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We investigate the ion distribution and overcharging at charged interfaces with dielectric inhomogeneities in the presence of asymmetric electrolytes containing polyvalent and monovalent ions. We formulate an effective "dressed counterion"…

Soft Condensed Matter · Physics 2015-03-17 Matej Kanduc , Ali Naji , Jan Forsman , Rudolf Podgornik

We study the effective interaction between differently charged polyelectrolyte-colloid complexes in electrolyte solutions via Monte Carlo simulations. These complexes are formed when short and flexible polyelectrolyte chains adsorb onto…

Soft Condensed Matter · Physics 2010-05-05 D. Truzzolillo , F. Bordi , F. Sciortino , S. Sennato

We analytically calculate the correlation potential of a test ion near a \emph{strongly} charged plate inside a dilute $m:-n$ electrolyte. We do this by calculating the electrostatic Green's function in the presence of a nonlinear…

Soft Condensed Matter · Physics 2014-03-19 Bing-Sui Lu , Xiangjun Xing

Poisson-Boltzmann theory is the cornerstone for soft matter electrostatics. We provide novel exact analytical solutions to this non-linear mean-field approach, for the diffuse layer of ions in the vicinity of a planar or a cylindrical…

Soft Condensed Matter · Physics 2020-01-29 L. Samaj , E. Trizac

In the present work, we have extended a weak coupling theory [A. Bakhshandeh, A. P. dos Santos and Y. Levin Phys. Rev. Lett 107, 107801 (2011)] for systems with added 1:1 electrolyte. To study the accuracy of the developed theory, we…

Soft Condensed Matter · Physics 2020-08-18 Amin Bakhshandeh

The hypernetted chain/mean spherical approximation (HNC/MSA) integral equation is obtained and solved numerically for a totally asymmetric primitive model electrolyte around a spherical macroparticle. The ensuing radial distribution…

Debye-Huckel (DH) theory is extended to treat two-component size- and charge-asymmetric primitive models, focussing primarily on the 1:1 additive hard-sphere electrolyte with, say, negative ion diameters, a--, larger than the positive ion…

Statistical Mechanics · Physics 2009-11-07 Daniel M. Zuckerman , Michael E. Fisher , Stefan Bekiranov

The ionic adsorption around a weakly charged spherical colloid, immersed in size-asymmetric 1:1 and 2:2 salts, is studied. We use the primitive model of an electrolyte to perform Monte Carlo simulations as well as theoretical calculations…

Soft Condensed Matter · Physics 2008-03-29 G. I. Guerrero-García , E. González-Tovar , M. Chávez-Páez , Marcelo Lozada-Cassou

Correlation functions in concentrated ionic systems are studied within the mesoscopic theory at the level of the Gaussian approximation. The previously neglected fluctuation contribution to the inverse charge-charge correlation function is…

Soft Condensed Matter · Physics 2025-06-26 O. Patsahan , A. Ciach

We study the surface tension of ionic solutions at air/water and oil/water interfaces. By using field-theoretical methods and including a finite proximal surface-region with ionic-specific interactions. The free energy is expanded to…

Soft Condensed Matter · Physics 2015-03-31 Tomer Markovich , David Andelman , Rudolf Podgornik

Water-in-Salt-Electrolytes (WiSEs) are a promising class of next-generation electrolytes. Unlike classical dilute electrolytes or more conventional battery electrolytes, WiSEs are characterised by their super-concentrated salt concentration…

The electroviscous effects in the pressure-driven flow of electrolyte liquid through an asymmetrically charged contraction-expansion (4:1:4) slit microfluidic device have been investigated numerically. The mathematical model (i.e.,…

Fluid Dynamics · Physics 2023-11-23 Jitendra Dhakar , Ram Prakash Bharti

We derive a Debye-H\"uckel-like model of the electric ion-ion interaction for non-constant dielectric susceptibility, which does not depend on any kind of charging process due to its foundation in the general framework of non-equilibrium…

Chemical Physics · Physics 2025-02-24 Wolfgang Dreyer , Rüdiger Müller

Employing recent advances in response theory and nonequilibrium ensemble reweighting, we study the dynamic and static correlations that give rise to an electric field-dependent ionic conductivity in electrolyte solutions. We consider…

Soft Condensed Matter · Physics 2021-07-28 Dominika Lesnicki , Chloe Y. Gao , David T. Limmer , Benjamin Rotenberg

In this work, the pressure-driven flow of symmetric electrolyte liquid through a heterogeneously charged contraction-expansion (4:1:4) microfluidic device has been investigated numerically. Total potential ($U$), ion concentrations…

Fluid Dynamics · Physics 2023-12-27 Jitendra Dhakar , Ram Prakash Bharti

We study the role of ionic correlations on the electroosmotic flow in planar double-slit channels, without salt. We propose an analytical theory, based on recent advances in the understanding of correlated systems. We compare the theory…

Soft Condensed Matter · Physics 2021-02-04 Ivan Palaia , Igor M. Telles , Alexandre P. dos Santos , Emmanuel Trizac

Salt transport in bulk electrolytes is limited by diffusion and convection, but in microstructures with charged surfaces (e.g. microfluidic devices, porous media, soils, or biological tissues) surface conduction and electro-osmotic flow…

Fluid Dynamics · Physics 2015-05-30 Ali Mani , Martin Z. Bazant

This paper builds on two previous works, Lindgren et al. J. Comp. Phys. 371, 712-731 (2018) and Quan et al. arXiv:1807.05384 (2018), to devise a new method to solve the problem of calculating electrostatic interactions in a system composed…

Soft Condensed Matter · Physics 2019-02-20 Eric B. Lindgren , Chaoyu Quan , Benjamin Stamm

Solvation effect might have a tremendous influence on chemical reactions. However, precise quantum chemistry calculations are most often done either in vacuum neglecting the role of the solvent or using continuum solvent model ignoring its…

Chemical Physics · Physics 2020-07-14 Guillaume Jeanmairet , Maximilien Levesque , Daniel Borgis

In this paper, we theoretically study the electrostatic interaction between a pair of identical colloids with constant surface potentials sitting in close vicinity of each other at a fluid interface. By employing a simplified yet reasonable…

Soft Condensed Matter · Physics 2020-07-29 Rick Bebon , Arghya Majee
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