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By combining neutron four-circle diffraction and polarized neutron diffraction techniques we have determined the complex spin structures of a multiferroic, YMn2O5, that exhibits two ferroelectric phases at low temperatures. The obtained…

In this paper, we report on the magnetic and magnetocaloric features of Dy-substituted YMn$_2$O$_5$ (Y$_{1-x}$Dy$_x$Mn$_2$O$_5$) with $x=$ 0.6, 0.8, and 1 series elaborated by sol-gel method. X-ray diffraction and Raman measurements attest…

Materials Science · Physics 2024-01-04 H. Chouaibi , S. Mansouri , S. Aitjmal , M. Balli , O. Chdil , M. Abbasi Eskandari , S. H. Bukhari , P. Fournier

Neutron diffraction measurements under high magnetic fields have been performed for the multiferroic compound HoMn$_{2}$O$_{5}$. At zero field, high-temperature incommensurate magnetic (HT-ICM) -- commensurate magnetic (CM) --…

Strongly Correlated Electrons · Physics 2007-05-23 H. Kimura , Y. Kamada , Y. Noda , K. Kaneko , N. Metoki , K. Kohn

We have studied the crystal and magnetic structures of the magnetoelectric materials RMn2O5 (R = Tb, Ho, Dy) using neutron diffraction as a function of temperature. All three materials display incommensurate antiferromagnetic ordering below…

Strongly Correlated Electrons · Physics 2009-11-11 G. R. Blake , L. C. Chapon , P. G. Radaelli , S. Park , N. Hur , S-W. Cheong , J. Rodriguez-Carvajal

Magnetic structure evolution of multiferroic hexagonal $YMn_{1-x}Fe_{x}O_{3}$ (${x} = 0, 0.05,$ and $0.1$) has been studied by carrying out detailed temperature-dependent neutron diffraction at zero- and 5T-fields. Thermodynamic data…

Materials Science · Physics 2017-07-26 Sonu Namdeo , S. S. S. Rao , S. D. Kaushik , V. Siruguri , A. M. Awasthi

We have successfully induced multiferroic behavior in the A-type antiferromagnet SmMnO3 by the substitution of Y at the Sm site. A magnetic transition develops at 24 K for Sm1-xYxMnO3 (x=0.4,0.5) which is not present in the parent compound.…

Strongly Correlated Electrons · Physics 2011-05-17 D. O'Flynn , C. V. Tomy , M. R. Lees , A. Daoud-Aladine , G. Balakrishnan

We have determined the magnetic structure of the low-temperature incommensurate phase of multiferroic YMn2O5 using single-crystal neutron diffraction. By employing corepresentation analysis, we have ensured full compliance with both…

Materials Science · Physics 2009-11-13 P. G. Radaelli , C. Vecchini , L. C. Chapon , P. J. Brown , S. Park , S-W. Cheong

X-ray resonant scattering has been used to measure the magnetic order of the Dy ions below 40K in multiferroic DyMn$_{2}$O$_{5}$. The magnetic order has a complex behaviour. There are several different ordering wavevectors, both…

Strongly Correlated Electrons · Physics 2008-04-21 R. A. Ewings , A. T. Boothroyd , D. F. McMorrow , D. Mannix , H. C. Walker , B. M. R. Wanklyn

We report the observation of a magnetic polarization of the O\,$2p$-states in YMn$_2$O$_5$ through the use of soft X-ray resonant scattering at the oxygen $K$-edge. Remarkably, we find that the temperature dependence of the integrated…

Strongly Correlated Electrons · Physics 2015-03-19 S. Partzsch , S. B. Wilkins , J. P. Hill , E. Schierle , E. Weschke , D. Souptel , B. Büchner , J. Geck

We have investigated the effects of substituting In for Mn on the antiferromagnetic phase transition in YMnO3 using magnetic, dielectric, and specific heat measurements. We prepared a set of isostructural phase pure hexagonal…

Materials Science · Physics 2015-05-14 A. Dixit , Andrew E. Smith , M. A. Subramanian , G. Lawes

