English
Related papers

Related papers: Significant Conditions on the Two-electron Reduced…

200 papers

We review and supplement the recent result by the authors on the reduction of the three dimensional $R$ (3d $R$) satisfying the tetrahedron equation to the quantum $R$ matrices for the $q$-oscillator representations of $U_q(D^{(2)}_{n+1})$,…

Mathematical Physics · Physics 2017-02-01 Atsuo Kuniba , Masato Okado

Correlation-driven phenomena in molecular periodic systems are challenging to predict computationally not only because such systems are periodically infinite but also because they are typically strongly correlated. Here we generalize the…

Chemical Physics · Physics 2022-04-18 Simon Ewing , David A. Mazziotti

Recent advances in quantum crystallography have shown that, beyond conventional charge density refinement, a one-electron reduced density matrix (1-RDM) satisfying N-representability conditions can be reconstructed using jointly…

Quantum Physics · Physics 2024-03-04 Sizhuo Yu , Jean-Michel Gillet

Quantum state tomography is a fundamental task in quantum information science, enabling detailed characterization of correlations, entanglement, and electronic structure in quantum systems. However, its exponential measurement and…

The variational determination of the two-particle density matrix is an interesting, but not yet fully explored technique that allows to obtain ground-state properties of a quantum many-body system without reference to an $N$-particle wave…

Strongly Correlated Electrons · Physics 2012-05-22 Brecht Verstichel , Helen van Aggelen , Ward Poelmans , Dimitri Van Neck

A reduced-density-matrix (RDM)-based approach to {\em ab initio} cavity quantum electrodynamics (QED) is developed. The expectation value of the Pauli-Fierz Hamiltonian is expressed in terms of one- and two-body electronic and photonic…

Chemical Physics · Physics 2022-11-23 Joel D. Mallory , A. Eugene DePrince

The accurate description of the non-linear response of many-electron systems to strong-laser fields remains a major challenge. Methods that bypass the unfavorable exponential scaling with particle number are required to address larger…

Fermionic reduced density matrices summarize the key observables in fermionic systems. In electronic systems, the two-particle reduced density matrix (2-RDM) is sufficient to determine the energy and most physical observables of interest.…

Quantum Physics · Physics 2023-06-12 Linqing Peng , Xing Zhang , Garnet Kin-Lic Chan

The simulation of strongly correlated many-electron systems is one of the most promising applications for near-term quantum devices. Here we use a class of eigenvalue solvers (presented in Phys. Rev. Lett. 126, 070504 (2021)) in which a…

Quantum Physics · Physics 2022-04-18 Scott E. Smart , Jan-Niklas Boyn , David A. Mazziotti

In the search for accurate approximate solutions of the many-body Schr\"odinger equation, reduced density matrices play an important role, as they allow to formulate approximate methods with polynomial scaling in the number of particles.…

Quantum Physics · Physics 2024-12-19 Elias Pescoller , Marie Eder , Iva Březinová

An active space variational calculation of the 2-electron reduced density matrix (2-RDM) is derived and implemented where the active orbitals are correlated within the pair approximation. The pair approximation considers only doubly…

Chemical Physics · Physics 2020-10-13 Kade Head-Marsden , David A. Mazziotti

Two Higgs doublet models (2HDM) provide the low energy effective field theory (EFT) description in many well motivated extensions of the Standard Model. It is therefore relevant to study their properties, as well as the theoretical…

High Energy Physics - Phenomenology · Physics 2023-05-03 Henning Bahl , Marcela Carena , Nina M. Coyle , Aurora Ireland , Carlos E. M. Wagner

It is a hard and important problem to find the criterion of the set of positive-definite matrixes which can be written as reduced density operators of a multi-partite quantum state. This problem is closely related to the study of many-body…

Quantum Physics · Physics 2009-11-10 Yong-Jian Han , Yong-Sheng Zhang , Guang-Can Guo

Folding grid value vectors of size $2^L$ into $L$th order tensors of mode sizes $2\times \cdots\times 2$, combined with low-rank representation in the tensor train format, has been shown to lead to highly efficient approximations for…

Numerical Analysis · Mathematics 2019-11-19 Markus Bachmayr , Vladimir Kazeev

The N-representability problem for reduced density matrices remains a fundamental challenge in electronic structure theory. Following our previous work that employs a unitary-evolution algorithm based on an adaptive derivative-assembled…

The one-particle reduced density-matrix (1-RDM) functional theory is a promising alternative to density-functional theory (DFT) that uses the 1-RDM rather than the electronic density as a basic variable. However, long-standing challenges…

Quantum Physics · Physics 2024-08-20 Matthieu Vladaj , Quentin Marécat , Bruno Senjean , Matthieu Saubanère

We develop tractable convex relaxations for rank-constrained quadratic optimization problems over $n \times m$ matrices, a setting for which tractable relaxations are typically only available when the objective or constraints admit spectral…

Optimization and Control · Mathematics 2026-05-22 Ryan Cory-Wright , Jean Pauphilet

We examine the binding conditions for atoms in non-relativistic QED, and prove that removing one electron from an atom requires a positive energy. As an application, we establish the existence of a ground state for the Helium atom.

Mathematical Physics · Physics 2015-06-26 Jean-Marie Barbaroux , Thomas Chen , Semjon Vugalter

We derive and analyze a hierarchy of approximations to the strongly correlated limit of the Hohenberg-Kohn functional. These "density representability approximations" are obtained by first noting that in the strongly correlated limit,…

Chemical Physics · Physics 2013-10-25 Gero Friesecke , Christian B. Mendl , Brendan Pass , Codina Cotar , Claudia Klüppelberg

As a universal quantum mechanical approach to the dynamical many-body problem, the time-dependent density functional theory (TDDFT) might be inadequate to describe crucial observables that rely on two-body evolution behavior, like the…

Computational Physics · Physics 2025-11-17 Jiong-Hang Liang , Yunfeng Xiong