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When applying a voltage bias across a thin nanopore, localized Joule heating can lead to single bubble nucleation, offering a unique platform for studying nanoscale bubble behavior, which is still poorly understood. Accordingly, we…

Bubble nucleation in liquid confined in nanochannel is studied using molecular dynamics simulations and compared against nucleation in the liquid over smooth (i.e. without confinement). Nucleation is achieved by heating part of a surface to…

Fluid Dynamics · Physics 2022-01-24 Manish Gupta , Shalabh C. Maroo

We analyze the properties of naturally formed nano-bubbles in Lennard-Jones molecular dynamics simulations of liquid-to-vapor nucleation in the boiling and the cavitation regimes. The large computational volumes provide a realistic…

Statistical Mechanics · Physics 2015-06-23 Raymond Angélil , Jürg Diemand , Kyoko Tanaka , Hidekazu Tanaka

Recent research has revealed several different techniques for nanoscopic gas nucleation on submerged surfaces, with findings seemingly in contradiction with each other. In response to this, we have systematically investigated the occurrence…

Cavitation, the formation of vapor bubbles in metastable liquids, is highly sensitive to nanoscale surface defects. Using molecular dynamics simulations and classical nucleation theory, we show that pure water confined within defect-free…

Soft Condensed Matter · Physics 2025-01-22 Marin Šako , Fabio Staniscia , Roland R. Netz , Emanuel Schneck , Matej Kanduč

Understanding the nucleation and growth dynamics of the surface bubbles generated on a heated surface can benefit a wide range of modern technologies, such as the cooling systems of electronics, refrigeration cycles, nuclear reactors and…

Acoustic cavitation is known to trigger ice nucleation in supercooled water. Several competing and still debatable mechanisms have been proposed in the literature and are related to the pressure field in the vicinity of the bubble at the…

Chemical Physics · Physics 2018-10-22 Olivier Louisnard , Fabienne Espitalier

The transition from nucleate to film boiling on micro/nano textured surfaces is of crucial importance in a number of practical applications, where it needs to be avoided to enable safe and efficient heat transfer. Previous studies have…

Fluid Dynamics · Physics 2022-07-21 Soumyadeep Paul , Wei-Lun Hsu , Yusuke Ito , Hirofumi Daiguji

Nucleation in small volumes of water has garnered renewed interest due to the relevance of pore condensation and freezing under conditions of low partial pressures of water, such as in the upper troposphere. Molecular simulations can in…

Chemical Physics · Physics 2023-06-23 John A. Hayton , Michael B. Davies , Thomas F. Whale , Angelos Michaelides , Stephen J. Cox

Water electrolysis in a microsystem is observed and analyzed on a short-time scale ~10 us. Very unusual properties of the process are stressed. An extremely high current density is observed because the process is not limited by the…

Soft Condensed Matter · Physics 2013-07-18 Vitaly B. Svetovoy , Remco G. P. Sanders , Miko C. Elwenspoek

We analyze thermodynamics of water samples confined in nanopores and prove that although the freezing temperature can be dramatically lower, the suppression of the ice nucleation leading to the freezing temperature depression is a truly…

Soft Condensed Matter · Physics 2012-06-18 P. O. Fedichev , L. I. Menshikov

We present a multi-scale formalism that accounts for the formation of nano-scale bubbles/cavities owing to a burst of water molecules after the passage of high energy charged particles that leads to the formation of hot non-ionizing…

We study the role of surface topology, surface chemistry, and wall superheat temperature on the onset of boiling, bubble nucleation and growth, and the possible formation of an insulating vapour film by means of large-scale MD simulations.…

Soft Condensed Matter · Physics 2020-07-10 Armin Shahmardi , Outi Tammisola , Mauro Chinappi , Luca Brandt

We report on the nucleation of bubbles on solids that are gently rubbed against each other in a liquid. The phenomenon is found to depend strongly on the material and roughness of the solid surfaces. For a given surface, temperature, and…

Fluid Dynamics · Physics 2016-04-18 Sander Wildeman , Henri Lhuissier , Chao Sun , Detlef Lohse , Andrea Prosperetti

We present results from direct, large-scale molecular dynamics (MD) simulations of homogeneous bubble (liquid-to-vapor) nucleation. The simulations contain half a billion Lennard-Jones (LJ) atoms and cover up to 56 million time-steps. The…

Chemical Physics · Physics 2015-06-23 Jürg Diemand , Raymond Angélil , Kyoko K. Tanaka , Hidekazu Tanaka

The basic physics of nucleation in solid \hl{single-crystal} nanoparticles is revealed by a phase-field theory that includes surface energy, chemical reactions and coherency strain. In contrast to binary fluids, which form arbitrary contact…

Materials Science · Physics 2014-09-17 Daniel A. Cogswell , Martin Z. Bazant

Water can exist in a metastable liquid state under tension for long times before the system relaxes into the vapor via cavitation, i.e., bubble nucleation. Microscopic information on the cavitation process can be extracted from experimental…

Chemical Physics · Physics 2016-10-19 Georg Menzl , Christoph Dellago

Shock wave induced cavitation experiments and atomic force microscopy measurements of flat polyamide and hydrophobized silicon surfaces immersed in water are performed. It is shown that surface nanobubbles, present on these surfaces, do not…

The theory of false vacuum decay in a thermal system may have a cross-over from predominantly thermal transitions to quantum transitions as the temperature is decreased. New numerical methods and results are presented here that can be used…

High Energy Physics - Theory · Physics 2023-03-01 Mario Gutierrez Abed , Ian G. Moss

It has been conjectured that roughness plays a role in surface nucleation, the tendency for freezing to begin preferentially at the liquid-gas interface. Using high speed imaging, we sought evidence for freezing at the contact line on…

Soft Condensed Matter · Physics 2015-06-23 C. W. Gurganus , J. C. Charnawskas , A. B. Kostinski , R. A. Shaw
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