The crystal growth and the structural, transport and magnetic properties of the magnetically frustrated YbMn$_2$Sb$_2$ single crystals are reported. The crystals show a trigonal symmetry (space group $P\bar{3}m1$), where corrugated…

Atomic Physics · Physics 2020-04-27 J. Munevar , F. R. Arantes , L. Mendonça-Ferreira , M. A. Avila , R. A. Ribeiro

Polarized neutron diffraction experiments have been performed on multiferroic materials $R$Mn$_{2}$O$_{5}$ ($R=$Ho, Er) under electric fields in the ferroelectric commensurate (CM) and the low-temperature incommensurate (LT-ICM) phases,…

Strongly Correlated Electrons · Physics 2015-05-13 S. Wakimoto , H. Kimura , M. Fukunaga , K. Nishihata , M. Takeda , K. Kakurai , Y. Noda , Y. Tokura

The electric polarization and its magnetic origins in multiferroic RMn2O5, where R is rare-earth ion, are still issues under debate. In this work, the temperature-dependent electric polarization of DyMn2O5, the most attractive member of…

Materials Science · Physics 2014-02-06 Z. Y. Zhao , M. F. Liu , X. Li , L. Lin , Z. B. Yan , S. Dong , J. -M. Liu

The mixed-valent multiferroic compound CaMn7O12 is studied for its magnetic and electric properties. The compound undergoes magnetic ordering below 90 K with a helimagnetic structure followed by a low temperature magnetic anomaly observed…

Strongly Correlated Electrons · Physics 2013-07-23 J. Sannigrahi , S. Chattopadhyay , D. Dutta , S. Giri , S. Majumdar

The low-temperature ferroelectric polarization of multiferroic $YMn_2O_5$ is completely reversed at a critical pressure of 10 kbar and the phase transition from the incommensurate to the commensurate magnetic phase is induced by pressures…

Strongly Correlated Electrons · Physics 2009-11-13 Rajit P. Chaudhury , Clarina R. dela Cruz , Bernd Lorenz , Yanyi Sun , Ching-Wu Chu , S. Park , Sang-W. Cheong

The polycrystalline co-doped samples of Sm0.5Y0.5Fe0.58Mn0.42O3 were prepared by solid-state reaction route and its various physical properties with their correlations have been investigated. The dc magnetization measurements on the sample…

We have performed simultaneous measurements of magnetic chirality by using polarized neutrons and electric polarization along the b-axis of single crystals of YMn$^{4+}$(Mn$_{1-x}$Ga$_{x}$)$^{3+}$O$_{5}$ with $x=0.047$ and 0.12, in which…

Materials Science · Physics 2015-06-17 S. Wakimoto , H. Kimura , Y. Sakamoto , M. Fukunaga , Y. Noda , M. Takeda , K. Kakurai

A scheme for making ab-initio calculations of the dynamic paramagnetic spin susceptibilities of solids at finite temperatures is described. It is based on Time-Dependent Density Functional Theory and employs an electronic multiple…

Strongly Correlated Electrons · Physics 2007-05-23 J. B. Staunton , J. Poulter , B. Ginatempo , E. Bruno , D. D. Johnson

The results of ac and dc magnetization and heat capacity measurements as a function of temperature (T = 1.8 to 300 K) are reported for a quasi-one-dimensional compound, Ca$_3$CuMnO$_6$, crystallizing in a triclinically distorted…

Strongly Correlated Electrons · Physics 2009-11-10 Kausik Sengupta , S. Rayaprol , K. K. Iyer , E. V. Sampathkumaran

We report temperature (T) dependence of dc magnetization, electrical resistivity (rho(T)), and heat-capacity of rare-earth (R) compounds, Gd3RuSn6 and Tb3RuSn6, which are found to crystallize in the Yb3CoSn6-type orthorhombic structure…

Strongly Correlated Electrons · Physics 2017-06-28 Sanjay K Upadhyay , Kartik K Iyer , E. V. Sampathkumaran
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