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We investigate optical second-harmonic generation (SHG) from metasurfaces where noncentrosymmetric V-shaped gold nanoparticles are ordered into regular array configurations. In contrast to expectations, a substantial enhancement of the SHG…

Plasmonic resonance of a metallic nanostructure results from coherent motion of its conduction electrons driven by incident light. At the resonance, the induced dipole in the nanostructure is proportional to the number of the conduction…

Materials Science · Physics 2016-04-20 Mingliang Zhang , Hongping Xiang , Xu Zhang , Gang Lu

We derive the semiclassical series for the partition function of a one-dimensional quantum-mechanical system consisting of a particle in a single-well potential. We do this by applying the method of steepest descent to the path-integral…

Quantum Physics · Physics 2009-10-31 C. A. A. de Carvalho , R. M. Cavalcanti , E. S. Fraga , S. E. Joras

Topological photonics and acoustics have recently garnered wide research interests for their topological ability to manipulate the light and sound at surfaces. Conventionally, the supercell technique is the standard approach to calculating…

Optics · Physics 2025-12-24 Yi-Xin Sha , Ming-Yao Xia , Ling Lu , Yi Yang

Second-harmonic generation (SHG) is a quintessential probe of inversion symmetry breaking in condensed matter. While perturbative $\chi^{(2)}$ processes are well-documented, the nonperturbative regime under intense driving remains largely…

Strongly Correlated Electrons · Physics 2026-04-08 Keisuke Kitayama , Masao Ogata

The optical properties of clusters with metallic spherical particles embedded in an insulating matrix are studied. A theoretical approach is proposed for the calculation of the macroscopic dielectric response for a collection of spheres at…

Soft Condensed Matter · Physics 2009-10-31 Leonid G. Grechko , Vitaly N. Pustovit , Keith W. Whites

Colloidal quantum dots (QDs) are an attractive medium for nonlinear optics and deterministic heterogeneous integration with photonic devices. Their intrinsic nonlinearities can be strengthened further by coupling QDs to low mode-volume…

High-harmonic generation (HHG), an extreme nonlinear effect, introduces an unprecedented paradigm to detect emergent quantum phases and electron dynamics inconceivable in the framework of linear and low-order nonlinear processes. As an…

Nonlinear optics is essential for many recent photonic technologies. Here, we introduce a novel multi-scale approach to simulate the nonlinear optical response of molecular nanomaterials combining ab initio quantum-chemical and classical…

Second-order nonlinear optical response allows to detect different properties of the system associated with the inversion symmetry breaking. Here, we use a second harmonic generation effect to investigate the alignment of a…

Mesoscale and Nanoscale Physics · Physics 2020-07-03 E. A. Stepanov , S. V. Semin , C. R. Woods , M. Vandelli , A. V. Kimel , K. S. Novoselov , M. I. Katsnelson

A basic concept in chain-particle cluster-motion, from frozen glassy state to melt state, is the 2D soft nano-scale mosaic structure formed by 8 orders of 2D interface excitation (IE) loop-flows, from small to large in inverse cascade and…

Soft Condensed Matter · Physics 2011-05-26 Jia-lin Wu

We study the quantum evolution in dimension three of a system composed by a test particle interacting with an environment made of $N$ harmonic oscillators. At time zero the test particle is described by a spherical wave, i.e. a highly…

Mathematical Physics · Physics 2015-06-15 Carla Recchia , Alessandro Teta

The second-order $\chi^{2}$ process underpins many important nonlinear optical applications in the field of classical and quantum optics. Generally, the $\chi^{2}$ process manifests itself only in a non-centrosymmetric dielectric medium via…

Optics · Physics 2022-06-29 Yadong Wang , Daniel Burt , Kunze Lu , Donguk Nam

An ensemble of classical subsystems interacting with surrounding particles has been considered. In general case, a phase volume of the subsystems ensemble was shown to be a function of time. The evolutional equations of the ensemble are…

Statistical Mechanics · Physics 2015-06-24 S. R. Sharov

Non-classical state generation is an important component throughout experimental quantum science for quantum information applications and probing the fundamentals of physics. Here, we investigate permutations of quantum non-demolition…

Quantum Physics · Physics 2019-10-02 T. J. Milburn , M. S. Kim , M. R. Vanner

We study theoretically the quantum optical properties of hybrid molecules composed of an individual quantum dot and a metallic nanoparticle. We calculate the resonance fluorescence of this hybrid system. Its incoherent part, the one arising…

Quantum Physics · Physics 2010-04-12 A. Ridolfo , O. Di Stefano , N. Fina , R. Saija , S. Savasta

We address the quantum-classical correspondence for chaotic systems with a crossover between symmetry classes. We consider the energy level statistics of a classically chaotic system in a weak magnetic field. The generating function of…

Chaotic Dynamics · Physics 2015-05-13 Keiji Saito , Taro Nagao , Sebastian Muller , Petr Braun

A beyond electric-dipole light-matter theory is needed to describe emerging X-ray and THz applications for characterization and control of quantum materials but inaccessible as nondipole lattice-aperiodic terms impede on the use of Bloch's…

Using a real-space high order finite-difference approach, we investigate the electronic structure of large spherical silicon nanoclusters. Within Kohn-Sham density functional theory and using pseudopotentials, we report the self-consistent…

Materials Science · Physics 2023-06-21 Mehmet Dogan , Kai-Hsin Liou , James R. Chelikowsky

Topology ultimately unveils the roots of the perfect quantization observed in complex systems. The 2D quantum Hall effect is the celebrated archetype. Remarkably, topology can manifest itself even in higher-dimensional spaces in which…

Superconductivity · Physics 2021-01-25 H. Weisbrich , R. L. Klees , G. Rastelli , W. Belzig