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Related papers: Quantitative cw Overhauser DNP Analysis of Hydrati…

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We report achieving enhanced nuclear magnetization in a magnetic resonance force microscope experiment at 0.6 tesla and 4.2 kelvin using the dynamic nuclear polarization (DNP) effect. In our experiments a microwire coplanar waveguide…

Dynamic nuclear polarization (DNP) is an NMR sensitivity enhancement technique that mediates polarization transfer from unpaired electrons to NMR-active nuclei. Despite its success in elucidating important structural information on…

In III-V semiconductor nano-structures the electron and nuclear spin dynamics are strongly coupled. Both spin systems can be controlled optically. The nuclear spin dynamics is widely studied, but little is known about the initialization…

Mesoscale and Nanoscale Physics · Physics 2018-04-05 M. Manca , G. Wang , T. Kuroda , S. Shree , A. Balocchi , P. Renucci , X. Marie , M. V. Durnev , M. M. Glazov , K. Sakoda , T. Mano , T. Amand , B. Urbaszek

Dynamic Nuclear Polarization (DNP) is transforming NMR and MRI by significantly enhancing sensitivity through the transfer of polarization from electron spins to nuclear spins via microwave irradiation. However, the use of monochromatic…

Quantum Physics · Physics 2024-10-28 Mayur Jhamnani , Sajith V Sadasivan , Sheetal Kumar Jain , Asif Equbal

Dynamic nuclear polarization (DNP) is an important method to enhance the limited sensitivity of nuclear magnetic resonance (NMR). Using the existing mechanisms such as Overhauser DNP (ODNP) is still difficult to achieve significant…

Chemical Physics · Physics 2025-03-31 Maria Grazia Concilio , Yiwen Wang , Linjun Wang , Xueqian Kong

Nuclear spin coherence and relaxation dynamics of all constituent isotopes of an n-doped CdTe/(Cd,Mg)Te quantum well structure are studied employing optically detected nuclear magnetic resonance. Using time-resolved pump-probe Faraday…

Mesoscale and Nanoscale Physics · Physics 2019-04-04 E. Evers , T. Kazimierczuk , F. Mertens , D. R. Yakovlev , G. Karczewski , T. Wojtowicz , J. Kossut , M. Bayer , A. Greilich

The significance of nuclear spin polarisation in time-resolved optical studies of III-V semiconductors is addressed. Electron Larmor beats in pump-probe reflectivity from a GaAs/AlGaAs quantum well show Overhauser shift of 0.7 T due to…

Mesoscale and Nanoscale Physics · Physics 2009-10-31 A. Malinowski , R. T. Harley

Dynamic nuclear polarisation (DNP) refers to a class of techniques used to increase the signal in nuclear magnetic resonance measurements by transferring spin polarisation from ensembles of highly polarised electrons to target nuclear…

Quantum Physics · Physics 2020-12-24 L. T. Hall , D. A. Broadway , A. Stacey , D. A. Simpson , J-P. Tetienne , L. C. L. Hollenberg

Nuclear electric resonance (NER) is based on nuclear magnetic resonance mediated by spatial oscillations of electron spin domains excited by a radio frequency (RF) electric field, and it allows us to investigate the spatial distribution of…

Mesoscale and Nanoscale Physics · Physics 2012-10-25 S. Watanabe , G. Igarashi , N. Kumada , Y. Hirayama

We report on the direct measurement of the electron spin splitting and the accompanying nuclear Overhauser (OH) field, and thus the underlying nuclear spin polarization (NSP) and fluctuation bandwidth, in a single InAs quantum dot under…

Mesoscale and Nanoscale Physics · Physics 2021-01-04 Aaron M. Ross , Allan S. Bracker , Michael K. Yakes , Daniel Gammon , L. J. Sham , Duncan G. Steel

Dynamic nuclear polarization (DNP) is a method of enhancing NMR signals via the transfer of polarization from electron spins to nuclear spins using on-resonance microwave (MW) irradiation. In most cases, monochromatic continuous-wave (MCW)…

Chemical Physics · Physics 2022-11-17 Daphna Shimon , Kelly A. Cantwell , Linta Joseph , Chandrasekhar Ramanathan

In dynamic nuclear polarization (DNP) experiments, the compound is driven out-of-equilibrium by microwave (MW) irradiation of the radical electron spins. Their stationary state has been recently probed via electron double resonance (ELDOR)…

Strongly Correlated Electrons · Physics 2017-02-28 Filippo Caracciolo , Marta Filibian , Pietro Carretta , Alberto Rosso , Andrea De Luca

Nuclear spin optical rotation (NSOR) is a recently developed technique for detection of nuclear magnetic resonance via rotation of light polarization, instead of the usual long-range magnetic fields. NSOR signals depend on hyperfine…

Chemical Physics · Physics 2012-02-21 Junhui Shi , Suvi Ikäläinen , Juha Vaara , Michael V. Romalis

The Knight shift of Ga-71 nuclei is measured in two different electron-doped multiple quantum well samples using optically pumped NMR. These data are the first direct measurements of the electron spin polarization,…

Mesoscale and Nanoscale Physics · Physics 2009-10-31 P. Khandelwal , N. N. Kuzma , S. E. Barrett , L. N. Pfeiffer , K. W. West

We introduce a coarse-grained deep neural network model (CG-DNN) for liquid water that utilizes 50 rotational and translational invariant coordinates, and is trained exclusively against energies of ~30,000 bulk water configurations. Our…

One of solution-state Nuclear Magnetic Resonance (NMR)'s main weaknesses, is its relative insensitivity. J-driven Dynamic Nuclear Polarization (JDNP) was recently proposed for enhancing the sensitivity of solution-state NMR, by bypassing…

Chemical Physics · Physics 2023-08-07 Maria Grazia Concilio , Lucio Frydman

Dynamic nuclear polarization (DNP) is a promising strategy for generating a significantly increased non-thermal spin polarization in nuclear magnetic resonance (NMR) applications thereby circumventing the need for strong magnetic fields.…

Quantum Physics · Physics 2015-07-15 Alexander Karabanov , Daniel Wisniewski , Igor Lesanovsky , Walter Köckenberger

Dynamic nuclear polarization (DNP) using the boron vacancy ($\mathrm{V_B^-}$) in hexagonal boron nitride (hBN) has gained increasing attention. Understanding this DNP requires systematically investigating the optically detected magnetic…

Para- and ortho- isomers of water have different chemical and physical properties. Excitations by magnetic field, laser emission or hydrodynamic cavitation are reported to change energetic levels and spin configurations of water molecules…

Chemical Physics · Physics 2022-05-18 Serge Kernbach

We show that optical pumping of electron spins in individual InGaAs quantum dots leads to strong nuclear polarisation that we measure via the Overhauser shift (OHS) in magneto-photoluminescence experiments between 0 and 4T. We find a…

Mesoscale and Nanoscale Physics · Physics 2009-11-11 P. -F. Braun , B. Urbaszek , T. Amand , X. Marie , O. Krebs , B. Eble , A. Lemaitre , P. Voisin