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We present a theory of the local field corrections to the spontaneous emission rate for the array of silicon nanocrystals in silicon dioxide. An analytical result for the Purcell factor is obtained. We demonstrate that the local-field…

Optics · Physics 2015-06-23 Alexander N. Poddubny

We analytically study the spontaneous emission of a single optical dipole emitter in the vicinity of a plasmonic nanoshell, based on the Lorenz-Mie theory. We show that the fluorescence enhancement due to the coupling between optical…

The emission by an initially completely inverted atomic ensemble in the long-wavelength regime is simultaneously enhanced by both collective effects (Dicke effect) and dielectric environments (Purcell effect), thus giving rise to a combined…

Quantum Physics · Physics 2018-04-05 Sebastian Fuchs , Stefan Yoshi Buhmann

Interaction between plasmonic nanostructures and molecules is modeled based on the concept of quantized optical cavity for surface enhanced Raman scattering process. We have found that the background emission from plasmonic nanostructures…

Optics · Physics 2017-03-22 Yuqing Cheng , Jingyi Zhao , Te Wen , Guantao Li , Jianning Xu , Qihuang Gong , Guowei Lu

The altered spontaneous emission of an emitter near an arbitrary body can be elucidated using an energy balance of the electromagnetic field. From a classical point of view it is trivial to show that the field scattered back from any body…

Optics · Physics 2015-06-04 Murugesan Venkatapathi

Recently the photonic golden rule, which predicts that the spontaneous emission rate of an atom depends on the projected local density of states (LDOS), was shown to fail in an optical medium with a linear gain amplifier. We present a…

Optics · Physics 2024-01-31 Juanjuan Ren , Sebastian Franke , Becca VanDrunen , Stephen Hughes

Plasmons can be excited during photoemission and produce spectral photoelectron features that yield information on the nanoscale optical response of the probed materials. However, these so-called plasmon satellites have so far been observed…

Mesoscale and Nanoscale Physics · Physics 2023-09-06 P. A. D. Gonçalves , F. Javier García de Abajo

Colour centres in diamond are promising candidates as a platform for quantum technologies and biomedical imaging based on spins and/or photons. Controlling the emission properties of colour centres in diamond is a key requirement for…

Multilayer hyperbolic metamaterials consisting of alternating metal and dielectric layers have important applications in spontaneous emission enhancement. In contrast to the conventional choice of at least dozens of layers in multilayer…

Optics · Physics 2020-10-15 Ling Li , Changjun Min , Xiaocong Yuan

By means of quantum tensor network calculations, we investigate the large Purcell effect experienced by an organic molecule placed in the vicinity of a plasmonic nanostructure. In particular, we consider a donor-{\pi} bridge-acceptor dye at…

Mesoscale and Nanoscale Physics · Physics 2020-12-17 D. Zhao , R. E. F. Silva , C. Climent , J. Feist , A. I. Fernández-Domínguez , F. J. García-Vidal

The enhancement of two-photon spontaneous emission (2PSE) from trivalent and divalent rare earth ions in proximity to graphene and graphene nanoribbons is calculated for achievable experimental conditions using a combination of finite…

Mesoscale and Nanoscale Physics · Physics 2023-05-24 Colin Whisler , Gregory Holdman , D. D. Yavuz , Victor W. Brar

The radiative lifetime of molecules or atoms can be increased by placing them within a tuned conductive cavity that inhibits spontaneous emission. This was examined as a possible means of enhancing three-body, singlet-based upconversion,…

Atomic and Molecular Clusters · Physics 2017-04-11 Michael D. LaCount , Mark T. Lusk

Subwavelength periodic confinement can collectively and selectively enhance local light intensity and enable control over the photo-induced phase transformations at the nanometer scale. Standard nanofabrication process can result in…

We observe a sixfold Purcell broadening of the D$_2$ line of an optically trapped $^{87}\text{Rb}$ atom strongly coupled to a fiber cavity. Under external illumination by a near-resonant laser, up to $90\%$ of the atom's fluorescence is…

The spontaneous emission rate of dipole emitters close to plasmonic dimers are theoretically studied within a nonlocal hydrodynamic model. A nonlocal model has to be used since quantum emitters in the immediate environment of a metallic…

We demonstrate that the emission of light by fluorescent molecules in the proximity of periodic arrays of nanoantennas or plasmonic crystals can be strongly modified when the arrays are covered by a dielectric film. The coupling between…

Optics · Physics 2009-01-14 G. Vecchi , V. Giannini , J. Gómez Rivas

Recent developments in thin-film fabrication and processing open up interesting possibilities for both established and emerging optics technologies. There, one of the key questions requiring more complete understanding is by how much one…

Optics · Physics 2025-01-03 Pyry Kivisaari , Mikko Partanen , Jani Oksanen

One central theme in quantum photonics is tailoring the interactions between atoms/spins and their electromagnetic (EM) environments. Considerable effort has focused on engineering spontaneous emission by shaping EM environments, known as…

Quantum Physics · Physics 2026-05-20 Wenbo Sun , Shoaib Mahmud , Wei Zhang , Runwei Zhou , Pronoy Das , Dan Jiao , Zubin Jacob

Excitons spread through diffusion and interact through exciton-exciton annihilation. Nanophotonics can counteract the resulting decrease in light emission. However, conventional enhancement treats emitters as immobile and noninteracting.…

The interaction of single quantum emitters with an optical cavity enables the realization of efficient spin-photon interfaces, an essential resource for quantum networks. The dynamical control of the spontaneous emission rate of quantum…