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High molecular weight polymer solutions have a powerful tendency to deposit adsorbed layers when exposed to even mildly attractive surfaces. The equilibrium properties of these dense interfacial layers have been extensively studied…

Soft Condensed Matter · Physics 2007-05-23 Ben O'Shaughnessy , Dimitrios Vavylonis

Many drug delivery systems suffer from undesirable interactions with the host immune system. It has been experimentally established that covalent attachment (irreversible adsorption) of suitable macromolecules to the surface of the drug…

Biological Physics · Physics 2007-05-23 Radek Erban , Jonathan Chapman , Kerry D. Fisher , Ioannis G. Kevrekidis , Leonard W. Seymour

We study the behavior of a flexible polymer chain in the presence of a low-molecular weight solvent in the vicinity of a liquid-gas critical point within the framework of a self-consistent field theory. The total free energy of the dilute…

Statistical Mechanics · Physics 2015-07-29 Yu. A. Budkov , A. L. Kolesnikov , N. Georgi , M. G. Kiselev

We prove to all orders of renormalized perturbative polymer field theory the existence of a short chain expansion applying to polymer solutions of long and short chains. For a general polymer network with long and short chains we show…

Condensed Matter · Physics 2016-08-31 Christian von Ferber

An extended theoretical study of interface potentials in adsorbed colloid-polymer mixtures is performed. To describe the colloid-polymer mixture near a hard wall, a simple Cahn-Nakanishi-Fisher free-energy functional is used. The bulk phase…

Soft Condensed Matter · Physics 2015-06-19 Jesper Koning , Yves Vandecan , Joseph Indekeu

This work presents a general and unified theory describing block copolymer self-assembly in the presence of free surfaces and nanoparticles in the context of Self-Consistent Filed Theory. Specifically, the derived theory applies to free and…

Soft Condensed Matter · Physics 2021-12-17 Daniil Bochkov , Ivana Bagaric , Gaddiel Ouaknin , Frederic Gibou

In the present study, we have investigated, using Monte Carlo simulations (MC), the adsorption of polyelectrolytes on the charged nanopatterned surfaces. Different surface patterns were considered and we noticed that the amount of…

Soft Condensed Matter · Physics 2020-02-04 Amin Bakhshandeh , Maximiliano Segala

In detailed microcanonical analyses of densities of states obtained by extensive multicanonical Monte Carlo computer simulations, we investigate the caloric properties of conformational transitions adsorbing polymers experience near…

Statistical Mechanics · Physics 2019-03-27 Monika Möddel , Wolfhard Janke , Michael Bachmann

We consider an inextensible, semiflexible polymer or worm-like chain which is confined in the transverse direction by a parabolic potential and subject to a longitudinal force at the ends, so that the polymer is stretched out and…

Soft Condensed Matter · Physics 2015-05-28 Theodore W. Burkhardt

The surface tension, the adsorption, and the depletion thickness of polymers close to a single nonadsorbing colloidal sphere are computed by means of Monte Carlo simulations. We consider polymers under good-solvent conditions and in the…

Soft Condensed Matter · Physics 2014-05-06 Giuseppe D'Adamo , Andrea Pelissetto , Carlo Pierleoni

We formulate and characterize a model to describe the dynamics of semiflexible polymers in the presence of activity due to motor proteins attached irreversibly to a substrate, and a transverse pulling force acting on one end of the…

Biological Physics · Physics 2016-02-12 Abhishek Chaudhuri , Debasish Chaudhuri

The conformation and the phase diagram of a membrane protein are investigated via grand canonical ensemble approach using a homopolymer model. We discuss the nature and pathway of $\alpha$-helix integration into the membrane that results…

Soft Condensed Matter · Physics 2009-10-31 Pyeong Jun Park , W. Sung

We show that the structural properties and phase behavior of a self-avoiding polymer chain on adhesive substrate, subject to pulling at the chain end, can be obtained by means of a Grand Canonical Ensemble (GCE) approach. We derive…

Soft Condensed Matter · Physics 2009-04-05 S. Bhattacharya , V. G. Rostiashvili , A. Milchev , T. A. Vilgis

Mean-field theory is used to model polyelectrolyte adsorption and the possibility of overcompensation of charged surfaces. For charged surfaces that are also chemically attractive, the overcharging is large in high salt conditions,…

Soft Condensed Matter · Physics 2009-11-10 Adi Shafir , David Andelman

Selective targeting of membranes with a specific receptor profile is an ongoing challenge in targeted drug delivery. We investigate the adsorption of copolymers on a multicomponent receptor-covered surface using grand-canonical Monte Carlo…

Soft Condensed Matter · Physics 2026-05-27 Vid Ravnik , Urban Bren , Tine Curk

We analyze the interaction of two conducting, charged polymer chains in solution using a minimal model for their electronic degrees of freedom. We show that a crossing of the two chains in which the polymers pass within Angstroms of each…

Soft Condensed Matter · Physics 2009-11-10 Jeremy D. Schmit , Alex J. Levine

A key assumption of polymer physics is that the random chains polymers extend in flow. Recent experimental evidence has shown that polymer chains compress in Couette flow in a manner counter to expectation. Here, scaling arguments developed…

Soft Condensed Matter · Physics 2018-06-05 Dave E. Dunstan

We present the exact solutions of various directed walk models of polymers confined to a slit and interacting with the walls of the slit via an attractive potential. We consider three geometric constraints on the ends of the polymer and…

Statistical Mechanics · Physics 2009-11-11 R Brak , A L Owczarek , A Rechnitzer , S G Whittington

We consider a lattice model of a semiflexible homopolymer chain in a bad solvent. Beside the temperature $T$, this model is described by (i) a curvature energy $\varepsilon_h$, representing the stiffness of the chain (ii) a…

Condensed Matter · Physics 2009-10-28 S. Doniach , T. Garel , H. Orland

We consider three different continuum polymer models, that all depend on a tunable parameter r that determines the strength of the excluded-volume interactions. In the first model chains are obtained by concatenating hard spherocylinders of…

Soft Condensed Matter · Physics 2017-10-25 Giuseppe D'Adamo , Andrea Pelissetto