Physics 2013-09-09 J. Nichols , J. Terzic , E. G. Bittle , O. B. Korneta , L. E. De Long , J. W. Brill , G. Cao , S. S. A. Seo

We report on a comprehensive investigation of the effects of strain and film thickness on the structural and magnetic properties of epitaxial thin films of the prototypal $J_\mathrm{eff}=1/2$ compound Sr$_2$IrO$_4$ by advanced X-ray…

We have investigated the electronic properties of epitaxial orthorhombic SrIrO3 thin-films under compressive strain. The metastable, orthorhombic SrIrO3 thin-films are synthesized on various substrates using an epi-stabilization technique.…

Strongly Correlated Electrons · Physics 2014-11-18 J. H. Gruenewald , J. Nichols , J. Terzic , G. Cao , J. W. Brill , S. S. A. Seo

We have investigated the transport and optical properties along the c-axis of a-axis-oriented Sr2IrO4 epitaxial thin-films grown on LaSrGaO4 (100) substrates. The c-axis resistivity is approximately one order of magnitude larger than that…

Strongly Correlated Electrons · Physics 2013-10-01 J. Nichols , O. B. Korneta , J. Terzic , L. E. De Long , G. Cao , J. W. Brill , S. S. A. Seo

Using density functional theory within the local spin density approximation, structural, electronic and magnetic properties of SRO are investigated. We examine the magnitude of the orthorhombic distortion in the ground state and also the…

Materials Science · Physics 2009-11-11 A. T. Zayak , X. Huang , J. B. Neaton , Karin M. Rabe

High quality epitaxial Sr2IrO4 thin films with various thicknesses (9-300 nm) have been grown on SrTiO3 (001) substrates, and their electric transport properties have been investigated. All samples showed the expected insulating behavior…

Materials Science · Physics 2014-08-29 Chengliang Lu , Andy Quindeau , Hakan Deniz , Daniele Preziosi , Dietrich Hesse , Marin Alexe

We have investigated the electronic and optical properties of (Sr$_{1-x}$Ca$_{x}$)$_2$IrO$_4$ (x= 0 - 0.375) and (Sr$_{1-y}$Ba$_y$)$_2$IrO$_4$ (y= 0 - 0.375) epitaxial thin-films, in which the bandwidth is systematically tuned via chemical…

Strongly Correlated Electrons · Physics 2017-06-20 M. Souri , B. H. Kim , J. H. Gruenewald , J. G. Connell , J. Thompson , J. Nichols , J. Terzic , B. I. Min , G. Cao , J. W. Brill , A. Seo

The large spin-orbit coupling in iridium oxides plays a significant role in driving novel physical behaviors, including emergent phenomena in the films and heterostructures of perovskite and Ruddlesden-Popper iridates. In this work, we…

Magneto-transport properties of SrIrO$_3$ thin films epitaxially grown on SrTiO$_3$, using reactive RF sputtering, are investigated. A large anisotropy between the in-plane and the out-of-plane resistivities is found, as well as a signature…

Strongly Correlated Electrons · Physics 2017-07-04 L. Fruchter , O. Schneegans , Z. Z. Li

We study the modification of the electronic structure in the strong spin-orbit coupled Sr$_2$IrO$_4$ by epitaxial strain using density functional methods. Structural optimization shows that strain changes the internal structural parameters…

Materials Science · Physics 2019-02-01 Churna Bhandari , Zoran S. Popović , S. Satpathy

Epitaxial strain provides important pathways to control the magnetic and electronic states in transition metal oxides. However, the large strain is usually accompanied by a strong reduction of the oxygen vacancy formation energy, which…

Enhanced magnetic moment and coercivity in SrRuO3 thin films are significant issues for advanced technological usages and hence are researched extensively in recent times. Most of the previous reports on thin films with enhanced magnetic…

Strongly Correlated Electrons · Physics 2020-06-24 Shekhar Tyagi , Gaurav Sharma , D. M. Phase , V. R. Reddy , V. G. Sathe

Using density-functional theory calculations, we investigate the magnetic as well as the dynamical properties of tetragonal SrRuO3 (SRO) under the influence of epitaxial strain. It is found that both the tensile and compressive strain in…

Strongly Correlated Electrons · Physics 2015-06-12 He He , Hang-Chen Ding , Yong-Chao Gao , Shi-Jing Gong , Xiangang Wan , Chun-Gang Duan

We use density functional theory plus dynamical mean-field theory (DFT+DMFT) to study multiple control parameters for tuning the metal-insulator transition (MIT) in CaVO$_3$ thin films. We focus on separating the effects resulting from…

Strongly Correlated Electrons · Physics 2018-02-14 Sophie Beck , Gabriele Sclauzero , Uday Chopra , Claude Ederer

We have investigated structural, transport, and optical properties of tensile strained (Sr$_{1-x}$La$_x$)$_3$Ir$_2$O$_7$ (x = 0, 0.025, 0.05) epitaxial thin-films. While High-T$_c$ superconductivity is predicted theoretically in the system,…

Strongly Correlated Electrons · Physics 2018-02-19 M. Souri , J. Terzic , J. M. Johnson , J. G. Connell , J. H. Gruenewald , J. Thompson , J. W. Brill , J. Hwang , G. Cao , A. Seo

CoV___O___ (CVO) stands out among spinel vanadates for its ultra-short V-V distances, placing it at the brink of itinerant electron behaviour-an ideal playground for strain engineering. In this work, we exploit this sensitivity by growing…

Effect of biaxial tensile strains on optical functions and band edge transitions of ultra thin epitaxial films was studied using as an example a 13 nm thick SrTiO3 films deposited on KTaO3(100) single-crystal substrates. Optical functions…

Materials Science · Physics 2015-05-14 A. Dejneka , M. Tyunina , J. Narkilahti , J. Levoska , D. Chvostova , L. Jastrabik , V. A. Trepakov

In the perovskite oxide SrCrO$_{3}$ the interplay between crystal structure, strain and orbital ordering enables a transition from a metallic to an insulating electronic structure under certain conditions. We identified a narrow window of…

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