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We apply techniques of subriemannian geometry on Lie groups to laser-induced population transfer in a three-level quantum system. The aim is to induce transitions by two laser pulses, of arbitrary shape and frequency, minimizing the pulse…

Optimization and Control · Mathematics 2007-05-23 Ugo Boscain , Thomas Chambrion , Jean-Paul Gauthier

We propose a method for achieving highly efficient transfer between the vibrational states in a diatomic molecule. The process is mediated by strong laser pulses and can be understood in terms of light-induced potentials. In addition to…

Quantum Physics · Physics 2009-11-06 M. Rodriguez , K. -A. Suominen , B. M. Garraway

We describe how active feedback routines can be applied at limited repetition rate (5 Hz) to optimize high-power $>10$ TW) laser interactions with clustered gases. Optimization of x-ray production from an argon cluster jet, using a genetic…

Accurate population transfer of uncoupled or weakly coupled spin states is crucial for many quantum information processing tasks. In this paper, we propose a fast and robust scheme for population transfer which combines invariant-based…

Quantum Physics · Physics 2022-06-01 Kangze Li , Guofu Xu

A technique for complete population transfer between the two end states $\ket{1}$ and $\ket{3}$ of a three-state quantum system with a train of $N$ pairs of resonant and coincident pump and Stokes pulses is introduced. A simple analytic…

Quantum Physics · Physics 2015-06-03 Andon A. Rangelov , Nikolay V. Vitanov

In the previous paper on this topic it was shown how, for a pulse of arbitrary shape and duration, the drive frequency can be analytically optimized to maximize the amplitude of the population oscillations between the selected two levels in…

Quantum Physics · Physics 2007-05-23 Duje Bonacci

Laser control of ultrafast double proton transfer is investigated for a two-dimensional model system describing stepwise and concerted transfer pathways. The pulse design has been done by employing optimal control theory in combination with…

Chemical Physics · Physics 2015-05-14 Mahmoud Abdel-Latif , Oliver Kühn

For a two-level system, it is believed that a far-off-resonant driving can not help coherent population transfer between the states. In this work, we propose a scheme to implement the coherent transfer with far-off-resonant driving. The…

Quantum Physics · Physics 2016-09-19 Z. C. Shi , W. Wang , X. X. Yi

We report and propose a simple scheme to achieve efficient and fast coherent population transfer (CPT) by utilizing either a nonlinearly chirped Gaussian shaped few-cycle laser pulse or an unchirped sinc-shaped few-cycle laser pulse. The…

Quantum Physics · Physics 2012-12-20 Parvendra Kumar , Amarendra K. Sarma

A method for solving the problem of efficient population transfer from the ground to some excited state by available technical means (varying resonator length) is proposed. We consider a mixture of similar quantum systems distributed in a…

Quantum Physics · Physics 2023-12-04 K. A. Lyakhov , A. N. Pechen

We propose a method to transfer the population and control the state of two-level and three-level atoms speeding-up Adiabatic Passage techniques while keeping their robustness versus parameter variations. The method is based on…

Quantum Physics · Physics 2010-09-20 Xi Chen , I. Lizuain , A. Ruschhaupt , D. Guery-Odelin , J. G. Muga

We present a fast phase gate scheme that is experimentally achievable and has an operation time more than two orders of magnitude faster than current experimental schemes for low numbers of pulses. The gate time improves with the number of…

Quantum Physics · Physics 2013-04-10 C. D. B. Bentley , A. R. R. Carvalho , D. Kielpinski , J. J. Hope

We demonstrate a method of adiabatic population transfer from a single quantum state into a coherent superposition of states. The transfer is executed with femtosecond pulses, spectrally shaped in simple and intuitive manner, which does not…

Quantum Physics · Physics 2015-05-14 S. Zhdanovich , E. A. Shapiro , J. W. Hepburn , M. Shapiro , V. Milner

The influence of photon-momentum recoil on adiabatic population transfer in an atomic three-level lambda system is studied. It is shown that the Doppler frequency shifts, due to atomic motion can play an important role in adiabatic…

Quantum Physics · Physics 2016-11-03 R. G. Unanyan

We report and propose a simple scheme to achieve the ultrafast and selective population transfer in four-level atoms by utilizing a single frequency chirped few-cycle pulse. It is demonstrated that the almost complete population may be…

Quantum Physics · Physics 2015-06-15 Parvendra Kumar , Amarendra K. Sarma

The optimal control of population transfer for multi-level systems is investigated from the perspective of quantum geometry. Firstly, the general theoretical framework of optimizing the stimulated Raman adiabatic passage (STIRAP) scheme…

Quantum Physics · Physics 2025-12-24 Guan-Qiang Li , Yu-Qi Zhang , Hao Guo , You-Jiao Dong , Zhi-Yu Lin , Ping Peng

This paper describes the first experimental demonstration of the guiding of a relativistic electron beam in a solid target using two co-linear, relativistically intense, picosecond laser pulses. The first pulse creates a magnetic field…

Ultrafast lasers ($< 500$ fs) have enabled laser-matter interactions at intensities exceeding $10^{18} \rm{Wcm}^{-2}$ with only millijoules of laser energy. However, as pulse durations become shorter, larger spectral bandwidths are…

The generation of ultrashort pulses hinges on the careful management of dispersion. Traditionally, this has exclusively involved second-order dispersion, while higher-order dispersion was treated as a nuisance to be minimized. Here we show…

We examine the stability of population transfer in two- and three-level systems against unwanted additional transitions. This population inversion is achieved by using recently proposed schemes called "shortcuts to adiabaticity". We…

Quantum Physics · Physics 2017-03-14 Anthony Kiely , Andreas Ruschhaupt