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In monolayer MoS2 optical transitions across the direct bandgap are governed by chiral selection rules, allowing optical valley initialization. In time resolved photoluminescence (PL) experiments we find that both the polarization and…

Mesoscale and Nanoscale Physics · Physics 2014-02-04 D. Lagarde , L. Bouet , X. Marie , C. R. Zhu , B. L. Liu , T. Amand , P. H. Tan , B. Urbaszek

Modern electronic devices heavily rely on the accurate control of charge and spin of electrons. The emergence of controllable valley degree of freedom brings new possibilities and presents a promising prospect towards valleytronics.…

We report experimental evidences on selective occupation of the degenerate valleys in MoS2 monolayers by circularly polarized optical pumping. Over 30% valley polarization has been observed at K and K' valley via the polarization resolved…

Mesoscale and Nanoscale Physics · Physics 2013-04-17 Hualing Zeng , Junfeng Dai , Wang Yao , Di Xiao , Xiaodong Cui

In this letter we present photoluminescence measurements with different excitation energies on single-layer MoS$_2$ and MoSe$_2$ in order to examine the resonance behavior of the conservation of circular polarization in these transition…

Applied Physics · Physics 2018-11-06 Hans Tornatzky , Anne-Marie Kaulitz , Janina Maultzsch

We have investigated the steady-sate valley polarization and valley coherence of encapsulated MoS2 monolayer as a function of the temperature and the power density with a continuous wave laser excitation. Both valley polarization and…

Materials Science · Physics 2021-11-01 Fabian Cadiz , Stefan Gerl , Takashi Taniguchi , Kenji Watanabe

A monolayer of $MoS_{2}$ has a non-centrosymmetric crystal structure, with spin polarized bands. It is a two valley semiconductor with direct gap falling in the visible range of the electromagnetic spectrum. Its optical properties are of…

Mesoscale and Nanoscale Physics · Physics 2023-06-09 Zhou Li , J. P. Carbotte

We investigate with polarized microphotoluminescence the optical pumping of the valley degree of freedom in charge-tunable MoS2 monolayers encapsulated with hexagonal boron nitride at cryogenic temperatures. We report a large steady state…

Mesoscale and Nanoscale Physics · Physics 2021-10-15 Sangjun Park , Steve Arscott , Takashi Taniguchi , Kenji Watanabe , Fausto Sirotti , Fabian Cadiz

We investigate valley exciton dynamics in MoSe2 monolayers in polarization- and time-resolved photoluminescence (PL) spectroscopy at 4K. Following circularly polarized laser excitation, we record a low circular polarization degree of the PL…

Materials Science · Physics 2015-03-19 G. Wang , E. Palleau , T. Amand , S. Tongay , X. Marie , B. Urbaszek

A photoinduced current of a layered MoS2-based transistor is studied from first-principles. Under the illumination of circular polarized light, a valley-polarized current is generated, which can be tuned by the gate voltage. For monolayer…

Mesoscale and Nanoscale Physics · Physics 2017-01-09 Yunjin Yu , Yanfeng Zhou , Langhui Wan , Bin Wang , Fuming Xu , Yadong Wei , Jian Wang

Interlayer valley excitons in bilayer MoS2 feature concurrently large oscillator strength and long lifetime, and hence represent an advantageous scenario for valleytronic applications. However, control of valley pseudospin of interlayer…

Electronic and spintronic devices rely on the fact that free charge carriers in solids carry electric charge and spin, respectively. There are, however, other properties of charge carriers that might be exploited in new families of devices.…

Mesoscale and Nanoscale Physics · Physics 2015-06-05 Kin Fai Mak , Keliang He , Jie Shan , Tony F. Heinz

Optical interband transitions in monolayer transition metal dichalcogenides such as WSe2 and MoS2 are governed by chiral selection rules. This allows efficient optical initialization of an electron in a specific K-valley in momentum space.…

Mesoscale and Nanoscale Physics · Physics 2014-09-09 G. Wang , L. Bouet , D. Lagarde , M. Vidal , A. Balocchi , T. Amand , X. Marie , B. Urbaszek

We report on controlling the spontaneous emission (SE) rate of a molybdenum disulfide (MoS$_2$) monolayer coupled with a planar photonic crystal (PPC) nanocavity. Spatially resolved photoluminescence (PL) mapping shows strong variations of…

We report experimental observation of 2s exciton radiative emission from monolayer tungsten diselenide, enabled by hexagonal boron nitride protected high-quality samples. The 2s luminescence is highly robust and persists up to 150K,…

Mesoscale and Nanoscale Physics · Physics 2018-01-31 Shao-Yu Chen , Thomas Goldstein , Jiayue Tong , Takashi Taniguchi , Kenji Watanabe , Jun Yan

We show room temperature valley coherence with in MoS2, MoSe2, WS2 and WSe2 monolayers using linear polarization resolved hot photoluminescence (PL), at energies close to the excitation - demonstrating preservation of valley coherence…

Mesoscale and Nanoscale Physics · Physics 2016-05-24 Sangeeth Kallatt , Govindarao Umesh , Kausik Majumdar

We investigate the valley related carrier dynamics in monolayer MoS2 using helicity resolved non-degenerate ultrafast pump-probe spectroscopy at the vicinity of the high-symmetry K point under the temperature down to 78 K. Monolayer MoS2…

Optics · Physics 2014-05-08 Qinsheng Wang , Shaofeng Ge , Xiao Li , Jun Qiu , Yanxin Ji , Ji Feng , Dong Sun

Monolayers of transition metal dichalcogenides (TMDCs) are atomically thin direct-gap semiconductors with potential applications in nanoelectronics, optoelectronics, and electrochemical sensing. Recent theoretical and experimental efforts…

Mesoscale and Nanoscale Physics · Physics 2013-02-26 Sanfeng Wu , Chunming Huang , Grant Aivazian , Jason S Ross , David H Cobden , Xiaodong Xu

In this letter, we address the chiral properties of valley exciton-polaritons in a monolayer of WS2 in the regime of strong light-matter coupling with a Tamm-Plasmon resonance. We observe that the valley polarization, which manifests in the…

Mesoscale and Nanoscale Physics · Physics 2017-12-13 N. Lundt , S. Stoll , P. Nagler , A. Nalitov , S. Klembt , S. Betzold , J. W. Goddard , E. Frieling , A. V. Kavokin , C. Schüller , T. Korn , S. Höfling , C. Schneider

Time reversal dictates that nonmagnetic, centrosymmetric crystals cannot be spin-polarized as a whole. However, it has been recently shown that the electronic structure in these crystals can in fact show regions of high spin-polarization,…

We calculate linear and nonlinear optical susceptibilities arising from the excitonic states of mono- layer MoS2 for in-plane light polarizations, using second-quantized bound and unbound exciton operators. Optical selection rules are…

Mesoscale and Nanoscale Physics · Physics 2018-04-11 Daniel B. S. Soh , Christopher Rogers , Dodd J. Gray , Eric Chatterjee , Hideo Mabuchi
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