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Reply to Comment by Flenner and Szamel on our paper in Nature Physics 8, 164 (2012).

Disordered Systems and Neural Networks · Physics 2013-09-09 Walter Kob , Sandalo Roldan-Vargas , Ludovic Berthier

Understanding glass formation is a challenge because the existence of a true glass state, distinct from liquid and solid, remains elusive: Glasses are liquids that have become too viscous to flow. An old idea, as yet unproven…

We investigate the characteristic length scales associated with the glass transition phenomenon. By studying an atomic glass-forming liquid in negatively curved space, for which the local order is well identified and the amount of…

Statistical Mechanics · Physics 2010-02-10 François Sausset , Gilles Tarjus

This is our reply to the comment by Sausset and Tarjus (arXiv:0802.1631) on our paper titled "Correlation between Dynamic Heterogeneity and Medium-Range Order in Two-Dimensional Glass-Forming Liquids" [Phys. Rev. Lett. Vol. 99, No. 21,…

Statistical Mechanics · Physics 2008-02-18 Takeshi Kawasaki , Takeaki Araki , Hajime Tanaka

We numerically obtain the first quantitative demonstration that development of spatial correlations of mobility as temperature is lowered is responsible for the ``decoupling'' of transport properties of supercooled liquids. This result…

Statistical Mechanics · Physics 2009-11-10 Ludovic Berthier

We study theoretically and numerically a family of multi-point dynamic susceptibilities that quantify the strength and characteristic lengthscales of dynamic heterogeneities in glass-forming materials. We use general theoretical arguments…

We present {\it block analysis}, an efficient method to perform finite-size scaling for obtaining the length scale of dynamic heterogeneity and the point-to-set length scale for generic glass-forming liquids. This method involves…

Soft Condensed Matter · Physics 2017-11-22 Saurish Chakrabarty , Indrajit Tah , Smarajit Karmakar , Chandan Dasgupta

Dynamic heterogeneity in glass-formers has been related to their static structure using the concept of dynamic propensity. We re-examine this relationship by analyzing dynamical fluctuations in two atomistic glass-formers and two…

Statistical Mechanics · Physics 2009-08-25 Ludovic Berthier , Robert L. Jack

We report an extensive and systematic investigation of the multi-point and multi-time correlation functions to reveal the spatio-temporal structures of dynamic heterogeneities in glass-forming liquids. Molecular dynamics simulations are…

Soft Condensed Matter · Physics 2013-01-04 Kang Kim , Shinji Saito

We show that in the equilibrium phase of glass-forming hard-sphere fluids in three dimensions, the static length scales tentatively associated with the dynamical slowdown and the dynamical length characterizing spatial heterogeneities in…

Disordered Systems and Neural Networks · Physics 2013-04-16 Patrick Charbonneau , Gilles Tarjus

The dynamics of glass formation in monatomic and binary liquids are studied numerically using a microscopic field theory for the evolution of the time-averaged atomic number density. A stochastic framework combining phase field crystal free…

Materials Science · Physics 2015-05-27 Joel Berry , Martin Grant

In this work we numerically investigate a new method for the characterization of growing length scales associated with spatially heterogeneous dynamics of glass-forming liquids. This approach, motivated by the formulation of the…

Disordered Systems and Neural Networks · Physics 2013-10-28 Kang Kim , Shinji Saito , Kunimasa Miyazaki , Giulio Biroli , David R. Reichman

The existence of heterogeneity in the dynamics of supercooled liquids is believed to be one of the hallmarks of the glass transition. Intense research has been carried out in the past to understand the origin of this heterogeneity in…

Soft Condensed Matter · Physics 2020-07-01 Indrajit Tah , Smarajit Karmakar

The growth of correlation lengths in equilibrium glass-forming liquids near the glass transition is considered a critical finding in the quest to understand the physics of glass formation. These understandings helped us understand various…

Soft Condensed Matter · Physics 2023-08-16 Anoop Mutneja , Smarajit Karmakar

Despite the use of glasses for thousands of years, the nature of the glass transition is still mysterious. On approaching the glass transition, the growth of dynamic heterogeneity has long been thought to play a key role in explaining the…

Soft Condensed Matter · Physics 2018-03-23 Lijin Wang , Ning Xu , W. H. Wang , Pengfei Guan

Dynamical four-point susceptibilities measure the extent of spatial correlations in the dynamics of glass forming systems. We show how these susceptibilities depend on the length scales that necessarily form part of their definition. The…

Statistical Mechanics · Physics 2007-05-23 David Chandler , Juan P. Garrahan , Robert L. Jack , Lutz Maibaum , Albert C. Pan

Understanding the mechanical properties of glasses remains elusive since the glass transition itself is not fully understood, even in well studied examples of glass formers in two dimensions. In this context we demonstrate here: (i) a…

We review the phenomena of dynamical heterogeneity in glass-forming systems and its description within replica and mean-field theories of the glass transition.

Disordered Systems and Neural Networks · Physics 2022-09-08 Giulio Biroli , Kunimasa Miyazaki , David R. Reichman

This is a commentary on two recent experimental papers in PNAS by Vivek et al. and Illing et al. that convincingly address an issue at the junction of two fundamental questions in glass physics: the role of the dimensionality of space on…

Statistical Mechanics · Physics 2022-06-08 Gilles Tarjus

A Comment on the Letter by Atsushi Ikeda and Kunimasa Miyazaki, [arXiv:1003.5472v2, Phys. Rev. Lett. 104, 255704 (2010)].

Soft Condensed Matter · Physics 2011-01-31 Rolf Schilling , Bernhard Schmid
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