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Related papers: Transient currents in a molecular photo-diode

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We study the electrophoretic flow of suspensions of charged colloids with a mesoscopic method that allows to model generic experimental conditions. We show that for highly charged colloids their electrophoretic mobility increases…

Soft Condensed Matter · Physics 2015-05-28 Giovanni Giupponi , Ignacio Pagonabarraga

We investigate the characteristic effects of nuclear motion on attosecond transient absorption spectra in molecules by calculating the spectrum for different model systems. Two models of the hydrogen molecular ion are considered: one where…

Atomic Physics · Physics 2015-04-16 Jens E. Bækhøj , Lun Yue , Lars Bojer Madsen

The time-dependent tunnelling current arising from the electron-hole recombination of exciton state is theoretically studied using the nonequilibrium Green's function technique and the Anderson model with two energy levels. The charge…

Mesoscale and Nanoscale Physics · Physics 2009-11-11 David M. -T. Kuo

We investigate transport properties of molecular junctions under two types of bias--a short time pulse or an AC bias--by combining a solution for the Green functions in the time domain with electronic structure information coming from ab…

Mesoscale and Nanoscale Physics · Physics 2010-06-18 San-Huang Ke , Rui Liu , Weitao Yang , Harold U. Baranger

Statistical properties of the electron transport flowing through nanostructures are strongly influenced by the interactions, geometry of the system and/or by type of the external electrodes. These factors affect not only the average current…

Mesoscale and Nanoscale Physics · Physics 2020-06-03 Grzegorz Michałek , Bogdan R. Bułka , Tadeusz Domański , Karol I. Wysokiński

The development of attosecond technology has enabled the real-time observation of coherent electron motion in atoms, molecules and condensed phases. Experimentally, it is now possible to generate laser pulses of durations of only a few tens…

Chemical Physics · Physics 2017-05-18 David Ayuso

We investigate transient dynamic response of an Anderson impurity quantum dot to a family of ramp-up driving voltage applied to the single coupling lead. Transient current is calculated based on a hierarchical equations of motion formalism…

Mesoscale and Nanoscale Physics · Physics 2009-11-13 Xiao Zheng , Jinshuang Jin , YiJing Yan

Radiative charge exchange collisions between a carbon atom C(${}^3$P) and a helium ion He+, both in their ground state, are investigated theoretically. Detailed quantum chemistry calculations are carried out to obtain potential energy…

Atomic Physics · Physics 2017-01-25 James F. Babb , B. M. McLaughlin

We present a theoretical analysis of heat transport through a single-molecule junction with two possible transport channels for electrons where interactions between electrons on the molecule and phonons in the nuclear environment is strong…

Mesoscale and Nanoscale Physics · Physics 2023-07-13 Natalya A. Zimbovskaya

An approach is presented to calculate characteristic current vs voltage curves for isolated molecules without explicit description of leads. The Hamiltonian for current-carrying molecules is defined by making resort to Lagrange multipliers,…

Materials Science · Physics 2007-05-23 Anna Painelli

Charge transport through molecular junctions is often described either as a purely coherent or a purely classical phenomenon, and described using the Landauer-B\"uttiker formalism or Marcus theory, respectively. Using a generalised quantum…

Mesoscale and Nanoscale Physics · Physics 2018-10-23 Jakub K. Sowa , Jan A. Mol , G. Andrew D. Briggs , Erik M. Gauger

The wide-band limit is a commonly used approximation to analyze transport through nanoscale devices. In this work we investigate its applicability to the study of charge and heat transport through molecular break junctions exposed to…

Mesoscale and Nanoscale Physics · Physics 2018-05-15 F. Covito , F. G. Eich , R. Tuovinen , M. A. Sentef , A. Rubio

Intense light with frequencies above typical atomic or molecular ionization potentials as provided by free-electron lasers couples many photons into extended targets such as clusters and biomolecules. This implies, in contrast to…

Atomic and Molecular Clusters · Physics 2011-05-25 Christian Gnodtke , Ulf Saalmann , Jan-Michael Rost

Understanding electron transport processes in molecular wires connected between contacts is a central focus in the field of molecular electronics. Especially, the dephasing effect causing tunneling-to-hopping transition has great importance…

Mesoscale and Nanoscale Physics · Physics 2012-06-26 Daijiro Nozaki , Claudia Gomes da Rocha , Horacio M. Pastawski , Gianaurelio Cuniberti

We have studied the electron transport through a quantum dot coupled to three leads in the presence of external microwave fields supplied to different parts of the considered mesoscopic system. Additionally, we introduced a possible…

Mesoscale and Nanoscale Physics · Physics 2009-11-11 T. Kwapinski , R. Taranko , E. Taranko

Based on the assumption that the contact barrier height determines the current flow in organic semiconductor-based electronic devices, charge injection at metal-organic (MO) interfaces has been extensively investigated, while space-charge…

Materials Science · Physics 2009-10-08 Yi Zheng , Andrew T. S. Wee , Cedric Troadec , N. Chandrasekhar

We derive and employ a semi-classical Langevin equation obtained from path-integrals to describe the ionic dynamics of a molecular junction in the presence of electrical current. The electronic environment serves as an effective…

Mesoscale and Nanoscale Physics · Physics 2012-07-03 Jing Tao Lü , Mads Brandbyge , Per Hedegård , Tchavdar N. Todorov , Daniel Dundas

Interfaces between molecules and 2D materials exhibit energy-driven functionalities, wherein charge transfer directs molecular motion. Unlike equilibrium systems, where molecular assemblies settle into static configurations, continuous…

Photo-induced phase-transitions (PIPTs) driven by highly cooperative interactions are of fundamental interest as they offer a way to tune and control material properties on ultrafast timescales. Due to strong correlations and interactions,…

Materials Science · Physics 2022-11-03 Sangeeta Rajpurohit , Jacopo Simoni , Liang Z. Tan

We review recent progresses in the theoretical description of correlation and quantum fluctuation phenomena in charge transport through single molecules, quantum dots, and quantum wires. A variety of physical phenomena is addressed,…

Mesoscale and Nanoscale Physics · Physics 2010-06-28 S. Andergassen , V. Meden , H. Schoeller , J. Splettstoesser , M. R. Wegewijs