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Interference between magnetic substates of the hyperfine structure states belonging to different fine structure states of the same term influences the polarization for some of the diagnostically important lines of the Sun's spectrum, like…

Solar and Stellar Astrophysics · Physics 2015-12-25 K. Sowmya , K. N. Nagendra , M. Sampoorna , J. O. Stenflo

We investigate molecular dynamics of multiple ionization in N2 through multiple core-level photoabsorption and subsequent Auger decay processes induced by intense, short X-ray free electron laser pulses. The timing dynamics of the…

The uncorrelated (``sequential'') and correlated (``nonsequential'') double ionization of the H2 molecule in strong laser pulses is investigated using the tools of nonlinear dynamics. We focus on the phase-space dynamics of this system,…

Chaotic Dynamics · Physics 2009-11-30 François Mauger , Cristel Chandre , T. Uzer

We report on the fragmentation of the water molecule by $1$ MeV H$^{+}$, He$^{+}$ and 650 keV N$^{+}$ ion impact. The fragment-ion energy spectra were measured by an electrostatic spectrometer at different observation angles. The obtained…

Atomic Physics · Physics 2017-09-13 S. T. S. Kovács , P. Herczku , Z. Juhász , L. Sarkadi , L. Gulyás , B. Sulik

We investigate dissociative single and double ionization of HeH+ induced by intense femtosecond laser pulses. By employing a semi-classical model with nuclear trajectories moving on field-dressed surfaces and ionization events treated as…

Atomic Physics · Physics 2018-10-24 Lun Yue , Philipp Wustelt , A. Max Sayler , Gerhard G. Paulus , Stefanie Gräfe

We report the observation of above-threshold dissociation of a multielectron molecular system, Na$_2^+$. The process is due to continuum-continuum transitions in a field-dressed molecular continuum. Three well resolved fragmentation…

Chemical Physics · Physics 2008-08-24 Qun Zhang , John W. Hepburn , Moshe Shapiro

A review of some recently developed methods of calculating multiple differential cross-sections of photoionization and electron impactionization of atoms and molecules having two active electrons is presented. The methods imply original…

Fragmentation of highly charged molecular ions or clusters consisting of more than two atoms can proceed in an onestep synchronous manner where all bonds break simultaneously or sequentially by emitting one ion after the other. We separated…

Joint electron-ion energy spectra for the dissociative ionization of a model H$_2^+$ in few-cycle, infrared laser pulses are calculated via the numerical ab initio solution of the time-dependent Schr\"odinger equation. A strong,…

Atomic Physics · Physics 2017-11-21 V. Mosert , D. Bauer

The toolbox for imaging molecules is well-equipped today. Some techniques visualize the geometrical structure, others the electron density or electron orbitals. Molecules are many-body systems for which the correlation between the…

We investigate the role of nuclear motion and strong-field-induced electronic couplings during the double ionization of deuterated water using momentum-resolved coincidence spectroscopy. By examining the three-body dicationic dissociation…

We present the first theoretical treatment of the formation of highly excited neutral H atoms (H$^{*}$) for strongly driven H$_{2}$. This process, with one electron ionizing and one captured in a Rydberg state, was recently reported in an…

Atomic Physics · Physics 2015-05-28 A. Emmanouilidou , D. Tchitchekova , C. Lazarou , U. Eichmann

We develop a time-dependent theory to investigate electron dynamics and photoionization processes of diatomic molecules interacting with strong laser fields including electron-electron correlation effects. We combine the recently formulated…

Chemical Physics · Physics 2016-02-02 Henrik R. Larsson , Sebastian Bauch , Lasse Kragh Sørensen , Michael Bonitz

Strong-field photoelectron momentum imaging of the prototypical biomolecule indole was disentangled in a combined experimental and computational approach. Experimentally, strong control over the molecules enabled the acquisition of…

Atomic Physics · Physics 2021-02-03 Joss Wiese , Jolijn Onvlee , Sebastian Trippel , Jochen Küpper

The full-dimensional time-dependent Schrodinger equation for the electronic dynamics of single-electron systems in intense external fields is solved directly using a discrete method. Our approach combines the finite-difference and Lagrange…

Atomic Physics · Physics 2009-11-10 Liang-You Peng , J F McCann , Daniel Dundas , K T Taylor , I D Williams

We present a very efficient technique for solving the three-dimensional time-dependent Schrodinger equation. Our method is applicable to a wide range of problems where a fullly three-dimensional solution is required, i.e., to cases where no…

Atomic Physics · Physics 2009-11-13 T. K. Kjeldsen , L. A. A. Nikolopoulos , L. B. Madsen

The development of intense high-energy radiation sources and the improvement of techniques for detecting charged fragments have made possible experiments on multiple ionization of a molecule with registration of the momentum and charge of…

We present a semiclassical two-step model for strong-field ionization that accounts for path interferences of tunnel-ionized electrons in the ionic potential beyond perturbation theory. Within the framework of a classical trajectory…

A clear understanding of the mechanisms that control the electron dynamics in strong laser field is still a challenge that requires to be interpreted by advanced theory. Development of accurate theoretical and computational methods, able to…

We review the main aspects of multiple photoionization processes in atoms exposed to intense, short wavelength radiation. The main focus is the theoretical framework for the description of such processes as well as the conditions under…

Atomic Physics · Physics 2014-01-21 P. Lambropoulos , G. M. Nikolopoulos