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The ability to optically initialize the electronic spin of the nitrogen-vacancy (NV) center in diamond has long been considered a valuable resource to enhance the polarization of neighboring nuclei, but efficient polarization transfer to…

Mesoscale and Nanoscale Physics · Physics 2018-08-01 F. Shagieva , S. Zaiser , P. Neumann , D. B. R. Dasari , R. Stöhr , A. Denisenko , R. Reuter , C. A. Meriles , J. Wrachtrup

Isolated nuclear spins offer a promising building block for quantum information processing systems, but their weak interactions often impede preparation, control, and detection. Hyperfine coupling to a proximal electronic spin can enhance…

Quantum Physics · Physics 2013-05-29 Benjamin Smeltzer , Jean McIntyre , Lilian Childress

We present high-resolution optically detected magnetic resonance (ODMR) spectroscopy on single nitrogen-vacancy (NV) center spins in diamond at and around zero magnetic field. The experimentally observed transitions depend sensitively on…

Mesoscale and Nanoscale Physics · Physics 2019-11-22 Johannes Kölbl , Mark Kasperczyk , Beat Bürgler , Arne Barfuss , Patrick Maletinsky

Recently there have been several theoretical and experimental studies of the prospects for magnetic field sensors based on crystal defects, especially nitrogen vacancy (NV) centres in diamond. Such systems could potentially be incorporated…

Materials Science · Physics 2011-11-15 Marcus Schaffry , Erik M. Gauger , John J. L. Morton , Simon C. Benjamin

Interfacial interactions are crucial in a variety of fields and can greatly affect the electric, magnetic, and chemical properties of materials. Among them, interface orbital hybridization plays a fundamental role in the properties of…

Etching experiments were performed that reveal the vertical distribution of optically active nitrogen-vacancy (NV) centers in diamond created in close proximity to a surface through ion implantation and annealing. The NV distribution…

Mesoscale and Nanoscale Physics · Physics 2009-11-13 Charles Santori , Paul E. Barclay , Kai-Mei C. Fu , Raymond G. Beausoleil

After initial proof-of-principle demonstrations, optically pumped nitrogen-vacancy (NV) centres in diamond have been proposed as a non-invasive platform to achieve hyperpolarisation of nuclear spins in molecular samples over macroscopic…

Mesoscale and Nanoscale Physics · Physics 2021-01-27 J. -P. Tetienne , L. T. Hall , A. J. Healey , G. A. L. White , M. -A. Sani , F. Separovic , L. C. L. Hollenberg

Two dimensional electronic spectroscopy and transient grating measurements were performed, for the first time, on nitrogen-vacancy centers in diamond. These measurements reveal energy transfer and vibrational pathways with consequences for…

Mesoscale and Nanoscale Physics · Physics 2012-07-19 V. M. Huxter , T. A. A. Oliver , D. Budker , G. R. Fleming

We present a theoretical analysis of the electron spin decoherence in single Nitrogen-Vacancy defects in ultra-pure diamond. The electron spin decoherence is due to the interactions with Carbon-13 nuclear spins in the diamond lattice. Our…

Other Condensed Matter · Physics 2009-11-13 J. R. Maze , J. M. Taylor , M. D. Lukin

The detection of nuclear spins using individual electron spins has enabled new opportunities in quantum sensing and quantum information processing. Proof-of-principle experiments have demonstrated atomic-scale imaging of nuclear-spin…

Using pulsed photoionization the coherent spin manipulation and echo formation of ensembles of NV- centers in diamond are detected electrically realizing contrasts of up to 17 %. The underlying spin-dependent ionization dynamics are…

Mesoscale and Nanoscale Physics · Physics 2017-01-25 Florian M. Hrubesch , Georg Braunbeck , Martin Stutzmann , Friedemann Reinhard , Martin S. Brandt

Creation of nitrogen-vacancy (NV) centers at the nanoscale surface region in diamond, while retaining their excellent spin and optical properties, is essential for applications in quantum technology. Here, we demonstrate the extension of…

Materials Science · Physics 2021-03-30 A. Watanabe , T. Nishikawa , H. Kato , M. Fujie , M. Fujiwara , T. Makino , S. Yamasaki , E. D. Herbschleb , N. Mizuochi

The negatively charged Nitrogen-Vacancy (NV-) center in diamond is one of the most versatile and robust quantum sensors suitable for quantum technologies, including magnetic field and temperature sensors. For precision sensing applications,…

We report measurements of optically detected magnetic resonance spectra of ensembles of negatively charged nitrogen-vacancy (NV) centers in diamonds in the presence of strain and DC external electric fields. The Stark shift of the spectral…

Atomic Physics · Physics 2018-02-27 Sarvagya Sharma , Chris Hovde , Douglas H. Beck , Fahad Alghannam

A new method for detecting the magnetic resonance of electronic spins at low temperature is demonstrated. It consists in measuring the signal emitted by the spins with a superconducting qubit that acts as a single-microwave-photon detector,…

Nitrogen-vacancy centers in diamond allow for coherent spin state manipulation at room temperature, which could bring dramatic advances to nanoscale sensing and quantum information technology. We introduce a novel method for the optical…

Precise readout of spin states is crucial for any approach towards physical realization of a spin-based quantum computer and for magnetometry with single spins. Here, we report a new method to strongly improve the optical readout fidelity…

Quantum Physics · Physics 2010-03-01 M. Steiner , P. Neumann , J. Beck , F. Jelezko , J. Wrachtrup

We study relaxation processes of the spins of dipolar-coupled negatively charged nitrogen vacancy (NV$^-$) centers under transverse electric and magnetic fields. Specifically, we uncover regimes where flip-flop, double-flip processes as…

Quantum Physics · Physics 2022-07-29 C. Pellet-Mary , M. Perdriat , P. Huillery , G. Hétet

We studied the dynamic nuclear spin polarization of nitrogen in negatively charged nitrogen-vacancy (NV) centers in diamond both experimentally and theoretically over a wide range of magnetic fields from 0 to 1100 G covering both the…

Quantum Physics · Physics 2021-01-04 Laima Busaite , Reinis Lazda , Andris Berzins , Marcis Auzinsh , Ruvin Ferber , Florian Gahbauer

We report a study of the magnetic field dependence of photoluminescence of NV$^-$ centers (negatively charged nitrogen-vacancy centers) in diamond single crystals. In such a magnetic field dependence characteristic sharp features are…

Quantum Physics · Physics 2017-09-27 Sergei V. Anishchik , Konstantin L. Ivanov
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