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Electric double layers (EDL) with counterions only, say electrons with the elementary charge $-e$, in thermal equilibrium at the inverse temperature $\beta$ are considered. In particular, we study the effect of the surface charge modulation…

Statistical Mechanics · Physics 2022-07-26 Ladislav Šamaj

Stochastic electrodynamics is the classical electrodynamic theory of interacting point charges which includes random classical radiation with a Lorentz-invariant spectrum whose scale is set by Planck's constant. Here we give a cursory…

Classical Physics · Physics 2019-03-05 Timothy H. Boyer

The wetting properties of immiscible two-phase systems are crucial in a wide range of applications, from lab-on-a-chip devices to field-scale oil recovery. It has long been known that effective wetting properties can be altered by the…

Fluid Dynamics · Physics 2018-07-11 Gaute Linga , Asger J. S. Bolet , Joachim Mathiesen

In this review, we shortly summarize the basic theoretical milestones achieved in the mean-field theory of room temperature ionic liquids (RTILs) on charged electrodes since the publication of Kornyshev's seminal paper in 2007. We pay…

Soft Condensed Matter · Physics 2021-12-28 Yury A. Budkov , Andrei L. Kolesnikov

Electrostatic cooling is known to occur in conductors and in porous electrodes in contact with aqueous electrolytes. Here we present for the first time evidence of electrostatic cooling at the junction of two electrolyte phases. These are,…

Chemical Physics · Physics 2019-12-24 S. Porada , H. V. M. Hamelers , P. M. Biesheuvel

We discuss the effect of an external electric field on the wetting of a solid surface by liquid. To this end, we use a model of the two-level-atom fluid for which the changes in interatomic interactions due to the presence of the field can…

Soft Condensed Matter · Physics 2017-02-20 Vasyl Myhal , Oleg Derzhko

The microscopic theory of chemical reactions is based on transition state theory, where atoms or ions transfer classically over an energy barrier, as electrons maintain their ground state. Electron transfer is fundamentally different and…

We briefly discuss our recent field-theoretic study of polyelectrolyte complexation, which occurs in solutions of two oppositely charged polyelectrolytes. Charged systems require theoretical methods beyond the mean-field (or self-consistent…

Soft Condensed Matter · Physics 2015-05-13 Yuri O. Popov , Jonghoon Lee , Glenn H. Fredrickson

Density functional theory can be extended to excited states by means of a unified variational approach for passive state ensembles. This extension overcomes the restriction of the typical density functional approach to ground states, and…

Chemical Physics · Physics 2019-07-10 Tim Gould , Stefano Pittalis

The Darwin approximation is investigated for its possible use in simulation of electromagnetic effects in large size, high frequency capacitively coupled discharges. The approximation is utilized within the framework of two different fluid…

Plasma Physics · Physics 2015-06-11 Denis Eremin , Torben Hemke , Ralf Peter Brinkmann , Thomas Mussenbrock

We consider an osmotic equilibrium between bulk solutions of polyelectrolyte bounded by semipermeable membranes and separated by a thin film of salt-free liquid. Although the membranes are neutral, the counter-ions of the polyelectrolyte…

Soft Condensed Matter · Physics 2012-01-19 Olga I. Vinogradova , Lyderic Bocquet , Artem N. Bogdanov , Roumen Tsekov , Vladimir Lobaskin

The consequences of source charge and surface modulation are studied within the framework of the Poisson-Boltzmann theory of electrolyte solutions. Through a consideration of various examples, it is found that inherent modulation can lead…

Chemical Physics · Physics 2013-05-29 Jonathan Landy

According to classical electrolyte theories interactions in dilute (low ion density) electrolytes decay exponentially with distance, with the Debye screening length the characteristic length-scale. This decay length decreases monotonically…

Soft Condensed Matter · Physics 2016-07-15 Alexander M. Smith , Alpha A. Lee , Susan Perkin

We develop a Boltzmann-Langevin description of Coulomb drag effect in clean double-layer systems with large interlayer separation $d$ as compared to the average interelectron distance $\lambda_F$. Coulomb drag arises from density…

Mesoscale and Nanoscale Physics · Physics 2015-06-10 W. Chen , A. V. Andreev , A. Levchenko

We study the role of steric effects on the induced-charge electro-osmosis (ICEO) phenomenon using a recently developed mesoscale fluid model. A hybrid Eulerian-Lagrangian method is used to simulate the dynamics of discrete immersed ions in…

In the present paper, we develop a semiclassical quasi-static model accounting for molecular double ionization in an intense laser pulse. With this model, we achieve insight into the dynamics of two highly-correlated valence electrons under…

Atomic and Molecular Clusters · Physics 2009-11-13 Di-Fa Ye , Jing Chen , Jie Liu

In this paper, we study the theory of second gradient electromagnetostatics as the static version of second gradient electrodynamics. The theory of second gradient electrodynamics is a linear generalization of higher order of classical…

Classical Physics · Physics 2020-07-03 Markus Lazar , Jakob Leck

We present a model for the rate of temperature relaxation between electrons and ions in plasmas. The model includes self-consistently the effects of particle screening, electron degeneracy and correlations between electrons and ions. We…

Plasma Physics · Physics 2015-05-13 Jérôme Daligault , Guy Dimonte

We study the adsorption-desorption transition of polyelectrolyte chains onto planar, cylindrical and spherical surfaces with arbitrarily high surface charge densities by massive Monte Carlo computer simulations. We examine in detail how the…

Soft Condensed Matter · Physics 2016-10-05 Sidney J. de Carvalho , Ralf Metzler , Andrey G. Cherstvy

We investigate the effect of excluded volume interactions on the electrolyte distribution around a charged macroion. First, we introduce a criterion for determining when hard-core effects should be taken into account beyond standard mean…

Soft Condensed Matter · Physics 2009-11-11 D. Antypov , M. Barbosa , C. Holm