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A new method of estimating high-order virial coefficients for fluids composed of equal three-dimensional rigid spheres is proposed. The predicted $B_{11}$ and $B_{12}$ values are in good agreement with reliable estimates previously…

Statistical Mechanics · Physics 2014-03-07 C. C. F. Florindo , A. B. M. S. Bassi

The fourth virial coefficient is calculated exactly for a fluid of hard spheres in odd dimensions up to 11.

Statistical Mechanics · Physics 2009-11-10 I. Lyberg

We present new results for the virial coefficients B_k with k <= 10 for hard spheres in dimensions D=2,...,8.

Statistical Mechanics · Physics 2016-10-06 Nathan Clisby , Barry M. McCoy

We exactly calculate the fourth virial coefficient for hard spheres in even dimensions for D=4,6,8,10, and 12.

Statistical Mechanics · Physics 2016-10-06 N. Clisby , B. M. McCoy

Exact results are given for the fourth virial coefficient of hard spheres in even dimensions up through 12. The fifth and sixth virial coefficients are numerically computed for dimensions 2 through 50 and it is found that the sixth virial…

Statistical Mechanics · Physics 2007-05-23 N. Clisby , B. M. McCoy

Using the first seven known virial coefficients and forcing it to possess two branch-point singularities, a new equation of state for the hard-sphere fluid is proposed. This equation of state predicts accurate values of the higher virial…

Soft Condensed Matter · Physics 2009-06-26 Andrés Santos , Mariano López de Haro

A new closed virial equation of state of hard-sphere fluids is proposed which reproduces the calculated or estimated values of the first sixteen virial coefficients at the same time as giving very good accuracy when compared with computer…

Chemical Physics · Physics 2016-07-14 Jianxiang Tian , Yuanxing Gui , Angel Mulero

We evaluate the virial coefficients B_k for k<=10 for hard spheres in dimensions D=2,...,8. Virial coefficients with k even are found to be negative when D>=5. This provides strong evidence that the leading singularity for the virial series…

Statistical Mechanics · Physics 2016-10-06 N. Clisby , B. M. McCoy

The composition-independent virial coefficients of a $d$-dimensional binary mixture of (additive) hard hyperspheres following from a recent proposal for the equation of state of the mixture [Santos, A., Yuste, S. B., and L\'opez de Haro,…

Statistical Mechanics · Physics 2007-05-23 A. Santos , S. B. Yuste , M. López de Haro

Virial expansion is a traditional approach in statistical mechanics that expresses thermodynamic quantities, such as pressure $p$, as power series of density or chemical potential. Its radius of convergence can serve as a potential…

Statistical Mechanics · Physics 2025-01-28 Kiyoharu Kawana

Recent values for virial coefficients up to B12, when expressed in powers of density relative to maximum close packing,lead to a closed equation-of-state for the equilibrium fluid. The series obtained converges for all densities;it becomes…

Statistical Mechanics · Physics 2008-02-02 Leslie V. Woodcock

The fourth virial coefficient is calculated exactly for a fluid of hard spheres in even dimensions. For this purpose the complete star cluster integral is expressed as the sum of two three-folded integrals only involving spherical angular…

Statistical Mechanics · Physics 2022-05-11 Ignacio Urrutia

We review a virial-type estimate which bounds the strength of interaction for a gas of $N$ hard spheres (billiard balls) dispersing into Euclidean space $\mathbb{R}^d$. This type of estimate has been known for decades in the context of…

Analysis of PDEs · Mathematics 2018-07-10 Ryan Denlinger

The asymptotic expansion method is extended by using currently available accurate values for the first ten virial coefficients for hard sphere fluids. It is then used to yield an equation of state for hard sphere fluids, which accurately…

Chemical Physics · Physics 2019-03-27 Jianxiang Tian , Hua Jiang , Yuanxing Gui , A. Mulero

Although many equations of state of hard-disk fluids have been proposed, none is capable of reproducing the currently calculated or estimated values of the first eighteen virial coefficients at the same time as giving very good accuracy…

Chemical Physics · Physics 2016-06-27 Jianxiang Tian , Yuanxing Gui , A. Mulero

A correlation between maxima in virial coefficients (Bn), and "kissing" numbers for hard hyper-spheres up to dimension D=5, indicates a virial equation and close-packing relationship. Known virial coefficients up to B7, both for hard…

Statistical Mechanics · Physics 2011-05-23 Leslie V. Woodcock

We evidence via a computation in the reciprocal space the asymptotic behaviour of the high order virial coefficients for a hard sphere system. These coefficients, if their order is high enough, are those of a geometric series. We thus are…

Statistical Mechanics · Physics 2015-03-23 Richard Bonneville

Different theoretical approaches for the thermodynamic properties and the equation of state for multicomponent mixtures of nonadditive hard spheres in $d$ dimensions are presented in a unified way. These include the theory by Hamad, our…

Soft Condensed Matter · Physics 2010-05-27 Andrés Santos , Mariano López de Haro , Santos B. Yuste

We compute the fourth virial coefficient of a binary nonadditive hard-sphere mixture over a wide range of deviations from diameter additivity and size ratios. Hinging on this knowledge, we build up a $y$ expansion [B. Barboy and W. N.…

Soft Condensed Matter · Physics 2011-10-25 G. Pellicane , F. Saija , C. Caccamo , P. V. Giaquinta

Here we present new results obtained for the equation of state with induced surface and curvature tensions. The explicit formulas for the first five virial coefficients of system pressure and for the induced surface and curvature tension…

Nuclear Theory · Physics 2020-12-22 Nazar S. Yakovenko , Kyrill A. Bugaev , Larissa V. Bravina , Evgeny E. Zabrodin
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