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We develop a technique for generating a set of optimized local basis functions to solve models in the Kohn-Sham density functional theory for both insulating and metallic systems. The optimized local basis functions are obtained by solving…

Computational Physics · Physics 2015-05-30 Lin Lin , Jianfeng Lu , Lexing Ying , E. Weinan

Closed bipartite quantum systems subject to fast local unitary control are studied using quantum optimal control theory and a method of reduced control systems based on the Schmidt decomposition. Particular focus is given to the…

Quantum Physics · Physics 2024-05-31 Emanuel Malvetti , Léo Van Damme

We focus on finding a coarse grained description able to reproduce the thermodynamic behavior of a molecular system by using mesoparticles representing several molecules. Interactions between mesoparticles are modelled by an interparticle…

Soft Condensed Matter · Physics 2015-06-17 Gerome Faure , Jean-Bernard Maillet , Gabriel Stoltz

Aiming to combine density functional theory (DFT) and wavefunction theory, we study a mapping from the many-body interacting system to an effectively-interacting Kohn-Sham system instead of a non-interacting Kohn-Sham system. Because a…

Chemical Physics · Physics 2020-02-19 Shunsuke A. Sato , Angel Rubio

The exchange-correlation energy in Kohn-Sham density functional theory can be expressed exactly in terms of the change in the expectation of the electron-electron repulsion operator when, in the many-electron hamiltonian, this same operator…

Strongly Correlated Electrons · Physics 2009-08-05 Paola Gori-Giorgi , Giovanni Vignale , Michael Seidl

A single-term density functional model for nondynamic and strong correlation is presented, based on single-determinant Kohn-Sham density functional theory. It is derived from modeling the adiabatic connection and contains only two nonlinear…

Chemical Physics · Physics 2015-12-21 Jing Kong , Emil Proynov

Accurate control of quantum states is crucial for quantum computing and other quantum technologies. In the basic scenario, the task is to steer a quantum system towards a target state through a sequence of control operations. Determining…

Quantum Physics · Physics 2024-06-14 Yan Zhu , Tailong Xiao , Guihua Zeng , Giulio Chiribella , Ya-Dong Wu

We extend random matrix theory to consider randomly interacting spin systems with spatial locality. We develop several methods by which arbitrary correlators may be systematically evaluated in a limit where the local Hilbert space dimension…

Statistical Mechanics · Physics 2020-01-08 Siddhardh C. Morampudi , Chris R. Laumann

An explicit expression for the quadratic density-response function of a many-electron system is obtained in the framework of the time-dependent density-functional theory, in terms of the linear and quadratic density-response functions of…

Materials Science · Physics 2009-11-10 V. U. Nazarov , J. M. Pitarke , C. S. Kim , Y. Takada

Kohn-Sham (KS) density functional theory (DFT) is a very efficient method for calculating various properties of solids as, for instance, the total energy, the electron density, or the electronic band structure. The KS-DFT method leads to…

Materials Science · Physics 2019-09-20 Fabien Tran , Jan Doumont , Leila Kalantari , Ahmad W. Huran , Miguel A. L. Marques , Peter Blaha

We propose an active-space approximation to reduce the quantum resources required for variational quantum eigensolver (VQE). Starting from the double exponential unitary coupled-cluster ansatz and employing the downfolding technique, we…

Strongly Correlated Electrons · Physics 2023-06-06 Nhan Trong Le , Lan Nguyen Tran

A precise time-dependent control of a quantum system relies on an accurate account of the quantum interference among the system, the control and the environment. A diagrammatic technique has been recently developed to precisely calculate…

Mesoscale and Nanoscale Physics · Physics 2015-05-30 Ching-Kit Chan , L. J. Sham

We propose a local, O(N) molecular dynamics algorithm for the simulation of charged systems. The long ranged Coulomb potential is generated by a propagating electric field that obeys modified Maxwell equations. On coupling the…

Soft Condensed Matter · Physics 2009-11-10 Jörg Rottler , A. C. Maggs

Local noise can produce quantum correlations on an initially classically correlated state, provided that it is not represented by a unital or semi-classical channel \cite{DagmarBruss}. We find the power of any given local channel for…

Quantum Physics · Physics 2015-06-12 Tahere Abad , Vahid Karimipour , Laleh Memarzadeh

We investigate the influence of an additional bosonic bath onto the real-time dynamics of a localized orbital coupled to conduction band with an energy-dependent coupling function $\Gamma(\varepsilon) \propto |\varepsilon|^r$. Recently, a…

Strongly Correlated Electrons · Physics 2015-12-22 Christian Kleine , Frithjof B. Anders

Qubit reset is crucial in quantum technology and is typically achieved by coupling the qubit to a dissipative environment. However, the achievable speed and fidelity are limited by qubit-environment entanglement. We use exact tensor-network…

Quantum Physics · Physics 2026-03-11 Carlos Ortega-Taberner , Eoin O'Neill , Paul Eastham

External potentials play a crucial role in modelling quantum systems, since, for a given inter- particle interaction, they define the system Hamiltonian. We use the metric space approach to quantum mechanics to derive, from the energy…

Quantum Physics · Physics 2017-01-04 P. M. Sharp , I. D'Amico

In the density functional (DF) theory of Kohn and Sham, the kinetic energy of the ground state of a system of noninteracting electrons in a general external field is calculated using a set of orbitals. Orbital free methods attempt to…

Strongly Correlated Electrons · Physics 2009-11-13 Jeng-Da Chai , John D Weeks

Enhanced experimental capabilities to control nonlocal and power-law decaying interactions are currently fuelling intense research in the domain of quantum many-body physics. Compared to their counterparts with short-ranged interactions,…

Statistical Mechanics · Physics 2025-09-16 Robert Mattes , Igor Lesanovsky , Federico Carollo

The study of density-dependent stochastic population processes is important from a historical perspective as well as from the perspective of a number of existing and emerging applications today. In more recent applications of these…

Optimization and Control · Mathematics 2017-09-26 Yingdong Lu , Mark Squillante , Chai Wah Wu