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We describe a method to probe the spectral fluctuations of a transition over broad ranges of frequencies and timescales with the high spectral resolution of Fourier spectroscopy, and a temporal resolution as high as the excited state…

We present a simple method to extract the homogeneous linewidth of a single photon emitter line exhibiting fast (down to 1 ns) spectral diffusion (SD). It is based on a recently developed technique using photon correlation measurements on…

Mesoscale and Nanoscale Physics · Physics 2012-09-07 S. Bounouar , A. Trichet , M. Elouneg-Jamroz , R. André , E. Bellet-Amalric , C. Bougerol , M. Den Hertog , K. Kheng , S. Tatarenko , J. -Ph. Poizat

Hyperspectral imaging aims at providing information on both the spatial and the spectral distribution of light, with high resolution. However, state-of-the-art protocols are characterized by an intrinsic trade-off imposing to sacrifice…

Optics · Physics 2024-07-22 Gianlorenzo Massaro , Francesco V. Pepe , Milena D'Angelo

The inherent non-linearity of intensity correlation functions can be used to spatially distinguish identical emitters beyond the diffraction limit, as achieved, for example, in Super-Resolution Optical Fluctuation Imaging (SOFI). Here, we…

Optics · Physics 2024-12-18 Yifan Chen , Chieh Tsao , Hendrik Utzat

High peak power ultrafast lasers are widely used in nonlinear spectroscopy but often limit its spectral resolution because of the broad frequency bandwidth of ultrashort laser pulses. Improving the resolution by achieving spectrally narrow…

Optics · Physics 2009-11-13 Stanislav O. Konorov , Xiaoji G. Xu , John W. Hepburn , Valery Milner

Natural laser emission may be produced whenever suitable atomic energy levels become overpopulated. Strong evidence for laser emission exists in astronomical sources such as Eta Carinae, and other luminous stars. However, the evidence is…

Astrophysics · Physics 2009-06-23 Dainis Dravins , Claudio Germana

Optical scattering presents a major obstacle to high resolution imaging in biological tissue and other turbid media. Conventional photoacoustic imaging can partially overcome this obstacle, enabling imaging of optical absorption in the…

Frequency-filtered photon correlations have been proven to be extremely useful in grasping how the detection process alters photon statistics. Harnessing the spectral correlations also permits refinement of the emission and unraveling of…

An absolute measurement of the components of the shear rate tensor $\mathcal{S}$ in a fluid can be found by measuring the photon correlation function of light scattered from particles in the fluid. Previous methods of measuring…

Soft Condensed Matter · Physics 2015-10-28 Elliot Jenner , Brian D'Urso

We investigate the possibility of measuring the homogeneous and inhomogeneous contribution to the linewidth of a spectrally diffusing single photon emitter using a simple photon correlation spectroscopy method (PCS). The photon energy…

Mesoscale and Nanoscale Physics · Physics 2012-01-20 Aurelien Trichet , Samir Bounouar

Diffusion coefficient measurements are important for many biological and material investigations, such as particle dynamics, kinetics, and size determinations. Amongst current measurement methods, single particle tracking (SPT) offers the…

Biomolecules · Quantitative Biology 2011-07-12 Shannon Kian Zareh , Michael C. DeSantis , Jonathan Kessler , Je-Luen Li , Y. M. Wang

Photon correlation spectroscopy (PCS) is based on measuring the temporal correlation of the light intensity scattered by the investigated sample. A typical setup requires a temporally coherent light source. Here, we show that a…

Optics · Physics 2015-05-30 D. Salerno , D. Brogioli , F. Croccolo , R. Ziano , F. Mantegazza

Neutron correlation spectroscopy can exceed direct spectroscopy in the incoming beam intensity by up to two orders of magnitude at the same energy resolution. However, the propagation of the counting noise in the correlation algorithm of…

Instrumentation and Detectors · Physics 2016-09-13 F. Mezei , M. T. Caccamo , F. Migliardo , S. Magazù

By utilizing the frequency anticorrelation of two-photon states produced via spontaneous parametric down conversion (SPDC), the working principle of a novel remote spectrometer is demonstrated. With the help of a local scanning…

Quantum Physics · Physics 2016-09-08 Giuliano Scarcelli , Alejandra Valencia , Samuel Gompers , Yanhua Shih

Spectroscopy is a well-established nonintrusive tool that has played an important role in identifying substances and quantifying their compositions, from quantum descriptions to chemical and biomedical diagnostics. Challenges exist in…

Atmospheric and Oceanic Physics · Physics 2020-12-02 S. Yu , Z. Zhang , H. Xia , X. Dou , M. Li , T. Wei , L. Wang , P. Jiang , Y. Wu , C. Zhang , L. You , Y. Hu , T. Wu , L. Zhao , M. Shangguan , L. Tao , J. Qiu

Fluorescence imaging is an essential diagnostic tool in many fields, but diffraction-limited optical imaging at depth is limited by scattering. Here, we present a method based on multiple random illuminations, combined with a computational…

Optics · Physics 2026-03-30 Lei Zhu , Tengfei Wu , Bernhard Rauer , Hilton B. de Aguiar , Sylvain Gigan

We present angular-resolved correlation measurements between photons after propagation through a three-dimensional disordered medium. The multiple scattering process induces photon correlations that are directly measured for light sources…

Optics · Physics 2011-06-30 Stephan Smolka , Otto L. Muskens , Ad Lagendijk , Peter Lodahl

A two level model of a single molecule undergoing spectral diffusion dynamics and interacting with a sequence of two short laser pulses is investigated. Analytical solution for the probability of n=0,1,2 photon emission events for the…

Chemical Physics · Physics 2009-11-13 F. Shikerman , E. Barkai

Linear (spectro) polarimetry is usually performed using separate photon flux measurements after spatial or temporal polarization modulation. Such classical polarimeters are limited in sensitivity and accuracy by systematic effects and…

Optics · Physics 2010-05-28 Frans Snik , Theodora Karalidi , Christoph U. Keller

In this paper, we have established the couple system of a spectroscope, CCD and computer and proposed a method of the rapid measurement on spectral characteristics such as central wavelengths, relative intensities, sensitivity lines and the…

Instrumentation and Detectors · Physics 2015-12-03 Chol-Sun Kim , Chol-Su Kim , Song-Jin Im
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