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We report a single crystal neutron and x-ray diffraction study of the hybrid improper multiferroic Ca3Mn1.9Ti0.1O7 (CMTO), a prototypical system where the electric polarization arises from the condensation of two lattice distortion…

We present an extensive overview of the phase diagram, spin-wave excitations, and finite-temperature transitions of the anisotropic-exchange magnets on an ideal nearest-neighbor triangular lattice. We investigate transitions between five…

Strongly Correlated Electrons · Physics 2022-02-23 P. A. Maksimov , Zhenyue Zhu , Steven R. White , A. L. Chernyshev

Non-collinear two-dimensional triangular lattice antiferromagnets (2D TLAF) are currently an area of very active research due to their unique magnetic properties, which lead to non-trivial quantum effects that experimentally manifest…

Strongly Correlated Electrons · Physics 2018-10-12 J. C. Leiner , Taehun Kim , Kisoo Park , Joosung Oh , T. G. Perring , H. C. Walker , X. Xu , Y. Wang , S. -W. Cheong , Je-Geun Park

The magnetic ground state and the crystalline electric field level scheme of the triangular lattice antiferromagnet KCeO$_2$ are investigated. Below $T_N =$ 300 mK, KCeO$_2$ develops signatures of magnetic order in specific heat…

Magnetic order on the spatially anisotropic triangular lattice of $\alpha$-NaMnO$_2$ is studied via neutron diffraction measurements. The transition into a commensurate, collinear antiferromagnetic ground state with $\mathbf{k}=(0.5, 0.5,…

Strongly Correlated Electrons · Physics 2018-11-14 Rebecca L. Dally , Robin Chisnell , Leland Harriger , Yaohua Liu , Jeffrey W. Lynn , Stephen D. Wilson

We successfully synthesize single crystals of the verdazyl radical $\alpha$-2,3,5-Cl$_3$-V. $Ab$ $initio$ molecular orbital calculations indicate that the two dominant antiferromagnetic interactions, $J_{\rm{1}}$ and $J_{\rm{2}}$ ($\alpha…

Strongly Correlated Electrons · Physics 2017-06-26 Hironori Yamaguchi , Yusuke Tamekuni , Yoshiki Iwasaki , Rei Otsuka , Yuko Hosokoshi , Takanori Kida , Masayuki Hagiwara

The spin-1/2 stacked triangular antiferromagnet CsCu$_{1-x}$Co$_x$Cl$_3$ with $0.015<x<0.032$ undergoes two phase transitions at zero field. The low-temperature phase is produced by the small amount of Co$^{2+}$ doping. In order to…

Strongly Correlated Electrons · Physics 2009-10-31 T. Ono , T. Kato , H. Tanaka , A. Hoser , N. Stusser , U. Schotte

The Heisenberg model on a face center cubic (fcc) lattice is a typical three-dimensional frustrated spin system expected to have magnetization plateaus and supersolid phases. There are model compounds $A_2$CoTeO$_6$ ($A$ = Ca, Sr, Pb) for…

Strongly Correlated Electrons · Physics 2019-04-24 Katsuhiro Morita , Takami Tohyama

The observation of spinon excitations in the $S=\frac{1}{2}$ triangular antiferromagnet Ca$_3$ReO$_5$Cl$_2$ reveals a quasi-one-dimensional (1D) nature of magnetic correlations, in spite of the nominally 2D magnetic structure. This…

Strongly Correlated Electrons · Physics 2022-10-31 S. A. Zvyagin , A. N. Ponomaryov , J. Wosnitza , D. Hirai , Z. Hiroi , M. Gen , Y. Kohama , A. Matsuo , Y. H. Matsuda , K. Kindo

Hexagonal HoMnO$_{3}$ is a frustrated antiferromagnet (T$_{N}$=72 K) ferroelectric (T$_{C}$=875 K) in which these two order parameters are coupled. Our neutron measurements of the spin wave dispersion for the S=2 Mn$^{3+}$ on the layered…

