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The thermal conductivities of beta-Ga2O3 single crystals along four different crystal directions were measured in the temperature range of 80-495K using the time domain thermoreflectance (TDTR) method. A large anisotropy was found. At room…

Materials with high thermal conductivity are needed to conduct heat away from hot spots in high power electronics and optoelectronic devices. Cubic boron arsenide (c-BAs) has a high thermal conductivity due to its special phonon dispersion…

We review our recent development of a first-principles lattice dynamics method that can treat anharmonic effects nonperturbatively. The method is based on the self-consistent phonon theory and temperature-dependent phonon frequencies can be…

Materials Science · Physics 2018-01-29 Terumasa Tadano , Shinji Tsuneyuki

Recent theory has predicted large temperature differences between the in-plane (LA and TA) and out-of-plane (ZA) acoustic phonon baths in locally-heated suspended graphene. To verify these predictions, and their implications for…

Mesoscale and Nanoscale Physics · Physics 2020-03-18 Robin J. Dolleman , Gerard J. Verbiest , Yaroslav M. Blanter , Herre S. J. van der Zant , Peter G. Steeneken

Declining the lattice thermal conductivity in graphene is essential for its thermoelectric applications. In high electron density systems, scatterings of phonons by electrons are no less than the phonon scatterings by other phonons. With…

Materials Science · Physics 2019-08-08 Ajit Jena , Wu Li

We investigated theoretically the phonon thermal conductivity of single layer graphene. The phonon dispersion for all polarizations and crystallographic directions in graphene lattice was obtained using the valence-force field method. The…

Materials Science · Physics 2009-04-08 D. L. Nika , E. P. Pokatilov , A. S. Askerov , A. A. Balandin

We present here a theoretical method to determine the phononic contribution to the thermal conductance of nanoscale systems in the phase-coherent regime. Our approach makes use of classical molecular dynamics (MD) simulations to calculate…

Mesoscale and Nanoscale Physics · Physics 2022-11-09 Fabian Müller , Peter Nielaba , Juan Carlos Cuevas , Fabian Pauly

The anharmonic phonon properties of type-I filled inorganic clathrates Ba8 Ga16 Ge30 and Sr8 Ga16 Ge30 are obtained from the first-principles calculations by considering the temperature-dependent sampling of the potential energy surface and…

Materials Science · Physics 2022-02-16 Shravan Godse , Yagyank Srivastava , Ankit Jain

We calculate the thermal conductivity (\k{appa}) of both bulk crystalline and single-chain polyethylene (PE) using the first-principles-based anharmonic lattice dynamics. Despite its low \k{appa} in amorphous state, the predicted bulk…

Mesoscale and Nanoscale Physics · Physics 2017-01-11 Xinjiang Wang , Massoud Kaviany , Baoling Huang

Fine-tuning the functional properties of nanomaterials is crucial for technological applications. Superlattices, characterized by periodic repetitions of two or more materials in different dimensions, have emerged as a promising area of…

Knowledge of the mean free path distribution of heat-carrying phonons is key to understanding phonon-mediated thermal transport. We demonstrate that thermal conductivity measurements of thin membranes spanning a wide thickness range can be…

First-principles density-functional calculations are performed to investigate the thermal transport properties in graphene nanoribbons (GNRs). The dimensional crossover of thermal conductance from one to two dimensions (2D) is clearly…

Mesoscale and Nanoscale Physics · Physics 2015-06-04 Jian Wang , Xiao-Ming Wang , Yun-Fei Chen , Jian-Sheng Wang

The Green-Kubo lattice thermal conductivity computed using the full classical heat current of a crystalline solid is compared with results obtained from the quadratic component of the heat current and from the commonly used Peierls heat…

Materials Science · Physics 2026-05-20 Andrey Pereverzev

Superlattices are promising low-dimensional nanomaterials for thermoelectric technology that is capable of directly converting low-grade heat energy to useful electrical power. In this work, the thermal conductivities of GaAs/Ge…

Mesoscale and Nanoscale Physics · Physics 2017-06-28 Roger Jia , Lingping Zeng , Gang Chen , Eugene A. Fitzgerald

First-principles prediction of thermal conductivity and radiative properties is crucial. However, computing phonon scattering, especially for four-phonon scattering, could be prohibitively expensive, and the thermal conductivity even for…

Materials Science · Physics 2023-11-23 Ziqi Guo , Zherui Han , Dudong Feng , Guang Lin , Xiulin Ruan

We apply standard, first-principles calculations to a complete treatment of lattice dynamics in the harmonic approximation. The algorithm makes use of the straightforward ``frozen-phonon'' approach to the calculation of vibrational spectra…

Materials Science · Physics 2007-05-23 Hadley M. Lawler , Eric K. Chang , Eric L. Shirley

Phonon-mediated thermal conductivity, which is of great technological relevance, fundamentally arises due to anharmonic scattering from interatomic potentials. Despite its prevalence, accurate first-principles calculations of thermal…

Materials Science · Physics 2017-08-16 Ching Hua Lee , Chee Kwan Gan

Nano-engineering crystalline materials can be used to tailor their thermal properties. By adding new nanoscale phonon scattering centers and controlling their size, one can effectively decrease the phonon mean free path and hence the…

Thermal transport in the Si/SiO$_2$ multishell nanotubes is investigated theoretically. The phonon energy spectra are obtained using the atomistic Lattice Dynamics approach. Thermal conductivity is calculated using the Boltzmann transport…

Materials Science · Physics 2021-04-30 C. Isacova , A. Cocemasov , D. L. Nika , V. M. Fomin

Thermal conductivity in dielectric crystals is the result of the relaxation of lattice vibrations described by the phonon Boltzmann transport equation. Remarkably, an exact microscopic definition of the heat carriers and their relaxation…

Materials Science · Physics 2016-10-26 Andrea Cepellotti , Nicola Marzari