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We explore the electronic structure of ultralong-range pentaatomic Rydberg molecules from a merger of a Rydberg atom and two ground state heteronuclear diatomic molecules. Our focus is on the interaction of Rb($23s$) and Rb($n=20$, $l\ge…

Most experiments with ultracold atoms in optical lattices have contact interactions, and therefore operate at high densities of around one atom per site to observe the effect of strong interactions. Strong ranged interactions can be…

Quantum Physics · Physics 2023-06-06 Daniel Malz , J. Ignacio Cirac

Cold Rydberg atoms, known for their long lifetimes and strong dipole-dipole interactions that lead to the Rydberg blockade phenomenon, are among the most promising platforms for quantum simulations, quantum computation and quantum networks.…

We address the technical challenges when performing quantum information experiments with ultracold Rydberg atoms in lattice geometries. We discuss the following key aspects: (i) The coherent manipulation of atomic ground states, (ii) the…

Atomic Physics · Physics 2017-01-04 J. B. Naber , J. Vos , R. J. Rengelink , R. J. Nusselder , D. Davtyan

We report on the study of state-changing collisions between Rydberg atoms and ground state atoms. We employ high-resolution momentum spectroscopy to identify the final states. In contrast to previous studies, we find that the outcome of…

Atomic Physics · Physics 2021-07-14 Philipp Geppert , Max Althön , Daniel Fichtner , Herwig Ott

Rydberg-mediated quantum optics is a useful route toward deterministic quantum information processing based on single photons and quantum networks, but is bottlenecked by the fast motional dephasing of Rydberg atoms. Here, we propose and…

In this work we discuss the rotational structure of Rydberg molecules. We calculate the complete wave function in a laboratory fixed frame and derive the transition matrix elements for the pho- toassociation of free ground state atoms. We…

Atomic Physics · Physics 2018-08-01 O. Thomas , C. Lippe , T. Eichert , H. Ott

Ultrafast electron diffraction and time-resolved serial crystallography are the basis of the ongoing revolution in capturing at the atomic level of detail the structural dynamics of molecules. However, most experiments employ the classical…

A quantum-feedback-based scheme is proposed for generating multipartite entanglements of Rydberg atoms in a dissipative optical cavity. The Rydberg blockade mechanism efficiently prevents double excitations of the system, which is further…

Quantum Physics · Physics 2017-02-15 X. Q. Shao , J. H. WU , X. X. Yi

The interaction between atoms and a quantized radiation field is fundamentally important in quantum optics and quantum information science. Due to their unusual properties, Rydberg atoms are promising building blocks for two-qubit gates and…

Quantum Physics · Physics 2026-01-06 Francisco D. Santillan , Andreas Hanke

We analyze in detail the possibility to use charge-dipole interaction between a single polar molecule or a 1D molecular array and a single Rydberg atom to read out rotational populations. The change in the Rydberg electron energy is…

Quantum Physics · Physics 2016-10-05 Elena Kuznetsova , Seth T. Rittenhouse , H. R. Sadeghpour , Susanne F. Yelin

Synthetic dimension platforms offer unique pathways for engineering quantum matter. We compute the phase diagram of a many-body system of ultracold atoms (or polar molecules) with a set of Rydberg states (or rotational states) as a…

Rydberg blockade of ultracold atoms is considered now as one of the most promising tools for the implementation of quantum computing, but its fidelity can be substantially compromised by detrimental excitation of the neighbouring atoms.…

Atomic Physics · Physics 2017-05-05 Yurii V. Dumin

We study resonant optical excitations of strongly-interacting Rydberg states of atoms in the presence of relaxations. We employ the quantum stochastic (Monte Carlo) wavefunctions to simulate the dissipative dynamics of tens of atoms in…

Quantum Physics · Physics 2013-06-25 David Petrosyan

Quantum gates and entanglement based on dipole-dipole interactions of neutral Rydberg atoms are relevant to both fundamental physics and quantum information science. The precision and robustness of the Rydberg-mediated entanglement…

Quantum Physics · Physics 2022-12-14 Xiao-Feng Shi

This paper is a proposal for the generation of many-body entangled state in atomic and mechanical systems. Application of strong Rydberg dressing interaction and fast bifurcation scheme in an ultra-stable Cs lattice clock in this proposal…

Quantum Physics · Physics 2018-10-24 Mohammadsadegh Khazali

The yield of neutral excited atoms and low-energy photoelectrons generated by the electron dynamics in the combined Coulomb and laser field after tunneling is investigated. We present results of Monte-Carlo simulations built on the two-step…

Atomic Physics · Physics 2015-05-13 N. I. Shvetsov-Shilovski , S. P. Goreslavski , S. V. Popruzhenko , W. Becker

We introduce a computational method developed for study of long-range molecular Rydberg states of such systems that can be approximated by two electrons in a model potential of the atomic cores. Only diatomic molecules are considered. The…

Chemical Physics · Physics 2016-01-26 Michal Tarana , Roman Čurík

We present an efficient method for producing $N$ particle entangled states using Rydberg blockade interactions. Optical excitation of Rydberg states that interact weakly, yet have a strong coupling to a second control state is used to…

Quantum Physics · Physics 2010-11-01 M. Saffman , K. Molmer

We describe a quantum information architecture consisting of a hybrid array of optically-trapped molecules and atoms. This design leverages the large transition dipole moments of Rydberg atoms to mediate fast, high-fidelity gates between…

Atomic Physics · Physics 2023-01-13 Kenneth Wang , Conner P. Williams , Lewis R. B. Picard , Norman Y. Yao , Kang-Kuen Ni