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We demonstrate that the driving forces for ion adsorption to the air-water interface for point charge models results from both cavitation and a term that is of the form of a negative electrochemical surface potential. We carefully…

Soft Condensed Matter · Physics 2013-07-08 Marcel D. Baer , Abraham C. Stern , Yan Levin , Douglas J. Tobias , Christopher J. Mundy

Specific molecular interactions underlie unexpected and useful phenomena in nanofluidic systems, but require descriptions that go beyond traditional macroscopic hydrodynamics. In this letter, we demonstrate how equilibrium molecular…

Mesoscale and Nanoscale Physics · Physics 2023-06-07 Phillip Helms , Anthony R. Poggioli , David T. Limmer

In systems composed of water and hydrocarbons Van der Waals-interactions are dominated by the non-retarded, classical (Keesom) part of the Lifshitz-interaction; the interaction is screened by salt and extends over mesoscopic distances of…

Statistical Mechanics · Physics 2007-11-09 I. Pasichnyk , R. Everaers , A. C. Maggs

Bipolar nanopores have powerful rectification properties due to the asymmetry in the charge pattern on the wall of the nanopore. In particular, bipolar nanopores have positive and negative surface charges along the pore axis. Rectification…

Soft Condensed Matter · Physics 2020-11-25 Dávid Fertig , Mónika Valiskó , Dezső Boda

We study a two-dimensional fluid of dipolar hard disks by Monte Carlo simulations in a square with periodic boundary conditions and on the surface of a sphere. The theory of the dielectric constant and the asymptotic behaviour of the…

Soft Condensed Matter · Physics 2015-10-28 Jean-Michel Caillol , Jean-Jacques Weis

Grand canonical Monte Carlo simulation results are reported for an electric double layer modelled by a planar charged hard wall, anisotropic shape cations, and spherical anions at different electrolyte concentrations and asymmetric…

Soft Condensed Matter · Physics 2016-03-09 M. Kaja , S. Lamperski , W. Silvestre-Alcantara , L. B. Bhuiyan , D. Henderson

Neutral molecules with sufficiently large dipole moments can bind electrons in diffuse nonvalence orbitals with most of their charge density far from the nuclei, forming so-called dipole-bound anions. Because long-range correlation effects…

Chemical Physics · Physics 2018-10-30 Hongxia Hao , James Shee , Shiv Upadhyay , Can Ataca , Kenneth D. Jordan , Brenda M. Rubenstein

We study ion condensation onto a patterned surface of alternating charges. The competition between self-energy and ion-surface interactions leads to the formation of ionic crystalline structures at low temperatures. We consider different…

Statistical Mechanics · Physics 2009-11-13 Yuri S. Velichko , Francisco J. Solis , Sharon M. Loverde , Monica Olvera de la Cruz

We present the theory for retarded resonance interaction between two identical atoms at arbitrary positions near a metal surface. The dipole-dipole resonance interaction force that binds isotropically excited atom pairs together in free…

Materials Science · Physics 2013-04-10 Mathias Boström , Clas Persson , Barry W. Ninham , Patrick Norman , Bo E. Sernelius

Screening of a strongly charged macroion by oppositely charged colloidal particles, micelles, or short polyelectrolytes is considered. Due to strong lateral repulsion such multivalent counterions form a strongly correlated liquid at the…

Soft Condensed Matter · Physics 2009-10-31 T. T. Nguyen , A. Yu. Grosberg , B. I. Shklovskii

Electrostatic correlations and variable permittivity of electrolytes are essential for exploring many chemical and physical properties of interfaces in aqueous solutions. We propose a continuum electrostatic model for the treatment of these…

Soft Condensed Matter · Physics 2015-06-23 Manman Ma , Zhenli Xu

The presence of strong interactions in a many-body quantum system can lead to a variety of exotic effects. Here we show that even in a comparatively simple setup consisting of a charged impurity in a weakly interacting bosonic medium the…

Quantum Gases · Physics 2021-05-13 G. E. Astrakharchik , L. A. Peña Ardila , R. Schmidt , K. Jachymski , A. Negretti

Very recently the effect of equisized charged hard sphere solutes in a mixture with core-softened fluid model on the structural and thermodynamic anomalies of the system has been explored in detail by using Monte Carlo simulations and…

Soft Condensed Matter · Physics 2013-12-18 B. Hribar-Lee , O. Pizio

The forces between charged macromolecules, usually given in terms of osmotic pressure, are highly affected by the intervening ionic solution. While in most theoretical studies the solution is treated as a homogeneous structureless…

Soft Condensed Matter · Physics 2014-04-22 Dan Ben-Yaakov , David Andelman , Daniel Harries , Rudi Podgornik

Strong light-induced interactions between atoms are known to cause nonlinearities at a few-photon level which are crucial for applications in quantum information processing. Compared to free space, the scattering and the light-induced…

Quantum Physics · Physics 2021-12-22 Artur Skljarow , Harald Kübler , Charles S. Adams , Tilman Pfau , Robert Löw , Hadiseh Alaeian

Most organic and inorganic surfaces (e.g., glass, nucleic acids or lipid membranes) become charged in aqueous solutions. The resulting ionic distribution induces effective interactions between the charged surfaces. Stacks of like-charged…

In order to detect the effect of the surface charge discreteness on the properties at the solid-liquid interface, molecular dynamics simulation model taking consideration of the vibration of wall atoms was used to investigate the ion and…

Chemical Physics · Physics 2016-12-20 Yinghua Qiu , Yunfei Chen

Electrostatic correlation effects in inhomogeneous symmetric electrolytes are investigated within a previously developed electrostatic self-consistent (SC) theory (R.R. Netz and H. Orland, Eur. Phys.J. E 11, 301 (2003)). To this aim, we…

Soft Condensed Matter · Physics 2015-06-05 Sahin Buyukdagli , Cristian Achim , Tapio Ala-Nissila

Recent experiments (F.H.J. Van Der Heyden et al., PRL 96, 224502 (2006)) of streaming currents in silica nanochannels with divalent ions report charge inversion, i.e. interfacial charges attracting counterions in excess of their own nominal…

Materials Science · Physics 2007-06-26 Christian D. Lorenz , Alex Travesset

We apply a phenomenological theory of polar liquids to calculate the interaction energy between two plane surfaces at nm-distances. We show that depending on the properties of the surface-liquid interfaces, the interacting surfaces induce…

Soft Condensed Matter · Physics 2013-04-24 P. O. Fedichev , L. I. Menshikov