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Magnetically-driven ferroelectric atomic displacements of the order of 10$^{-3} Angstrom have been observed in orthorhombic (perovskite like) YMnO$_3$ by a single-crystal synchrotron x-ray diffraction. The refined polar structure shows the…

Strongly Correlated Electrons · Physics 2011-08-12 D. Okuyama , S. Ishiwata , Y. Takahashi , K. Yamauchi , S. Picozzi , K. Sugimoto , H. Sakai , M. Takata , R. Shimano , Y. Taguchi , T. Arima , Y. Tokura

The ferroelectric trends of rutile (TiO$_2$) in bulk and at the (110) surface are investigated by means of ab initio density functional theory. We discuss the underlying mechanism of the incipient ferroelectric behavior of rutile in terms…

Materials Science · Physics 2015-06-12 Anna Grünebohm , Peter Entel , Claude Ederer

We demonstrate that small but finite ferroelectric polarization ($\sim$0.01 $\mu$C/cm$^2$) emerges in orthorhombic LuFeO$_3$ ($Pnma$) at $T_N$ ($\sim$600 K) because of commensurate (k = 0) and collinear magnetic structure. The synchrotron…

Electronic, lattice, and spin interactions at the interfaces between crystalline complex transition metal oxides can give rise to a wide range of functional electronic and magnetic phenomena not found in bulk. At hetero-interfaces, these…

Strongly Correlated Electrons · Physics 2017-08-03 S. Koohfar , A. S. Disa , M. Marshall , F. J. Walker , C. H. Ahn , D. P. Kumah

Although multiferroics have undergone extensive examination for several decades, the occurrence of ferroelectricity induced by orbital order is only scarcely documented. In this study, we propose the existence of spontaneous ferroelectric…

Materials Science · Physics 2025-01-07 Xiao-Feng Luo , Xu He , Rui Wang , Hongjun Xiang , Jin-Zhu Zhao

Flexoelectricity is a universal effect that generates electric polarization due to broken inversion symmetry caused by local strain gradient. The large strain gradient at nanoscale makes flexo-electric effects, especially in nanoscopic…

Materials Science · Physics 2025-05-30 Xin Li , Guodong Ren , Yu Yun , Arashdeep Singh Thind , Amit Kumar Shah , Abbey Bowers , Rohan Mishra , Xiaoshan Xu

Hydrostatic pressure and oxygen vacancies usually have deleterious effects on ferroelectric materials because both tend to reduce their polarization. In this work we use first-principles calculations to study an important class of…

Materials Science · Physics 2021-12-15 Chengliang Xia , Yue Chen , Hanghui Chen

The past decade's discovery of topological excitations in nanoscale ferroelectrics has turned the prevailing view that the polar ground state in these materials is uniform. However, the systematic understanding of the topological polar…

Mesoscale and Nanoscale Physics · Physics 2023-04-05 Svitlana Kondovych , Maksim Pavlenko , Yurii Tikhonov , Anna Razumnaya , Igor Lukyanchuk

We model short-period superlattices of WO$_3$ and ReO$_3$ with first-principles calculations. In fully-relaxed superlattices, we observe that octahedral tilts about an axis in the planes of the superlattices do not propagate from one…

Materials Science · Physics 2014-06-02 Joseph T. Schick , Lai Jiang , Diomedes Saldana-Greco , Andrew M. Rappe

Electric fields have played a key role in discovering and controlling exotic electronic states of condensed matter. However, electric fields usually do not work in metals as free carriers tend to screen electrostatic fields. While a…

The commensurate and incommensurate magnetic structures of the magnetoelectric system YMn$_{2}$O$_{5}$, as determined from neutron diffraction, were found to be spin-density waves lacking a global center of symmetry. We propose a model,…

Materials Science · Physics 2009-11-11 L. C. Chapon , P. G. Radaelli , G. R. Blake , S. Park , S-W. Cheong

The instability of ferroelectric ordering in ultra-thin films is one of the most important fundamental issues pertaining realization of a number of electronic devices with enhanced functionality, such as ferroelectric and multiferroic…

Double-perovskite A2BB'O6 oxides with magnetic B and B' ions and E*-type antiferromagnetic order (E*-AFM, i.e. the ++-- structure) are believed to exhibit promising multiferroic properties, and Y2CoMnO6 (YCMO) is one candidate in this…

Materials Science · Physics 2015-10-28 C. Y. Ma , S. Dong , P. X. Zhou , Z. Z. Du , M. F. Liu , H. M. Liu , Z. B. Yan , J. M. Liu

We calculate from first principles the nonlinear piezoelectric response of ferroelectric PbTiO3 for the case of a polarization-enhancing electric field applied along the tetragonal axis. We focus mainly on the case of fixed in-plane lattice…

Materials Science · Physics 2011-03-03 Anindya Roy , Massimiliano Stengel , David Vanderbilt

Using first-principles density functional theoretical analysis, we predict coexisting ferroelectric and semi-metallic states in two-dimensional monolayer of h-NbN subjected to electric field and in-plane strain ($\epsilon$). At strains…

Mesoscale and Nanoscale Physics · Physics 2019-07-24 Anuja Chanana , Umesh V. Waghmare

Density functional calculations are performed to study the effect of epitaxial strain on PbZrO3. We find a remarkably small energy difference between the epitaxially strained polar R3c and nonpolar Pbam structures over the full range of…

Materials Science · Physics 2014-05-15 Sebastian E. Reyes-Lillo , Karin M. Rabe

We construct ferroelectric (LuFeO3)m/(LuFe2O4) superlattices with varying index m to study the effect of confinement on topological defects. We observe a thickness-dependent transition from neutral to charged domain walls and the emergence…

We use density-functional theory with the local-density approximation to study the structural and ferroelectric properties of SrTiO$_3$ under misfit strains. Both the antiferrodistortive (AFD) and ferroelectric (FE) instabilities are…

Materials Science · Physics 2009-11-11 Chien-Hung Lin , Chih-Meng Huang , G. Y. Guo

The perovskite oxide EuTiO3 (ETO) has attracted increased scientific interest due to its potential multiferroic properties and magnetic activity above and below its structural phase transition at TS=282K. Various experiments have indirectly…

Perovskite oxide ferroelectrics show classical soft mode behaviour typical for the onset of a homogeneous long-range polar state and a displacive phase transition. Besides these long wave length properties, local effects are observed by…

Other Condensed Matter · Physics 2007-05-23 A. Bussmann-Holder , H. Buettner , A. R. Bishop