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We propose a simple linear scaling expression in reciprocal space for evaluating the ion--electron potential of crystalline solids. The expression replaces the long-range ion--electron potential with an equivalent localized charge…

Materials Science · Physics 2016-12-21 Xuecheng Shao , Wenhui Mi , Qiang Xu , Yanchao Wang , Yanming Ma

The theory of self-reciprocal functions is applied to the study Mordell type integrals. We find two particular eigenfunctions of the double cosine Fourier transform and then use them to evaluate certain one- and two-dimensional Mordell type…

Classical Analysis and ODEs · Mathematics 2021-10-28 Martin Nicholson

The state of the art for integral evaluation is that analytical solutions to integrals are far more useful than numerical solutions. We evaluate certain integrals analytically that are necessary in some approaches in quantum chemistry. In…

Chemical Physics · Physics 2017-09-12 Sandor Kristyan

In the present paper, we develop a semiclassical quasi-static model accounting for molecular double ionization in an intense laser pulse. With this model, we achieve insight into the dynamics of two highly-correlated valence electrons under…

Atomic and Molecular Clusters · Physics 2009-11-13 Di-Fa Ye , Jing Chen , Jie Liu

Exploratory variational pseudopotential density functional calculations are performed for the electronic properties of many-electron systems in the 3D cartesian coordinate grid (CCG). The atom-centered localized gaussian basis set,…

Chemical Physics · Physics 2015-05-18 Amlan K Roy

We present a practical and accurate density functional for the exchange-correlation energy of electrons in two dimensions. The exchange part is based on a recent two-dimensional generalized-gradient approximation derived by considering the…

Strongly Correlated Electrons · Physics 2010-06-30 E. Rasanen , S. Pittalis , J. G. Vilhena , M. A. L. Marques

A method for calculating the electronic levels in the compact superheavy nuclear quasi-molecules, based on solving the two-center Dirac equation using the multipole expansion of two-center potential, is developed. For the internuclear…

Atomic Physics · Physics 2018-01-18 A. A. Roenko , K. A. Sveshnikov

The rigorous two-center approach based on the dual-kinetically balanced finite-basis-set expansion is applied to one-electron, heteronuclear diatomic Bi-Au, U-Pb, and Cf-U quasimolecules. The obtained $1\sigma$ ground-state energies are…

We establish a link between quantum mechanical molecular simulations and the transfer matrix of a molecule. The transfer matrix (T-matrix) of an object provides a complete description of its electromagnetic response. Once the T-matrices of…

Chemical Physics · Physics 2020-04-21 Ivan Fernandez-Corbaton , Carsten Rockstuhl , Wim Klopper

Several new formulas are developed that enable the evaluation of a family of definite integrals containing the product of two Whittaker W-functions. The integration is performed with respect to the second index, and the first index is…

Mathematical Physics · Physics 2015-06-26 Peter A. Becker

We give an overview of recent advances in analysis of equations of electrodynamics with the aid of biquaternionic technique. We discuss both models with constant and variable coefficients, integral representations of solutions, a numerical…

Mathematical Physics · Physics 2010-07-09 Kira V. Khmelnytskaya , Vladislav V. Kravchenko

We analyze wave functions constructed as a sum of product of two-electron functions, or as a polynomial of geminals, to investigate their ability to represent the ground state of a strongly correlated few-body system. The known difficulty…

Chemical Physics · Physics 2018-05-17 Airi Kawasaki , Osamu Sugino

Reliable quantum chemical methods for the description of molecules with dense-lying frontier orbitals are needed in the context of many chemical compounds and reactions. Here, we review developments that led to our newcomputational toolbo x…

In principle, many-electron correlation energy can be precisely computed from a reduced Wigner distribution function ($\mathcal{W}$) thanks to a universal functional transformation ($\mathcal{F}$), whose formal existence is akin to that of…

Chemical Physics · Physics 2019-01-23 Rutvij Vihang Bhavsar , Raghunathan Ramakrishnan

The potential curve, dissociation energy, equilibrium internuclear distance, and spectroscopic constants for the ground state of the Ca2 molecule are calculated with the help of the generalized relativistic effective core potential method…

Chemical Physics · Physics 2012-12-27 N. S. Mosyagin , A. N. Petrov , A. V. Titov , A. V. Zaitsevskii

Periodic configurations of electrodes, in particular of microelectrodes, have been of interest since the advent of microfabrication. In this report, theory which is common to any periodic cell (or any cell that can be extended periodically)…

Chemical Physics · Physics 2018-02-13 Cristian F. Guajardo Yévenes , Werasak Surareungchai

We investigate whether the entropic regularisation of the strictly-correlated-electrons problem can be used to build approximations for the kinetic correlation energy functional at large coupling strengths and, more generally, to gain new…

Chemical Physics · Physics 2019-12-13 Augusto Gerolin , Juri Grossi , Paola Gori-Giorgi

Memory function formalism or projection operator technique is an extremely useful method to study the transport and optical properties of various condensed matter systems. A recent revival of its uses in various correlated electronic…

Strongly Correlated Electrons · Physics 2016-09-22 Nabyendu Das , Pankaj Bhalla , Navinder Singh

In this work a general approach to compute a compressed representation of the exponential $\exp(h)$ of a high-dimensional function $h$ is presented. Such exponential functions play an important role in several problems in Uncertainty…

Numerical Analysis · Mathematics 2023-02-22 Martin Eigel , Nando Farchmin , Sebastian Heidenreich , Philipp Trunschke

We introduce two new approximation methods for the numerical evaluation of the long-range Coulomb potential and the approximation of the resulting high dimensional Two-Electron Integrals tensor (TEI) with long-range interactions arising in…

Numerical Analysis · Mathematics 2022-10-25 Siwar Badreddine , Igor Chollet , Laura Grigori