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We develop a simple thermodynamic model to describe the heat transfer mechanisms and generation of acoustic waves in photoacoustic Raman spectroscopy by small particulate suspensions in a gas. Using Langevin methods to describe the thermal…

Quantum Physics · Physics 2009-11-10 Kunal K. Das , Yuri V. Rostovtsev , Kevin Lehmann , Marlan O. Scully

Understanding and quantifying the fundamental physical property of coherence of thermal excitations is a long-standing and general problem in physics. The conventional theory, i.e. the phonon gas model, fails to describe coherence and its…

Computational Physics · Physics 2022-01-11 Zhongwei Zhang , Yangyu Guo , Marc Bescond , Jie Chen , Masahiro Nomura , Sebastian Volz

The measured frequencies and intensities of different first- and second- order Raman peaks of suspended graphene are used to show that optical phonons and different acoustic phonon polarizations are driven out of local equilibrium inside a…

Materials Science · Physics 2017-02-22 Sean Sullivan , Ajit Vallabhaneni , Iskandar Kholmanov , Xiulin Ruan , Jayathi Murthy , Li Shi

We derive expressions for energy flow in terms of lattice normal mode coordinates and energy transmission involving reduced group velocities. With a version of Landauer formula appropriate for lattice dynamic approach, the phonon…

Statistical Mechanics · Physics 2007-05-23 Jian Wang , Jian-Sheng Wang

Separating electron and phonon thermal conductivity components is imperative for understanding the principle thermal transport mechanisms in metals and highly desirable in many applications. In this work, we predict the mode-dependent…

Materials Science · Physics 2019-10-23 Zhen Tong , Shouhang Li , Xiulin Ruan , Hua Bao

We have investigated thermal conductivity of graphene laminate films deposited on polyethylene terephthalate substrates. Two types of graphene laminate were studied - as deposited and compressed - in order to determine the physical…

Materials Science · Physics 2014-11-21 H. Malekpour , K. -H. Chang , J. -C. Chen , C. -Y. Lu , D. L. Nika , K. S. Novoselov , A. A. Balandin

Thermal conductivity is a critical material property in numerous applications, such as those related to thermoelectric devices and heat dissipation. Effectively modulating thermal conductivity has become a great concern in the field of heat…

Materials Science · Physics 2023-04-06 Xiao Wan , Dongkai Pan , Jing-Tao Lü , Sebastian Volz , Lifa Zhang , Qing Hao , Yangjun Qin , Zhicheng Zong , Nuo Yang

The integration of optomechanics and optoelectronics in a single device opens new possibilities for developing information technologies and exploring fundamental phenomena. Gallium arsenide (GaAs) is a well-known material that can bridge…

Two-dimensional transition metal dichalcogenides (TMDCs) are finding promising electronic and optical applications due to their unique properties. In this letter, we systematically study the phonon transport and thermal conductivity of…

Materials Science · Physics 2014-09-30 Xiaokun Gu , Ronggui Yang

The transport relaxation rate 1/tau of a two-dimensional electron gas due to scattering by thermally excited surface acoustic phonons is calculated. The temperature dependence of 1/tau is found to be linear in T for high temperatures, but…

Mesoscale and Nanoscale Physics · Physics 2008-02-03 Andreas Knaebchen

We report first-principles calculations of the phonon dispersion spectrum, thermal expansion, and heat capacity of uranium dioxide. The so-called direct method, based on the quasiharmonic approximation, is used to calculate the phonon…

Materials Science · Physics 2015-05-30 Younsuk Yun , Dominik Legut , Peter M. Oppeneer

Materials with low thermal conductivity usually have complex crystal structures. Herein we experimentally find that a simple crystal structure material AgTlI2 (I4/mcm) owns an extremely low thermal conductivity of 0.25 W/mK at room…

Recently, an anisotropic Debye model [Dames et al., Physical Review B 87, 12 (2013)] was proposed for calculations of the interfacial thermal conductance and the minimum thermal conductivity of graphite-like layered materials. Despite…

Applied Physics · Physics 2018-12-13 Hongkun Li , Weidong Zheng , Yee Kan Koh

Discovering new materials with ultrahigh thermal conductivity has been a critical research frontier and driven by many important technological applications ranging from thermal management to energy science. Here we have rigorously…

Materials Science · Physics 2021-04-19 Huan Wu , Hang Fan , Yongjie Hu

We present a new method for predicting effective thermal conductivity ($\kappa_{\textrm{eff}}$) in materials, informed by ${ab\,initio}$ material property simulations. Using the Boltzmann transport equation in a Self-Adjoint Angular Flux…

Materials Science · Physics 2019-08-22 Jackson R. Harter , Aria Hosseini , Todd. S. Palmer , P. Alex Greaney

Ultrafast two-color pump-probe measurements, involving coherent acoustic phonon (CAP) waves, have provided information simultaneously on the mechanical properties and on the electronic structure of ferromagnetic GaMnAs. The elastic constant…

Materials Science · Physics 2012-09-18 J. Qi , J. A. Yan , H. Park , A. Steigerwald , Y. Xu , S. N. Gilbert , X. Liu , J. K. Furdyna , S. T. Pantelides , N. Tolk

Significant differences exist among literature for thermal conductivity of various systems computed using molecular dynamics simulation. In some cases, unphysical results, for example, negative thermal conductivity, have been found. Using…

Materials Science · Physics 2012-06-26 X. W. Zhou , S. Aubry , R. E. Jones , A. Greenstein , P. K. Schelling

Materials with very low thermal conductivity are of high interest for both thermoelectric and optical phase-change applications. Synthetic nanostructuring is most promising to suppress thermal conductivity by scattering phonons, but…

Thermal conductivities $\Lambda $ of amorphous carbon thin films are measured in the temperatures range 80--400 K using the $3\omega $ method. Sample films range from soft a-C:H prepared by remote-plasma deposition ($\Lambda = 0.20$ W…

Materials Science · Physics 2009-10-31 Andrew J. Bullen , Keith E. O'Hara , David G. Cahill , Othon Monteiro , Achim von Keudell

We develop a computational framework, based on the Boltzmann transport equation, with the ability to compute the thermal transport in nanostructured materials of any geometry using as the only input the bulk thermal conductivity…

Mesoscale and Nanoscale Physics · Physics 2014-10-20 Giuseppe Romano , Jeffrey C. Grossman