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Understanding the optical emission characteristics of semiconductor nanostructures is important when determing their device applicability. The emission depends on the material and its geometry, but also depends on other processes such as…

Mesoscale and Nanoscale Physics · Physics 2023-08-24 H. ~T. ~Sullivan , J. ~H. ~Cole

We investigate theoretically the rates of non-radiative decay of excited semiconducting nanotubes by a variety of decay mechanisms and compare with experimental findings. We find that the multi-phonon decay (MPD) of free excitons is too…

Strongly Correlated Electrons · Physics 2009-11-13 Vasili Perebeinos , Phaedon Avouris

The interaction between off-resonant laser pulses and excitons in monolayer transition metal dichalcogenides is attracting increasing interest as a route for the valley-selective coherent control of the exciton properties. Here, we extend…

We present an exciton/lattice model of the electronic dynamics of primary photoexcitations in a polymeric semiconductor heterojunction which includes both polymer pi-stacking, energetic disorder, and phonon relaxation. Results from our…

Materials Science · Physics 2013-09-26 Eric R. Bittner , Carlos Silva

Plasmonic structures are known to support the modes with subwavelength volumes in which the field matter interactions are greatly enhanced. Coupling between the molecular excitations and plasmons leading to formation of plexcitons has been…

Optics · Physics 2018-11-27 Jacob B Khurgin

Control of the band-edge offsets at heterojunctions between organic semiconductors allows efficient operation of either photovoltaic or light-emitting diodes. We investigate systems where the exciton is marginally stable against charge…

Soft Condensed Matter · Physics 2013-09-27 Arne C. Morteani , Paiboon Sreearunothai , Laura M. Herz , Richard H. Friend , Carlos Silva

We evaluate the rate of energy loss of a plasmon in a disorder-free carbon nanotube. The plasmon decays into neutral bosonic excitations of the electron liquid. The process is mediated either by phonon-assisted backscattering of a single…

Strongly Correlated Electrons · Physics 2011-09-12 Wei Chen , A. V. Andreev , E. G. Mishchenko , L. I. Glazman

The axion decay $a \to e^+ e^-$ via a plasmon is investigated in an external magnetic field. The results we have obtained demonstrate a strong catalyzing influence of the field as the axion lifetime in the magnetic field of order $10^{15}$…

High Energy Physics - Phenomenology · Physics 2009-10-31 N. V. Mikheev , A. Ya. Parkhomenko , L. A. Vassilevskaya

Exciton-surface plasmon coupling is at the heart of the most elementary light-matter interactions and is a result of not only an intrinsic property of the emitter but that of emitter-environment interaction. Thus, change of electromagnetic…

Optics · Physics 2022-03-11 J. S. Duan

We present results on the radiative lifetimes of excitons and trions in a monolayer of metal dichalcogenide MoS2. The small exciton radius and the large exciton optical oscillator strength result in radiative lifetimes in the 0.18-0.30 ps…

Mesoscale and Nanoscale Physics · Physics 2016-01-13 Haining Wang , Changjian Zhang , Weimin Chan , Christina Manolatou , Sandip Tiwari , Farhan Rana

The coupling with the lattice vibrations is shown to drastically modify the state--of--the--art picture of the excitonic states based on a frozen atom approximation. The zero--point vibrations renormalize the bare energies and optical…

Materials Science · Physics 2009-11-13 Andrea Marini

We theoretically investigate the nonlinear optical pulse responses of excitons in a thin film where the excitonic center-of-mass motion is confined. A large interaction volume between excitons and radiation yields particular coupled states…

Materials Science · Physics 2017-04-19 Takashi Kinoshita , Hajime Ishihara

Time-resolved photoluminescence spectra after nonresonant excitation show a distinct 1s resonance, independent of the existence of bound excitons. A microscopic analysis identifies excitonic and electron-hole plasma contributions. For low…

Condensed Matter · Physics 2009-11-10 S. Chatterjee , C. Ell , S. Mosor , G. Khitrova , H. M. Gibbs , W. Hoyer , M. Kira , S. W. Koch , J. P. Prineas , H. Stolz

Spatially indirect excitons in semiconducting double quantum wells have been shown to exhibit rich collective many-body behavior that result from the nature of the extended dipole-dipole interactions between particles. For many…

Disorder derived from defects or strain in monolayer TMDs can lead to a dramatic change in the physical behavior of the interband excitations, producing inhomogeneous spectral broadening and localization; leading to radiative lifetime…

Mesoscale and Nanoscale Physics · Physics 2018-12-05 Sabrine Ayari , Adlen Smiri , Aida Hichri , Sihem Jaziri , Thierry Amand

We investigate the dynamics of the exciton formation and relaxation on a picosecond time scale following a pulsed photoexcitation of a semiconductor. The study is conducted in the framework of the density matrix theory complemented with the…

Mesoscale and Nanoscale Physics · Physics 2015-12-25 Veljko Janković , Nenad Vukmirović

While exciton relaxation in transition metal dichalcogenides (TMDs) has been intensively studied, spatial exciton propagation has received only little attention - in spite of being a key process for optoelectronics and having already shown…

Mesoscale and Nanoscale Physics · Physics 2020-01-23 Roberto Rosati , Raül Perea-Causín , Samuel Brem , Ermin Malic

Linear-response time-dependent density-functional theory (TDDFT) can describe excitonic features in the optical spectra of insulators and semiconductors, using exchange-correlation (xc) kernels behaving as $-1/k^{2}$ to leading order. We…

Materials Science · Physics 2021-08-18 Jiuyu Sun , Cheng-Wei Lee , Alina Kononov , André Schleife , Carsten A. Ullrich

In this paper we study, in the time domain, the interaction between localized surface plasmons and photons in arbitrarily shaped metal nanoparticles, by using the Hopfield approach to quantize the plasmon modes, where the electron…

The effects of the electron-phonon interaction on optical excitations can be understood in terms of exciton-phonon coupling, and require a careful treatment in low-dimensional materials with strongly bound excitons or strong electron-hole…

Materials Science · Physics 2022-02-17 Gabriel Antonius , Steven G. Louie