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Related papers: Fluorographynes: Stability, Structural and Electro…

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In this letter we study the electronic structures and optical properties of partially and fully fluorinated graphene by a combination of abinitio G0W0 calculations and large-scale multi-orbital tight-binding simulations. We find that for…

Mesoscale and Nanoscale Physics · Physics 2015-02-25 Shengjun Yuan , Malte Rosner , Alexander Schulz , Tim O. Wehling , Mikhail I. Katsnelson

Using ab initio methods we have investigated the fluorination of graphene and find that different stoichiometric phases can be formed without a nucleation barrier, with the complete "2D-Teflon" CF phase being thermodynamically most stable.…

Materials Science · Physics 2011-01-26 Morgana A. Ribas , Abhishek K. Singh , Pavel B. Sorokin , Boris I. Yakobson

We performed a first principles investigation on the structural and electronic properties of group-IV (C, SiC, Si, Ge, and Sn) graphene-like sheets in flat and buckled configurations and the respective hydrogenated or fluorinated…

Materials Science · Physics 2012-04-16 Joelson Cott Garcia , Denille B. de Lima , Lucy V. C. Assali , João F. Justo

Recent synthesis of fluorinated graphene introduced interesting stable derivatives of graphene. In particular, fluorographene (CF), namely fully fluorinated chair conformation, is found to display crucial features, such as high mechanical…

Materials Science · Physics 2015-03-19 Hasan Sahin , Mehmet Topsakal , Salim Ciraci

DFT calculations of the electronic structure of graphane and stoichiometrically halogenated graphene derivatives (fluorographene and other analogous graphene halides) show (i) localized orbital basis sets can be successfully and effectively…

Materials Science · Physics 2012-09-20 František Karlický , Radek Zbořil , Michal Otyepka

Heterostructures prepared from graphene and fluorographene (FG) using the technology of 2D printing on solid and flexible substrates were fabricated and studied. Excellent stability of printed graphene layers and, to a lesser degree,…

We report a stoichiometric derivative of graphene with a fluorine atom attached to each carbon. Raman, optical, structural, micromechanical and transport studies show that the material is qualitatively different from the known…

\textit{Ab initio} calculations within the density functional theory formalism are performed to investigate the stability and electronic properties of fluorinated bilayer graphene (bilayer fluorographene). A comparison is made to previously…

Materials Science · Physics 2013-01-25 Jozef Sivek , Ortwin Leenaerts , Bart Partoens , Francois Peeters

Density functional modeling of atomic structure and calculation of electronic structure of one-side one-sublattice functionalized graphene (graphone) are performed for hydrogen and fluorine adatoms. Shown that using of fluorine for…

Mesoscale and Nanoscale Physics · Physics 2015-05-19 D. W. Boukhvalov

Different stoichiometric configurations of graphane and graphene fluoride are investigated within density functional theory. Their structural and electronic properties are compared, and we indicate the similarities and differences among the…

Materials Science · Physics 2011-11-23 O. Leenaerts , H. Peelaers , A. D. Hernandez-Nieves , B. Partoens , F. M. Peeters

A systematic study is conducted on the fluorination-enriched essential properties of 2D graphene and 1D graphene nanoribbons using the first-principles method. The combined effects, which arise from the significant chemical bonds in C-C,…

Materials Science · Physics 2017-12-21 Khanh Duy Nguyen , Thuy Ngoc Thanh Tran , Tien Thanh Nguyen , Yu-Huang Chiu , Ming-Fa Lin

A density functional theory study of the structural and electronic properties and relative stability of fluorinated sp3 silicon nanotubes and their corresponding silicon nanowires built along various crystallographic orientations is…

Materials Science · Physics 2013-08-07 Alon Hever , Jonathan Bernstein , Oded Hod

The microscopic knowledge of the structural, energetic, and electronic properties of scandium fluoride is still incomplete, despite the relevance of this material as an intermediate for the manufacturing of Al-Sc alloys. In a work based on…

Phosphorene, the monolayer form of the (black) phosphorus, was recently exfoliated from its bulk counterpart. Phosphorene oxide, by analogy to graphene oxide, is expected to have novel chemical and electronic properties, and may provide an…

Materials Science · Physics 2015-06-22 Gaoxue Wang , Ravindra Pandey , Shashi P. Karna

Graphynes and graphdiynes are carbon 2D allotrope structures presenting both sp2 and sp hybridized atoms. These materials have been theoretically predicted but due to intrinsic difficulties in their synthesis, only recently some of these…

Mesoscale and Nanoscale Physics · Physics 2017-02-21 Daniel Solis , Cristiano F. Woellner , Daiane D. Borges , Douglas S. Galvao

We study the electronic structure of diluted F atoms chemisorbed on graphene using density functional theory calculations. We show that the nature of the chemical bonding of a F atom adsorbed on top of a C atom in graphene strongly depends…

Mesoscale and Nanoscale Physics · Physics 2015-03-18 J. O. Sofo , A. M. Suarez , Gonzalo Usaj , P. S. Cornaglia , A. D. Hernández-Nieves , C. A. Balseiro

Based on first principles calculation, the electronic properties of graphene on metal (Ti, Ca, Ni, Mn, Co, Fe, Cr, K) modified SiO2 substrate have been studied. The results of binding energies supported graphene indicate that the metal…

Mesoscale and Nanoscale Physics · Physics 2012-03-02 L. Shen , F. Jiang , M. Xiao , R. Zhang , M. X. Yu , L. Miao , J. J. Jiang

We give the results of density functional calculations for graphene with a widely varying fluorine adsorptions. We give a systematic analysis of the adsorption energies, lattice constants, bulk modulus, bandgap openings, and magnetic…

Materials Science · Physics 2014-11-13 Chad E. Junkermeier , Stefan C. Badescu , Thomas L. Reinecke

The feature-rich electronic and magnetic properties of fluorine-doped graphene nanoribbons are investigated by the first-principles calculations. They arise from the cooperative or competitive relations among the significant chemical bonds,…

Mesoscale and Nanoscale Physics · Physics 2017-03-01 Duy Khanh Nguyen , Yu-Tsung Lin , Shih-Yang Lin , Yu-Huang Chiu , Ngoc Thanh Thuy Tran , Ming Fa-Lin

Graphene functionalization by hydrogen and fluorine has been proposed as a route to modulate its reactivity and electronic properties. However, until now, proposed systems present degradation and limited hydrogen adsorption capacity. In…

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