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Related papers: Longitudinal magnetic excitation in KCuCl3 studied…

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KCuCl$_3$ is a three dimensionally coupled spin dimer system, which undergoes a pressure-induced quantum phase transition from a gapped ground state to an antiferromagnetic state at a critical pressure of $P_{\rm c} \simeq 8.2$ kbar.…

Strongly Correlated Electrons · Physics 2009-11-13 K. Goto , T. Osakabe , K. Kakurai , Y. Uwatoko , A. Oosawa , J. Kawakami , H. Tanaka

Magnetization and neutron elastic scattering measurements under a hydrostatic pressure were performed on KCuCl3, which is a three-dimensionally coupled spin dimer system with a gapped ground state. It was found that an intradimer…

We report the observation of the $A_{\rm g}$-symmetric one-magnon Raman peak in the magnon Bose-Einstein condensation phase of TlCuCl$_{3}$. Its Raman shift traces the one-magnon energy at the magnetic $\Gamma$ point, and its intensity is…

Strongly Correlated Electrons · Physics 2009-11-13 Haruhiko Kuroe , Kouhei Kusakabe , Akira Oosawa , Tomoyuki Sekine , Fumiko Yamada , Hidekazu Tanaka , Masashige Matsumoto

The combination of electronic correlation and spin-orbit coupling is thought to precipitate a variety of highly unusual electronic phases in solids, including topological and quantum spin liquid states. We report a Raman scattering study…

Strongly Correlated Electrons · Physics 2015-04-22 Luke J. Sandilands , Yao Tian , Kemp W. Plumb , Young-June Kim , Kenneth S. Burch

NH4CuCl3 has two magnetization plateaus at one-quarter and three-quarters of the saturation magnetization, irrespective of the external field direction. Magnetic excitations in NH4CuCl3 have been investigated by means of neutron inelastic…

Strongly Correlated Electrons · Physics 2007-05-23 A. Oosawa , T. Ono , K. Kakurai , H. Tanaka

Raman spectroscopy is used to study magnetic excitations in the quasi one dimensional $S=1/2$ quantum spin systems Cu(Qnx)(Cl$_{1-x}$Br$_x$)$_2$. The low energy spectrum is found to be dominated by a two-magnon continuum as expected from…

Strongly Correlated Electrons · Physics 2016-03-15 G. Simutis , S. Gvasaliya , F. Xiao , C. P. Landee , A. Zheludev

The resonant Raman scattering of a quantum wire in a strong magnetic field is studied, focused on the effect of long range Coulomb interaction and the spin-charge separation. The energy-momentum dispersions of charge and spin excitation…

Mesoscale and Nanoscale Physics · Physics 2009-10-31 H. C. Lee

Pressure-dependent, low temperature inelastic light (Raman) scattering measurements of KCuF$_3$ show that applied pressure above $P^{*} \sim$ 7 kbar suppresses a previously observed structural phase transition temperature to zero…

Strongly Correlated Electrons · Physics 2015-05-28 S. Yuan , M. Kim , J. Seeley , S. Lal , P. Abbamonte , S. L. Cooper

We report on terahertz spectroscopy of quantum spin dynamics in $\alpha$-RuCl$_3$, a system proximate to the Kitaev honeycomb model, as a function of temperature and magnetic field. An extended magnetic continuum develops below the…

Strongly Correlated Electrons · Physics 2017-11-30 Zhe Wang , S. Reschke , D. Hüvonen , S. -H. Do , K. -Y. Choi , M. Gensch , U. Nage , T. Rõõm , A. Loidl

Magnetic Raman scattering from a frustrated spin-1/2 Heisenberg-chain is considered with a focus on the uniform phase of the spin-Peierls compound CuGeO_3. The Raman intensity is analyzed in terms of a Loudon-Fleury scattering process using…

Strongly Correlated Electrons · Physics 2016-08-31 Wolfram Brenig

Long-range entanglement in quantum spin liquids (QSLs) lead to novel low energy excitations with fractionalised quantum numbers and (in 2D) statistics. Experimental detection and manipulation of these excitations present a challenge…

Strongly Correlated Electrons · Physics 2021-11-22 Srishti Pal , Arnab Seth , Piyush Sakrikar , Anzar Ali , Subhro Bhattacharjee , D. V. S. Muthu , Yogesh Singh , A. K. Sood

Magnetic and lattice excitations in the quantum antiferromagnet (C$_4$H$_{12}$N$_2$)Cu$_2$Cl$_6$ (PHCC) are studied across two pressure-induced phase transition at $P_c=4.3~\mathrm{kbar}$ and $P_1=13.4~\mathrm{kbar}$ using Raman…

Strongly Correlated Electrons · Physics 2020-03-17 Simon Bettler , Gediminas Simutis , Gérard Perren , Dominic Blosser , Severian Gvasaliya , Andrey Zheludev

Magnetization maesurements under hydrostatic pressure were performed on an S=1/2 coupled spin system TlCuCl3 with a gapped ground state under magnetic field H parallel to the [2,0,1] direction. With increasing applied pressure P, the gap…

Statistical Mechanics · Physics 2009-11-10 Kenji Goto , Masashi Fujisawa , Toshio Ono , Hidekazu Tanaka , Yoshiya Uwatoko

We report a Raman scattering study of polycrystalline CaCu$_3$Ti$_4$O$_{12}$ (CCTO) under pressure up to 5.32 GPa. The pressure dependence of several Raman modes was investigated. No anomalies have been observed on the phonon spectra…

We investigated temperature dependent Raman spectra of the one-dimensional spin-ladder compound SrCu2O3. At low temperatures a two-magnon peak is identified at 3160+/-10 cm^(-1) and its temperature dependence analyzed in terms of a thermal…

Strongly Correlated Electrons · Physics 2008-01-09 A. Gössling , U. Kuhlmann , C. Thomsen , A. Löffert , C. Gross , W. Assmus

Raman excitation and emission spectra for the radial breathing mode (RBM) are reported, together with a preliminary analysis. From the position of the peaks on the two-dimensional plot of excitation resonance energy against Raman shift, the…

Mesoscale and Nanoscale Physics · Physics 2012-05-11 A. J. Ghandour , A. Sapelkin , I. Hernandez , D. J. Dunstan , I. F. Crowe , M. P. Halsall

We report on the lattice and spin dynamics in the monopnictide CrAs using polarized Raman scattering. This system exhibits a first-order magneto-structural phase transition at T_N~ 265 K, below which the magnetic moments of Cr form an…

Materials Science · Physics 2019-10-07 K. Sen , Y. Yao , R. Heid , A. Omoumi , F. Hardy , K. Willa , M. Merz , A. A. Haghighirad , M. Le Tacon

A pressure and temperature dependent Raman study of the vibrational and spin dynamics in CuGeO3 is presented. A new low temperature, high pressure phase has been identified, and a pressure-temperature phase-diagram is proposed for CuGeO3.…

Strongly Correlated Electrons · Physics 2009-10-28 P. H. M. van Loosdrecht , J. Zeman , G. Martinez , G. Dhalenne , A. Revcolevschi , .

Pressure and temperature dependent susceptibility and Raman scattering experiments on single crystalline Cu_xZn_(1-x)GeO_3 have shown an unusually strong increase of the spin-Peierls phase transition temperature upon applying hydrostatic…

We perform Raman spectroscopy studies on $\alpha$-RuCl$_3$ at room temperature to explore its phase transitions of magnetism and chemical bonding under pressures. The Raman measurements resolve two critical pressures, about $p_1=1.1$~GPa…

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