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Rate coefficients for the dissociative recombination, vibrational excitation and vibrational de-excitation of the BeT$^{+}$ ion for all vibrational levels of its ground electronic state ($ X\ensuremath{^{1}\Sigma^{+}},v_{i}^{+}=0,\dots,27$)…

Atomic Physics · Physics 2022-03-09 N. Pop , F. Iacob , S. Niyonzima , A. Abdoulanziz , V. Laporta , D. Reiter , I. F. Schneider , J. Zs Mezei

We show with first-principles molecular dynamics the persistence of intrinsic $\langle111\rangle$ Ti off-centerings for BaTiO$_3$ in its cubic paraelectric phase. Intriguingly, these are inconsistent with the Pm$\bar 3$m space group often…

Materials Science · Physics 2022-04-01 Michele Kotiuga , Samed Halilov , Boris Kozinsky , Marco Fornari , Nicola Marzari , Giovanni Pizzi

Perovskite material such as BCZT (Ba$_{0.875}$Ca$_{0.125}$(Zr$_{0.125}$Ti$_{0.875}$)O$_{3}$) is well known for its high value of piezoceramic properties and Curie temperature which has potential applications in sensors, actuators,…

Materials Science · Physics 2025-03-27 Debidutta Pradhan , Jagadish Kumar

Thermal properties - specific heat and heat conductivity coefficient - of polycrystalline BaTiO3 films on massive substrates were studied as a function of the temperature and the film thickness by ac-hot probe method. The anomalies of…

Variational methods are used to calculate structural and thermodynamical properties of a titrating polyelectrolyte in a discrete representation. The Coulomb interactions are emulated by harmonic repulsive forces, the force constants being…

chem-ph · Physics 2008-02-03 B. Jönsson , M. Ullner , C. Peterson , O. Sommelius , B. Söderberg

Specific-heat measurements are reported near the Curie temperature ($T_C$~= 320 K) on tri-glycine sulfate. Measurements were made on crystals whose surfaces were either non-grounded or short-circuited, and were carried out in magnetic…

Statistical Mechanics · Physics 2008-11-26 J. C. Lashley , C. P. Opeil , T. R. Finlayson , R. A. Fisher , N. Hur , M. F. Hundley , B. Mihaila , J. L. Smith

The effect of electron irradiation with the energy of 2.5 MeV on the temperature dependences of the resistivity of an optimally doped $YBa_2Cu_3O_{7-\delta}$ single crystal has been studied. The temperature dependences of both fluctuation…

Active thermal management requires advances in thermal switching materials, whose thermal conductivity responds to external stimuli. The electric field, as one of the most convenient and effective stimuli, has shown great potential in…

Materials Science · Physics 2025-11-20 Fanghao Zhang , Guanchun Rui , Yujie Quan , Shantal Adajian , Matthew Delmont , Q. M. Zhang , Bolin Liao

The temperature dependence of the rate of the reaction CH_4+H \to CH_3+H_2 is studied using classical collision theory with a temperature-dependent effective potential derived from a path integral analysis. Analytical expressions are…

Chemical Physics · Physics 2016-09-08 David Z. Goodson , Dustin W. Roelse , Wan-Ting Chiang , Steven M. Valone , J. D. Doll

We have investigated the atomistic structure of the 180-degree and 90-degree domain boundaries in the ferroelectric perovskite compound PbTiO3 using a first-principles ultrasoft-pseudopotential approach. For each case we have computed the…

Materials Science · Physics 2009-11-07 B. Meyer , David Vanderbilt

We present theoretical thermally-averaged rate constants for vibrational and rotational (de-)excitation of the H3+ ion by electron impact. The constants are calculated using the multi-channel quantum-defect approach. The calculation…

Atomic Physics · Physics 2015-05-18 Viatcheslav Kokoouline , Alexandre Faure , Jonathan Tennyson , Chris H. Greene

We present molecular dynamics simulations of a realistic model of an ultrathin film of BaTiO$_3$ sandwiched between short-circuited electrodes to determine and understand effects of film thickness, epitaxial strain and the nature of…

Materials Science · Physics 2009-11-13 Jaita Paul , Takeshi Nishimatsu , Y. Kawazoe , Umesh V. Waghmare

The large electrocaloric coupling in PbZrO3 allows using high-speed infrared imaging to visualize antiferroelectric switching dynamics via the associated temperature change. We find that in ceramic samples of homogeneous temperature and…

High-temperature electronic materials are in constant demand as the required operational range for various industries increases. Here we design $(A,A^\prime)B_2$O$_6$ perovskite oxides with [111] ``rock salt" $A$-site cation order and…

Materials Science · Physics 2014-06-11 Joshua Young , James M. Rondinelli

In this work we explore the overall structural behaviour of the [(CH3)2NH2][Mn(HCOO)3] multiferroic compound across the temperature range where its ferroelectric transition takes place by means of calorimetry, thermal expansion measurements…

We investigate the influence of quantum effects on the dielectric and piezoelectric properties of barium titanate in its (low-temperature) rhombohedral phase, and show the strongly anharmonic character of this system even at low…

Materials Science · Physics 2015-06-12 Gregory Geneste , Hichem Dammak , Marc Hayoun , Mickael Thiercelin

Potassium niobate (KNbO3) is a prototypical perovskite ferroelectric with large electro-optic and nonlinear optical responses, high optical damage thresholds and a rich sequence of temperature-driven phase transformations, making it a…

Materials Science · Physics 2026-01-27 Aiden Ross , Venkatraman Gopalan , Long-Qing Chen

This paper presents a multiscale approach to evaluate perovskite solar cell performance which determines material properties at the atomistic scale with first-principles calculations, and applies them in macro-scale device models. This work…

Lattice constant of Bi$_2$Se$_3$ and Sb$_2$Te$_3$ crystals is determined by X-ray powder diffraction measurement in a wide temperature range. Linear thermal expansion coefficients ($\alpha$) of the crystals are extracted, and considerable…

Strontium titanate (SrTiO3) is regarded as an essential material for oxide electronics. One of its many remarkable features is subtle structural phase transition, driven by antiferrodistortive lattice mode, from a high-temperature cubic…

Materials Science · Physics 2022-03-02 Ri He , Hongyu Wu , Linfeng Zhang , Xiaoxu Wang , Fangjia Fu , Shi Liu , Zhicheng Zhong