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In this work multiferroic thin films of Bi containing perovskite oxides are discussed, where the driving force for ferroelectricity are the Bi3+ lone-pair electrons. First, a brief introduction of Bi containing multiferroic perovskite…

Strongly Correlated Electrons · Physics 2014-02-11 Rainer Schmidt , Eric Langenberg , Jofre Ventura , Manuel Varela

B-site ordered thin films of double perovskite Sr$_2$CoIrO$_6$ were epitaxially grown by a metal-organic aerosol deposition technique on various substrates, actuating different strain states. X-ray diffraction, transmission electron…

Strongly Correlated Electrons · Physics 2018-05-23 S. Esser , C. F. Chang , C. -Y. Kuo , S. Merten , V. Roddatis , T. D. Ha , A. Jesche , V. Moshnyaga , H. -J. Lin , A. Tanaka , C. T. Chen , L. H. Tjeng , P. Gegenwart

Multiferroics are a unique class of materials where magnetic and ferroelectric orders coexist. The research on multiferroics contributes significantly to the fundamental understanding of the strong correlations between different material…

Materials Science · Physics 2021-11-03 A. C. Garcia-Castro , Yanjun Ma , Zachary Romestan , Eric Bousquet , Cheng Cen , Aldo H. Romero

Piezoelectrics interconvert mechanical energy and electric charge and are widely used in actuators and sensors. The best performing materials are ferroelectrics at a morphotropic phase boundary (MPB), where several phases can intimately…

We present a first-principles study of multiferroic BiFeO3 at high pressures. Our work reveals the main structural (change in Bi's coordination and loss of ferroelectricity), electronic (spin crossover and metallization), and magnetic (loss…

Materials Science · Physics 2009-12-17 O. E. Gonzalez-Vazquez , Jorge Iniguez

Chiral interactions within magnetic layers stabilize the formation of noncollinear spin textures, which can be leveraged to design devices with tailored magnetization dynamics. Here, we introduce chiral spin frustration in which…

Anisotropic strain engineering in epitaxial oxide films provides new opportunities to control the antiferromagnetic and structural properties crucial for advancements of antiferromagnetic spintronics. Here we report on a…

Antiferromagnetic thin films are currently generating considerable excitement for low dissipation magnonics and spintronics. However, while tuneable antiferromagnetic textures form the backbone of functional devices, they are virtually…

Magnetoelectric multiferroics, materials with intrinsically coupled electric polarization and magnetic order, promise ultralow-power switching, nonvolatile memory, and energy-efficient signal transduction. Yet practical deployment demands…

In the context of magnetism, frustration arises when a group of spins cannot find a configuration that minimizes all of their pairwise interactions simultaneously. We consider the effects of the geometric frustration that arises in a…

Statistical Mechanics · Physics 2015-05-19 A. Jagannathan , B. Motz , E. Vedmedenko

We describe the directional growth of ferroelectric domains in a multiferroic BiFeO3 thin film, which was grown epitaxially on a vicinal (001) SrTiO3 substrate. A detailed structural analysis of the film shows that a strain gradient, which…

Mesoscale and Nanoscale Physics · Physics 2015-05-14 T. H. Kim , S. -H. Baek , S. M. Yang , S. Y. Jang , D. Ortiz , T. K. Song , J. -S. Chung , C. -B. Eom , T. W. Noh , J. -G. Yoon

The quantitative understanding of converse magnetoelectric effects, i.e., the variation of the magnetization as a function of an applied electric field, in extrinsic multiferroic hybrids is a key prerequisite for the development of future…

Materials Science · Physics 2014-09-23 S. Geprägs , D. Mannix , M. Opel , S. T. B. Goennenwein , R. Gross

The dependencies on strain and oxygen vacancies of the ferroelectric polarization and the weak ferromagnetic magnetization in the multiferroic material bismuth ferrite, BiFeO_3, are investigated using first principles density functional…

Materials Science · Physics 2007-05-23 Claude Ederer , Nicola A. Spaldin

By performing first-principles calculations, we systematically explore the effect of epitaxial strain on the structure and properties of multiferroic TbMnO3. We show that, although the unstrained bulk TbMnO3 displays a non-collinear…

Materials Science · Physics 2015-05-20 Yusheng Hou , Jihui Yang , Xingao Gong , Hongjung Xiang

Elastic strain is potentially an important approach in tuning the properties of the improperly multiferroic hexagonal ferrites, the details of which have however been elusive due to the experimental difficulties. Employing the method of…

Due to the wide range of applications, theoretical models of Fe3O4 films are found to be important. Ultra thin Fe3O4 films with ferrite structure have been theoretically investigated using second order perturbed modified Heisenberg…

Materials Science · Physics 2019-02-26 P. Samarasekara

Highly ordered Bi2FeMnO6 epitaxial thin films have been successfully grown on SrTiO3 substrate. Both synchrotron X-ray reciprocal space mapping and high resolution transmission electron microscopy confirmed the alternative alignment of Fe…

Non-collinear spin order that breaks space inversion symmetry and allows efficient electric-field control of magnetism makes BiFeO$_3$ a promising candidate for applications in low-power spintronic devices. Epitaxial strain effects have…

The structural and ferroelectric domain variants of highly-strained BiFeO3 films grown on vicinal LaSrAlO4 substrates were studied by piezoelectric force microscopy and high-resolution X-ray reciprocal space mapping. Through symmetry…

Materials Science · Physics 2015-06-04 Lu You , Shintaro Yasui , Xi Zou , Hui Ding , Zuhuang Chen , Weigang Chen , Lang Chen , Hiroshi Funakubo , Junling Wang

The effect of high tensile strain and low dimensionality on the magnetic and electronic properties of CaMnO$_3$ ultrathin films, epitaxially grown on SrTiO$_3$ substrates, are experimentally studied and theoretically analyzed. By means of…

Materials Science · Physics 2020-09-02 A. López Pedroso , M. A. Barral , M. E. Graf , A. M. Llois , M. H. Aguirre , L. B. Steren , S. Di Napoli