Strongly Correlated Electrons · Physics 2009-11-11 O. P. Vajk , M. Kenzelmann , J. W. Lynn , S. B. Kim , S. -W. Cheong

Frustrated magnetic systems exhibit highly degenerate ground states and strong fluctuations, often leading to new physics. An intriguing example of current interest is the antiferromagnet on a diamond lattice, realized physically in A-site…

Materials Science · Physics 2011-09-21 G. J. MacDougall , D. Gout , J. L. Zarestky , G. Ehlers , A. Podlesnyak , M. A. McGuire , D. Mandrus , S. E. Nagler

Amplitude modes arising from symmetry breaking in materials are of broad interest in condensed matter physics. These modes reflect an oscillation in the amplitude of a complex order parameter, yet are typically unstable and decay into…

Strongly Correlated Electrons · Physics 2018-10-24 Rebecca L. Dally , Yang Zhao , Zhijun Xu , Robin Chisnell , M. B. Stone , Jeffrey W. Lynn , Leon Balents , Stephen D. Wilson

Double perovskites Sr2FeOsO6 and Ca2FeOsO6 show puzzling magnetic properties, the former a low-temperature antiferromagnet while the later a high-temperature insulating ferrimagnet. Here, in order to understand the underlying mechanism, we…

Materials Science · Physics 2015-08-24 Yusheng Hou , Hongjun Xiang , Xingao Gong

Exploration of nontrivial magnetic states induced by strong spin-orbit interaction is a central topic of frustrated magnetism. Extensive studies are concentrated on rare-earth-based magnets and 4d/5d transition metal compounds, which are…

Investigation of materials that exhibit quantum phase transition provides valuable insights into fundamental problems in physics. We present neutron scattering under pressure in a triangular-lattice antiferromagnet which has a quantum…

Novel magnetic phases are expected to occur in highly frustrated spin systems. Here we study the structurally perfect kagom\'e antiferromagnet CdCu$_3$(OH)$_6$(NO$_3$)$_2\cdot$H$_2$O by magnetization, magnetic torque, and heat capacity…

Strongly Correlated Electrons · Physics 2017-03-29 Ryutaro Okuma , Takeshi Yajima , Daisuke Nishio-Hamane , Tsuyoshi Okubo , Zenji Hiroi

The magnetic ground state of geometrically frustrated antiferromagnet attracts great research interests due to the possibility to realize novel quantum magnetic state such as a quantum spin liquid. Here we present a comprehensive magnetic…

Strongly Correlated Electrons · Physics 2025-06-09 Feihao Pan , Nan Zhao , Songnan Sun , Chenglin Shang , Peng Cheng , Jieming Sheng , Liusuo Wu

In our study, we conduct magnetization and heat capacity measurements to investigate field induced magnetic phase transitions within the newly synthesized compound K2Ni2(SeO3)3, a spin-1 dimer system arranged on a triangular lattice. From…

Strongly Correlated Electrons · Physics 2024-05-30 Lei Yue , Ziyou Lu , Kun Yan , Le Wang , Shu Guo , Ruixin Guo , Peng Chen , Xiaobin Chen , Jia-Wei Mei

A layered triangular lattice with spin-1/2 ions is an ideal platform to explore highly entangled exotic states like quantum spin liquid (QSL). Here, we report a systematic in-field neutron scattering study on a perfect two-dimensional…

Strongly Correlated Electrons · Physics 2024-07-18 Tao Xie , Jie Xing , S. E. Nikitin , S. Nishimoto , M. Brando , P. Khanenko , J. Sichelschmidt , L. D. Sanjeewa , Athena S. Sefat , A. Podlesnyak

We investigate the magnetic ground state of CuNdO$_2$, which is a delafossite with a triangular lattice of magnetic Nd$^{3+}$ ions that are well separated by non-magnetic Cu spacer layers. From inelastic neutron scattering measurements of…

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